Materials Literature
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We investigate the dependence of band dispersion of the quantum spin Hall effect (QSHE) edge states in the Kane-Mele model on crystallographic orientation of the edges. Band structures of the one-dimensional honeycomb lattice ribbons show the presence of the QSHE edge states at all orientations of the edges given suff…
The existence of topological superconductors preserving time-reversal symmetry was recently predicted, and they are expected to provide a solid-state realization of itinerant massless Majorana fermions and a route to topological quantum computation. Their first concrete example, CuxBi2Se3, was discovered last year, bu…
Moving crystal surfaces can undergo step-bunching instabilities, when subject to an electric current. We show analytically that an infinitesimal quantity of a dopant may invert the stability, whatever the sign of the current. Our study is relevant for experimental results [S. S. Kosolobov et al., JETP Lett. 81, 117 (2…
Phase field crystal methodology is applied, for the first time, to study the effect of alloy composition on the clustering behavior of a quenched/aged supersaturated ternary Al alloy system. An analysis of the work of formation is built upon the methodology developed in Fallah {\it et al.} to describe the dislocation-…
We measured the quantum-confined Stark effect (QCSE) of several types of fluorescent colloidal semiconductor quantum dots and nanorods at the single molecule level at room temperature. These measurements demonstrate the possible utility of these nanoparticles for local electric field (voltage) sensing on the nanoscale…
We report a facile strategy to prepare graphene oxide (GO)/polyaniline (PANI) nanocomposite by in situ polymerization with the assistance of supercritical carbon dioxide (SC CO 2 ). The morphology and chemical structure of the synthesized samples were characterized by scanning electron microscopy (SEM), transmission e…
We investigated ultrafast carrier dynamics in graphene with near-infrared transient absorption measurement after intense half-cycle terahertz pulse excitation. The terahertz electric field efficiently drives the carriers, inducing large transparency in the near-infrared region. Theoretical calculations using the Boltz…
We demonstrate that NaAlH(4) confined within the nanopores of a titanium-functionalized metal-organic framework (MOF) template MOF-74(Mg) can reversibly store hydrogen with minimal loss of capacity. Hydride-infiltrated samples were synthesized by melt infiltration, achieving loadings up to 21 wt %. MOF-74(Mg) possesse…
An all electrochemical route to functionalized graphene directly from a graphite electrode is described herein obviating the need for defect inducing oxidative or prolonged sonication treatments. Enhanced electrochemical expansion of graphite is achieved by sequential treatment, beginning with the established method o…
The topical and transdermal delivery of active cosmetic ingredients requires safe and non-toxic means of reaching the target sites without causing any irritation. Preservation of the active ingredients is also essential during formulation, storage and application of the final product. As many biologically active subst…
Polymer–nanoparticle composites play a vital role in ongoing materials development. The behavior of the glass transition of these materials is important for their processing and applications, and also represents a problem of fundamental physical interest. Changes of the polymer glass transition temperature Tg due to n…
Gravimetric, electrochemical impedance spectroscopy (EIS), linear polarization resistance (LPR), and potentiodynamic polarization (PDP) studies were carried out to investigate the comparative corrosion protection efficiency of four condensed uracils (CUs) on mild steel in 1 M HCl. EIS plots indicated that the addition…
A temperature controlled dual water/oil on-off switch is achieved by using a PMMA-b-PNIPAAm block-copolymer coated mesh, determined by the conformational change of the PNIPAAm chain around the lower critical solution temperature (LCST) and also the cooperation between PNIPAAm and PMMA. Water can permeate through the B…
Controlled synthesis of colloidal nanoparticles in organic solutions is among the most intensely studied topics in nanoscience because of the intrinsic advantages in terms of high yield and high uniformity in comparison with aqueous synthesis. However, systematic studies on the formation mechanism of nanoparticles wit…
We use x-ray photon correlation spectroscopy to investigate the structural relaxation process in a metallic glass on the atomic length scale. We report evidence for a dynamical crossover between the supercooled liquid phase and the metastable glassy state, suggesting different origins of the relaxation process across…
Nanoparticles offer potential as drug delivery systems for chemotherapeutics based on certain advantages of molecular drugs. In this study, we report that particle size exerts great influence on the penetration and retention behavior of nanoparticles entering tumors. On comparing gold-coated Au@tiopronin nanoparticles…
Lead chalcogenides have long been used for space-based and thermoelectric remote power generation applications, but recent discoveries have revealed a much greater potential for these materials. This renaissance of interest combined with the need for increased energy efficiency has led to active consideration of therm…
Strain and texture evolution (domain switching) of polycrystalline, ferroelectric BaTiO 3 was investigated in four‐point bending geometry. Lattice strains were measured by in situ synchrotron X ‐ray diffraction to address problems related to modeling the constitutive behavior of highly asymmetric ferroelectrics. The h…
Controlling defect structure in multiwalled carbon nanotube (MWCNT) is essential to realization of MWCNT devices. Here, we show that the diagram of the Raman intensity ratio of the G to D peaks and the G peak width can reveal two damaging stages of MWCNT films. In a transition period, additional peaks appeared in the…
Abstract Direct surface patterning due to photoinduced mass transport in amorphous As‐S‐Se films has been studied. Illumination of the films with two orthogonally (±45°) polarized beam interference pattern causes the formation of surface relief gratings on the films due to lateral mass transport regarding to light pro…