Materials Literature
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Here, we report on a new single-molecule-switching concept based on the coordination-sphere-dependent spin state of Fe(II) species. The perpendicular arrangement of two terpyridine (tpy) ligands within heteroleptic complexes is distorted by the applied electric field. Whereas one ligand fixes the complex in the juncti…
The creation of new organic-inorganic phototransistors with high and broad spectral photosensitivity is reported. The extended charge transport and photoconductivity between the layers in the bilayer structure results in a notable detectivity of over 10(12) Jones and a linear dynamic range of over 100 dB at a broad sp…
The phenomena based on spin-orbit interaction in heavy metal/ferromagnet/oxide structures have been investigated extensively due to their applicability to the manipulation of the magnetization direction via the in-plane current. This implies the existence of an inverse effect, in which the conductivity in such structu…
In p/n photoelectrochemical (PEC) cell systems, a low onset potential for the photoanode, as well as a high photocurrent, are critical for efficient water splitting. Here, we report a Mg-Zr cosubstituted Ta3N5 (Ta3N5:Mg+Zr) photoanode, designed to provide a more negative onset potential for PEC water splitting. The an…
Novel, tough, strong, and self-healable poly-acrylamide (PAAm) gels are fabricated by inducing an appropriate phase-separation structure using a poor solvent. The phase separation induces a gel-glass-like transition of the PAAm gels, providing the gels an anomalously high modulus (211 MPa), fracture stress (7.13 MPa),…
In present study, the microstructure, mechanical and electrochemical properties of aluminum–graphene nanoplatelets (GNPs) composites were investigated before and after extrusion. The contents of graphene nanoplatelets (GNPs) were varied from 0.25 to 1.0 wt.% in aluminum matrix. The composites were fabricated thorough…
Formamidinium lead triiodide (HC(NH 2 ) 2 PbI 3 or FAPbI 3 ) is gaining increasing interest in the field of mesoscopic perovskite solar cells (PSCs) for its broader light absorption compared with the more widely studied CH 3 NH 3 PbI 3 (MAPbI 3 ). Because FAPbI 3 has two polymorphs (“black” α-FAPbI 3 and “yellow” δ-FA…
Aluminum is an abundant and high-quality material for plasmonics with potential for large-area, low-cost photonic technologies. Here we examine aluminum nanoclusters with plasmonic Fano resonances that can be tuned from the near-UV into the visible region of the spectrum. These nanoclusters can be designed with specif…
Multiple attributes of the three-dimensional (3D) extracellular matrix (ECM) have been independently implicated as regulators of cell motility, including pore size, crosslink density, structural organization, and stiffness. However, these parameters cannot be independently varied within a complex 3D ECM protein networ…
BACKGROUND: Graphene and graphene-based nanocomposites are used in various research areas including sensing, energy storage, and catalysis. The mechanical, thermal, electrical, and biological properties render graphene-based nanocomposites of metallic nanoparticles useful for several biomedical applications. Epithelia…
Active modulation of the polarization states of terahertz light is indispensable for polarization-sensitive spectroscopy, having important applications such as non-contact Hall measurements, vibrational circular dichroism measurements and anisotropy imaging. In the terahertz region, the lack of a polarization modulato…
Extracellular vesicles (EVs) have emerged as a ubiquitous mechanism for transferring information between cells and organisms across all three kingdoms of life. In addition to their roles in normal physiology, vesicles also transport molecules from pathogens to hosts and can spread antigens as well as infectious agents…
An updated and expanded data set that consists of 214 plagioclase-liquid equilibrium pairs from 40 experimental studies in the literature is used to recalibrate the thermodynamic model for the plagioclase- liquid hygrometer of Lange et al. (2009); the updated model is applicable to metaluminous and alkaline magmas. Th…
As a promising two-dimensional conjugated polymer, graphitic carbon nitride (g-C3 N4 ) has been utilized as a low-cost, robust, metal-free, and visible-light-active photocatalyst in the field of solar energy conversion. This Review mainly describes the latest advances in g-C3 N4 photocatalysts for water splitting. The…
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Abstract High‐quality single crystals of Pb17O8Cl18 with sizes of up to 7 mm x 2 mm x 2 mm are grown from a stoichiometric melt of PbO and PbCl2 (430 °C, 48 h) by a modified crystallization method in an open system.
The Si–O bond breaking event in the α-quartz at the first triplet (T 1 ) excitation state is studied by using ab initio molecular dynamics (AIMD) and nudged elastic band calculations. A meta-stable non-bridging oxygen hole center and E′ center (NBOHC-E′) is observed in the AIMD which consists of a broken Si–O bond wit…
Ba 0.85 Sr 0.15 Ti 0.90 Zr 0.10 O 3 (BSZT) ceramics doped Sn was prepared by seed-induced method. The seed was prepared by molten salt method, NaCl-KCl (1:1 by mole) eutectic mixtures was used as the flux. The BSZT added seed with doped SnO were calcined at 1250 °C for 3 hrs and sintered at 1400 °C for 2 hrs, respecti…
Lightly manganese-modified, Aurivillius-type, Bi5Ti3FeO15(BTF) ceramics were synthesized by substituting a small amount of manganese ions onto the Ti4+sites using conventional solid-state reaction. The resultant manganese-modified BTF ceramics (BTF-Mn) exhibit better dielectric and piezoelectric properties by comparis…
Abstract We discuss numerical results of nanodomain interfaces using a new extended molecular statics algorithm for ferroelectric materials. The new algorithm is able to not only calculate the change of the polarization behavior caused by strain but also the influence on the polarization behavior due to mechanical str…