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Near bandgap second-order nonlinear optical characteristics of MoS2 monolayer transferred on transparent substrates

Daniel J. Clark、Chinh Tam Le、V. Senthilkumar 等 10 位作者2015-09-28Applied Physics Letters

We have investigated the second-order nonlinear optical (NLO) properties of CVD-grown MoS2 monolayer (ML) transferred onto transparent substrates such as fused silica and polyethylene terephthalate. The physical properties of the transferred MLs were characterized by optical and NLO methods. We measured the second-ord…

Perovskite Materials and Applications2D Materials and ApplicationsPlasmonic and Surface Plasmon Research

Radical Cation–Anion Coupling‐Induced Work Function Tunability in Anionic Conjugated Polyelectrolytes

Jong‐Hoon Lee、Byoung Hoon Lee、Song Yi Jeong 等 7 位作者2015-09-28Advanced Energy Materials

By coating conjugated polyelectrolytes (CPEs) on metals, the work function (WF) of metals can be tuned by electric dipoles formed through the self‐assembly of cation–anion pairs on the side chains of CPEs. Recently, it has been reported that a pertinent oxidative doping of anionic CPEs results in a reversed direction…

Organic Electronics and PhotovoltaicsPerovskite Materials and ApplicationsConducting polymers and applications

Mesoscopic quantum emitters from deterministic aggregates of conjugated polymers

Thomas Stangl、Philipp Wilhelm、Klaas Remmerssen 等 6 位作者2015-09-28Proceedings of the National Academy of Sciences

An appealing definition of the term "molecule" arises from consideration of the nature of fluorescence, with discrete molecular entities emitting a stream of single photons. We address the question of how large a molecular object may become by growing deterministic aggregates from single conjugated polymer chains. Eve…

Organic Electronics and PhotovoltaicsSpectroscopy and Quantum Chemical StudiesLuminescence and Fluorescent Materials

Ternary Phase-Separation Investigation of Sol-Gel Derived Silica from Ethyl Silicate 40

Shengnan Wang、David Wang、Simon Smart 等 4 位作者2015-09-28Scientific Reports

A ternary phase-separation investigation of the ethyl silicate 40 (ES40) sol-gel process was conducted using ethanol and water as the solvent and hydrolysing agent, respectively. This oligomeric silica precursor underwent various degrees of phase separation behaviour in solution during the sol-gel reactions as a funct…

Zeolite Catalysis and SynthesisMesoporous Materials and CatalysisAerogels and thermal insulation

High-TcSuperconductivity at the Interface between theCaCuO2andSrTiO3Insulating Oxides

D. Di Castro、C. Cantoni、F. Ridolfi 等 7 位作者2015-09-28Physical Review Letters

At interfaces between complex oxides it is possible to generate electronic systems with unusual electronic properties, which are not present in the isolated oxides. One important example is the appearance of superconductivity at the interface between insulating oxides, although, until now, with very low T(c). We repor…

Magnetic and transport properties of perovskites and related materialsAdvanced Condensed Matter PhysicsElectronic and Structural Properties of Oxides

Temperature-induced strain and doping in monolayer and bilayer isotopically labeled graphene

Tim Verhagen、Karolina Drogowska、Martin Kalbáč 等 4 位作者2015-09-28Physical Review B

The electronic band structure of graphene is strongly dependent on the amount of strain and/or doping present. We performed a comprehensive study of temperature-dependent strain and doping in isotopically labeled graphene mono- and bilayers on a ${\mathrm{SiO}}_{2}/\mathrm{Si}$ substrate by Raman spectral mapping at w…

Graphene research and applications2D Materials and ApplicationsQuantum and electron transport phenomena

Fluorescence intensity ratio method for temperature sensing

Yuan Zhou、Feng Qin、Yangdong Zheng 等 5 位作者2015-09-28Optics Letters

A thermometry method based on the ratio between the valley intensity formed by fluorescence peak overlap and the peak fluorescence intensity has been developed. Excited by a 405 nm laser, the valley to peak ratio (VPR) of the emissions originating from 5D0 to 7F2 Stark sublevels in Eu3+-doped CaWO4 shows a monotonic c…

Luminescence Properties of Advanced MaterialsSpectroscopy and Laser ApplicationsSolid State Laser Technologies

Protective Effects of Bovine Serum Albumin on Superparamagnetic Iron Oxide Nanoparticles Evaluated in the Nematode Caenorhabditis elegans

Laura Gonzalez-Moragas、Siming Yu、Elisa Carenza 等 5 位作者2015-09-28ACS Biomaterials Science & Engineering

Nanomaterials give rise to unique biological reactivity that needs to be thoroughly investigated. The quest for enhanced magnetic nanomaterials of different shapes, magnetic properties, or surface coatings continues for applications in drug delivery, targeting therapies, biosensing, and magnetic separation. In this co…

Nanoparticles: synthesis and applicationsGenetics, Aging, and Longevity in Model OrganismsSelenium in Biological Systems

A soft biomolecule actuator based on a highly functionalized bacterial cellulose nano-fiber network with carboxylic acid groups

Fan Wang、Jin‐Han Jeon、Sukho Park 等 6 位作者2015-09-28Soft Matter

Upcoming human-related applications such as soft wearable electronics, flexible haptic systems, and active bio-medical devices will require bio-friendly actuating materials. Here, we report a soft biomolecule actuator based on carboxylated bacterial cellulose (CBC), ionic liquid (IL), and poly (3,4-ethylenedioxythioph…

Advanced Sensor and Energy Harvesting MaterialsAdvanced Cellulose Research StudiesDielectric materials and actuators

Origin of Noise in Layered MoTe2 Transistors and its Possible Use for Environmental Sensors

Yen‐Fu Lin、Yong Xu、Che‐Yi Lin 等 8 位作者2015-09-28Advanced Materials

Low-frequency current fluctuations are monitored and the mechanism of electric noise investigated in layered 2H-type α-molybdenum ditelluride transistors. The charge transport mechanism of electric noise in atomically thin transition-metal dichalcogenides is studied under different environments; the development of a n…

Graphene research and applications2D Materials and ApplicationsMXene and MAX Phase Materials

DGDFT: A massively parallel method for large scale density functional theory calculations

Wei Hu、Lin Lin、Chao Yang2015-09-28The Journal of Chemical Physics

We describe a massively parallel implementation of the recently developed discontinuous Galerkin density functional theory (DGDFT) method, for efficient large-scale Kohn-Sham DFT based electronic structure calculations. The DGDFT method uses adaptive local basis (ALB) functions generated on-the-fly during the self-con…

Physics of Superconductivity and MagnetismGraphene research and applications2D Materials and Applications

A heat-switch-based electrocaloric cooler

Y. D. Wang、Sylvia Smullin、Martin J. Sheridan 等 6 位作者2015-09-28Applied Physics Letters

A heat-switch-based electrocaloric cooler is reported in this letter. The device consists of two silicon heat switches and an electrocaloric module based on BaTO3 multilayer capacitors (MLCs). To operate the cooler, the heat switches are actuated synchronously with the application of electric fields across the MLCs. H…

Ferroelectric and Piezoelectric MaterialsMultiferroics and related materialsAcoustic Wave Resonator Technologies

TEMPO-Oxidized Nanofibrillated Cellulose as a High Density Carrier for Bioactive Molecules

Ramon Weishaupt、Gilberto Siqueira、Mark Schubert 等 9 位作者2015-09-28Biomacromolecules

Controlled and efficient immobilization of specific biomolecules is a key technology to introduce new, favorable functions to materials suitable for biomedical applications. Here, we describe an innovative and efficient, two-step methodology for the stable immobilization of various biomolecules, including small peptid…

Advanced Cellulose Research Studiesbiodegradable polymer synthesis and propertiesElectrospun Nanofibers in Biomedical Applications

Atomic Disorders Induced by Silver and Magnesium Ion Migrations Favor High Thermoelectric Performance in α‐MgAgSb‐Based Materials

Dandan Li、Huaizhou Zhao、Shanming Li 等 12 位作者2015-09-28Advanced Functional Materials

Thermoelectric devices can directly convert thermal energy to electricity or vice versa with the efficiency being determined by the materials’ dimensionless figure of merit ( ZT ). Since the revival of interests in the last decades, substantial achievements have been reached in search of high‐performance thermoelectri…

Advanced Thermoelectric Materials and DevicesSuperconductivity in MgB2 and AlloysThermal Expansion and Ionic Conductivity

Tetragonal magnetic phase inBa1−xKxFe2As2from x-ray and neutron diffraction

Jared M. Allred、Sevda Avcı、Duck Young Chung 等 11 位作者2015-09-28Physical Review B

Combined neutron and x-ray diffraction experiments demonstrate the formation of a low-temperature minority magnetic tetragonal phase in ${\mathrm{Ba}}_{0.76}{\mathrm{K}}_{0.24}{\mathrm{Fe}}_{2}{\mathrm{As}}_{2}$ in addition to the majority magnetic, orthorhombic phase. The coincident enhancement in the magnetic ($\fra…

Corporate Taxation and AvoidanceIron-based superconductors researchIntellectual Capital and Performance Analysis

Ag@Au core-shell dendrites: a stable, reusable and sensitive surface enhanced Raman scattering substrate

Hong Yin、Zhao Yang Chen、Yong Zhao 等 10 位作者2015-09-28Scientific Reports

Surface enhanced Raman scattering (SERS) substrate based on fabricated Ag@Au core-shell dendrite was achieved. Ag dendrites were grown on Si wafer by the hydrothermal corrosion method and Au nanofilm on the surface of Ag dendritic nanostructure was then fabricated by chemical reduction. With the help of sodium borohyd…

Gold and Silver Nanoparticles Synthesis and ApplicationsAdvanced biosensing and bioanalysis techniquesNanocluster Synthesis and Applications

Reconfigurable Photonic Capsules Containing Cholesteric Liquid Crystals with Planar Alignment

Sang Seok Lee、Su Kyung Kim、Su Kyung Kim 等 7 位作者2015-09-28Angewandte Chemie International Edition

Cholesteric liquid crystals (CLCs) reflect selected wavelengths of light owing to their periodic helical structures. The encapsulation of CLCs leads to photonic devices that can be easily processed and might be used as stand-alone microsensors. However, when CLCs are enclosed by polymeric membranes, they usually lose…

Liquid Crystal Research AdvancementsAdvanced Materials and MechanicsElectrowetting and Microfluidic Technologies

Magnetoelectric Coupling Induced by Interfacial Orbital Reconstruction

Bin Cui、Cheng Song、Haijun Mao 等 9 位作者2015-09-28Advanced Materials

Reversible orbital reconstruction driven by ferroelectric polarization modulates the magnetic performance of model ferroelectric/ferromagnetic heterostructures without onerous limitations. Mn-d(x2-y2) orbital occupancy and related interfacial exotic magnetic states are enhanced and weakened by negative and positive el…

Magnetic and transport properties of perovskites and related materialsMultiferroics and related materialsAdvanced Condensed Matter Physics

Thermal conductivity of silicon nitride membranes is not sensitive to stress

Hossein Ftouni、Christophe Blanc、Dimitri Tainoff 等 9 位作者2015-09-28Physical Review B

We have measured the thermal properties of suspended membranes from 10 to 300 K for two amplitudes of internal stress (about 0.1 and 1 GPa) and for two different thicknesses (50 and 100 nm). The use of the original $3\ensuremath{\omega}$-Volklein method has allowed the extraction of both the specific heat and the ther…

Thermal properties of materialsMechanical and Optical ResonatorsQuantum Electrodynamics and Casimir Effect

Interfacial Donor–Acceptor Engineering of Nanofiber Materials To Achieve Photoconductivity and Applications

Ling Zang2015-09-28Accounts of Chemical Research

Self-assembly of π-conjugate molecules often leads to formation of well-defined nanofibril structures dominated by the columnar π-π stacking between the molecular planes. These nanofibril materials have drawn increasing interest in the research frontiers of nanomaterials and nanotechnology, as the nanofibers demonstra…

Conducting polymers and applicationsMolecular Junctions and NanostructuresLuminescence and Fluorescent Materials