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Isolation and characterization of the principal kinetic product in the preparation of a sterically hindered tetra-arylporphyrin: X-ray structure of a bis(dipyrromethene) complex of zinc, Zn II (C 22 H 13 Cl 4 N 2 ) 2 · toluene

Craig L. Hill、Michael M. Williamson1985-01-01Journal of the Chemical Society Chemical Communications

The principal kinetic product in the Rothemund template synthesis of sterically hindered tetra-arylporphyrins is not the metalloporphyrin complex but the bis(dipyrromethene) complex; the latter has been isolated from a typical porphyrin preparation, that of tetrakis(2,6-dichlorophenyl)porphyrin, and characterized by u…

Porphyrin and Phthalocyanine ChemistryMetal-Catalyzed Oxygenation MechanismsSurface Chemistry and Catalysis

Structure–property correlations in some nematic main–chain polyesters

A. Blumstein、M. M. Gauthier、O. Thomas 等 4 位作者1985-01-01Faraday Discussions of the Chemical Society

The homologous series of thermotropic nematic main-chain polyesters [graphic omitted] has been investigated. In the case of even values of n, a smectic phase appears at n= 18. An odd–even oscillation of nematic order parameters associated with the mesogen is observed near the clearing temperature, Tc. At the same time…

Liquid Crystal Research AdvancementsSurfactants and Colloidal SystemsAdvanced Materials and Mechanics

Structural analysis of liquid formamide

Michihiro Miyake、Osamu Kaji、Nobuhiro Nakagawa 等 4 位作者1985-01-01Journal of the Chemical Society Faraday Transactions 2 Molecular and Chemical Physics

The structure of liquid formamide has been examined by X-ray analysis. It is concluded that there are distorted ring dimers which consist of hydrogen-bonded formamide molecules in the liquid state. The most likely model is similar to the crystal structure of formamide.

Liquid Crystal Research AdvancementsSurfactants and Colloidal Systems

Kinetics and mechanism of the reactions of PH3 with O(3 P) and N(4 S) atoms

Peter A. Hamilton、Timothy P. Murrells1985-01-01Journal of the Chemical Society Faraday Transactions 2 Molecular and Chemical Physics

The reactions of ground-state oxygen and nitrogen atoms with phosphine have been studied using a discharge-flow system with detection of both free-radical and molecular species by molecular-beam sampling mass spectrometry. By observing the decay of PH3 in an excess of O, the rate constant for the reaction O + PH3 [gra…

Atmospheric chemistry and aerosolsCatalytic Processes in Materials ScienceCatalysis and Oxidation Reactions

Pyridine-metal complexes

Piotr Tomasik、Zbigniew Ratajewicz、George R. Newkome 等 4 位作者1985-01-01Wiley eBooks

Essentials of Coordination Chemistry. Sigma Pyridine Coordination Compounds with Nontransition Metals. Sigma Pyridine Coordination Compounds with Transition Metals. Coordination Compounds of Metals with Pyridine--l----Oxides. Pi--Coordination Compounds of Pyridine with Metals. Pyridine Intercalation Compounds. Clathra…

Solid-state spectroscopy and crystallography

Frustration in polymers

M. Kléman1985-01-01Journal de Physique Lettres

The local configuration of polymers results from a competition between entropy effects and attractive forces which provide a high density. The resulting frustration is studied geometrically in a curved space representation reminiscent of the curved space representation for blue phases. Within this frame work, we study…

Liquid Crystal Research AdvancementsMaterial Dynamics and PropertiesSurfactants and Colloidal Systems

Fatigue Properties of Type 304 Stainless Steel in High Pressure Hydrogen at Room Temperature

Seiji Fukuyama、Kiyoshi Yokogawa、Kiyokatsu Kudo 等 4 位作者1985-01-01Transactions of the Japan Institute of Metals

The fatigue properties of the soluted and the sensitized type 304 stainless steel were investigated in high pressure hydrogen up to 4.0 MPa at room temperature. It is found that both the number of cycles to failure and the fatigue limits of the soluted and the sensitized steel decreased with increasing hydrogen pressu…

Microstructure and Mechanical Properties of SteelsHydrogen embrittlement and corrosion behaviors in metalsMaterial Properties and Failure Mechanisms

Electron optical synthesis and optimization

M. Szilágyi1985-01-01Proceedings of the IEEE

A novel approach to electron/ion optical synthesis and optimization is presented. Low-aberration field distributions are sought by dynamic programming or optimal control procedures in the form of continuous curves constructed of cubic splines. A very simple algorithm is proposed for the reconstruction of the electrode…

Advanced Electron Microscopy Techniques and ApplicationsAdvancements in Photolithography TechniquesElectron and X-Ray Spectroscopy Techniques

Tuning of reactivity in epoxidation of alkenes by iron and ruthenium complexes associated to non-porphyrinic ligands

CHRISTIAN ESKENAZI、G.G.A. Balavoine、Florent Meunier 等 4 位作者1985-01-01Journal of the Chemical Society Chemical Communications

RuCl3·n(H2O) or FeSO4 associated with bipyridyl or substituted phenanthrolines, catalyse the expoxidation of stilbenes by IO4– or ClO–; using phenanthrolines bearing electron donating or withdrawing groups, it is possible to modulate the reactivity of these systems.

Metal complexes synthesis and propertiesPorphyrin and Phthalocyanine ChemistryMetal-Catalyzed Oxygenation Mechanisms

Surface Analysis of Gas Atomized Ferritic Steel Powder

I. Olefjord、Lars Nyborg1985-01-01Powder Metallurgy

The surface of gas atomized ferritic powder, Fe–25Cr, was studied by ESCA and Auger spectro- scopy. During atomization reaction products are formed on the surface of the powder. Due to the very low oxygen potential in the atomizer only oxides of the strong oxide forming elements Cr, Mn, and Si are formed during coolin…

Fusion materials and technologiesHigh-Temperature Coating BehaviorsNuclear Materials and Properties

Octahedral Compositions of Individual Particles in Smectite-Palygorskite and Smectite-Sepiolite Assemblages

Hélène Paquet、Joëlle Duplay、Marie-Madeleine Valleron-Blanc 等 4 位作者1985-01-01Clay Minerals Society eBooks

Abstract Chemical analyses were carried out on individual particles in <2-μm size fractions to study smectite-palygorskite and smectite-sepiolite assemblages extracted from calcareous and dolomitic continental formations in Provence, southeastern France. A plot of the octahedral composition of 145 individual pa…

Clay minerals and soil interactions

Chapter 9. Conduction electron spin resonance in metallic systems

R.N. Edmonds、M. R. Harrison、Peter P. Edwards1985-01-01Annual Reports Section C (Physical Chemistry)

R. N. Edmonds, M. R. Harrison and P. P. Edwards, Annu. Rep. Prog. Chem., Sect. C: Phys. Chem., 1985, 82, 265 DOI: 10.1039/PC9858200265

Magnetism in coordination complexesLanthanide and Transition Metal ComplexesElectron Spin Resonance Studies

Oxygen exchange and protonation of polyanions: a multinuclear magnetic resonance study of tetradecavanadophosphate(9–) and decavanadate(6–)

Aidan T. Harrison、Oliver W. Howarth1985-01-01Journal of the Chemical Society Dalton Transactions

Unlike decavanadate(6–), tetradecavanadophosphate(9–) shows pH-dependent differential rates of exchange of oxygen with solvent water. If the anion's structure is described as a Keggin-type ‘sphere’ with polar ‘caps,’ then at pH > 5 the caps are kinetically stabilised with respect to the ‘equator,’ whereas at pH < 1 th…

Conducting polymers and applicationsPolyoxometalates: Synthesis and ApplicationsCovalent Organic Framework Applications

Crystal and molecular structures and magnetic properties of tetrameric copper( II ) complexes with 3-hydroxy-5-hydroxymethyl-4-(4′-hydroxy-4′-phenyl-2′-azabut-1′-en-1′-yl)-2-methylpyridine (H 2 L 3 ), [Cu 4 L 3 4 ]·9CH 3 OH and 3-hydroxy-5-hydroxymethyl-4-(4′-hydroxy-3′-methyl-4′-phenyl-2′azabut-1′-en-1′-yl)-2-methylpyridine (H 2 L 1 ), [Cu 4 -L 1 4 ]· 8CH 3 CH 2 OH : two complexes with ferromagnetic ground states

Harald Astheimer、Françoise Nepveu、Leonhard Walz 等 4 位作者1985-01-01Journal of the Chemical Society Dalton Transactions

The crystal and molecular structures of the title compounds [Cu4L34]·9CH3OH (3) and [Cu4L14]·8CH3CH2OH (4) have been determined from single-crystal X-ray diffraction data and refined to final R values of 0.062 (R′= 0.052) using 2 191 independent reflections for (3) and 0.062 (R′= 0.055) using 2 458 independent reflect…

Metal complexes synthesis and propertiesMagnetism in coordination complexesMetal-Catalyzed Oxygenation Mechanisms

An Electrochemical Investigation of Localized Corrosion on Titanium in Chloride Environments

P. McKay、D. B. Mitton1985-01-01CORROSION

Electrochemical methods have been used to study the crevice and pitting corrosion behavior of unalloyed titanium in chloride solutions at elevated temperatures (maximum 150 C). The investigation was focused primarily on crevice corrosion. The techniques which were used included simultaneous measurement of the corrosio…

Corrosion Behavior and InhibitionHydrogen embrittlement and corrosion behaviors in metalsConcrete Corrosion and Durability

Zur Kinetik des Wachstums und der Speicherung von Poly‐D(−)‐3‐hydroxybuttersäure bei Alcaligenes latus

G. Braunegg、B. Bogensberger1985-01-01Acta Biotechnologica

Abstract Alcaligenes latus strain DSM 1123 has been tested for the production of Poly‐D(−3)‐3‐hydroxybutyric acid using sucrose as the only carton source. The strain is capable of accumulating the polymer associated to the growth very fast and lup to high concentrations in the biomass. Alcaligenes lotus seems to be ve…

Enzyme Catalysis and Immobilizationbiodegradable polymer synthesis and propertiesMicrobial Metabolic Engineering and Bioproduction

Infrared mesh filters fabricated by electron-beam lithography

D. M. Byrne、Austin J. Brouns、F. C. Case 等 6 位作者1985-01-01Journal of Vacuum Science & Technology B Microelectronics Processing and Phenomena

Capacitive and inductive infrared mesh filters have been fabricated using electron-beam lithography combined with a lift-off procedure. A single level of PMMA was used to create positive tone patterns while a two-level metal-on-polymer process was used to create negative tone patterns. Resonant structures consisting o…

Photonic and Optical DevicesSemiconductor Lasers and Optical DevicesOptical Coatings and Gratings

Crystal and molecular structures and magnetic properties of bromo(3-dimethylaminopropan-1-olato)copper(II), chloro(3-dimethylaminopropan-1-olato) copper(II), and (3-diethylaminopropan-1-olato)isocyanatocopper(II)

Leonhard Walz、H. Paulus、W. Haase1985-01-01Journal of the Chemical Society Dalton Transactions

The crystal and molecular structures of the title compounds have been determined using three-dimensional X-ray diffractometer data and refined to a final R value of 0.0263 for bromo(3-dimethylaminopropan-1-olato)copper(II)(1), 0.0349 for chloro(3-dimethylaminopropan-1-olato)copper(II)(2), and 0.0268 for (3-diethylamin…

Metal complexes synthesis and propertiesMagnetism in coordination complexesMetal-Catalyzed Oxygenation Mechanisms