Materials Literature
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Motivated by recent experimental interest in tunneling into heavy electron materials, we present a theory for electron tunneling into a Kondo lattice. The passage of an electron into the Kondo lattice is accompanied by a simultaneous spin flip of the localized moments via cotunneling mechanism. We compute the tunnelin…
Using light to modulate biochemical agents in living organisms has a significant impact on photodynamic therapy and drug release. We demonstrate that a photoresponsive system can reversibly induce paralysis in nematodes as a model for living organisms when two different wavelengths of light are used to toggle the mole…
We explore electron transport through a moebius strip attached to two metallic electrodes by the use of Green's function technique. A parametric approach is used based on the tight-binding model to characterize the electron transport through such a bridge system and it is observed that the transport properties are sig…
Photonic and optoelectronic devices may offer the opportunity to realize efficient signal processing at speeds higher than in conventional electronic devices. Switches form the building blocks for circuits and fast photonic switches have been realized [1,2,3,4,5,6]. Recently, proof of principle of exciton optoelectron…
Recent quantitative measurements of the orbital to spin magnetic moment ratio $m_L/m_S$ in electron magnetic circular dichroism (EMCD) experiments have given a $m_L/m_S$ ratio that is larger than commonly accepted values. We demonstrate here that plural scattering may noticeably influence the $m_L/m_S$ ratio. An equat…
Industry has already commenced the large-scale production of some nanomaterials. Evidence for toxic effects of engineered nanoparticles (ENP) on model organisms is increasing. However, in order to assess the consequences of environmental hazards, a better understanding is required of the behavior of ENP in aquatic eco…
Plasma enhanced chemical vapour deposition (PECVD) has been widely discussed in the literature for the growth of carbon nanotubes (CNTs) and carbon nanofibres (CNFs) in recent years. Advantages claimed include lower growth temperatures relative to thermal CVD and the ability to grow individual, free-standing, vertical…
Luminescent semiconductor nanocrystals, also known as quantum dots (QDs), have advanced the fields of molecular diagnostics and nanotherapeutics. Much of the initial progress for QDs in biology and medicine has focused on developing new biosensing formats to push the limit of detection sensitivity. Nevertheless, QDs c…
Scanning transmission X-ray microscopy has been used to quantitatively map the composition of P3HT:PCBM blend films in the vicinity of PCBM crystals formed during annealing at 140 °C. The observed PCBM concentration profiles around these crystals have been fitted to Fick’s second law of diffusion and the diffusion con…
Magnesium hydride (MgH(2)) is an attractive candidate for solid-state hydrogen storage applications. To improve the kinetics and thermodynamic properties of MgH(2) during dehydrogenation-rehydrogenation cycles, a nanostructured MgH(2)-0.1TiH(2) material system prepared by ultrahigh-energy-high-pressure mechanical mill…
Abstract Here, a novel synthesis for near monodisperse, sub‐10 nm Bi 2 Te 3 nanoparticles is reported. A new reduction route to bismuth nanoparticles is described, which are then applied as starting materials in the formation of rhombohedral Bi 2 Te 3 nanoparticles. After ligand removal by a novel hydrazine hydrate et…
Proton-coupled electron transfer (PCET) reactions play an essential role in a broad range of energy conversion processes, including photosynthesis and respiration. These reactions also form the basis of many types of solar fuel cells and electrochemical devices. Recent advances in the theory of PCET enable the predict…
We present a technique for the replacement of oleate with a PEG-phosphate ligand [PEG = poly(ethylene glycol)] as an efficient method for the generation of water-dispersible NaYF(4) nanoparticles (NPs). The PEG-phosphate ligands are shown to exchange with the original oleate ligands on the surface of the NPs, resultin…
Ecotoxicological effects of nanoparticles (NP) are still poorly documented while their commercialization for industrial and household applications increases. The aim of this study was to evaluate the influence of physicochemical characteristics on metal oxide NP and carbon nanotubes toxicological effects toward bacter…
The application of nanotechnology in medicine and pharmaceuticals is a rapidly advancing field that is quickly gaining acceptance and recognition as an independent area of research called "nanomedicine". Urgent needs in this field, however, are biocompatible and bioactive materials for antifouling surfaces and nanopar…
Step-growth, radically mediated thiol-norbornene photopolymerization is used to create versatile, stimuli-responsive poly(ethylene glycol)-co-peptide hydrogels The reaction is cytocompatible and allows for the encapsulation of human mesenchymal stem cells with a viability greater than 95%. Cellular spreading is dictat…
This review discusses recent developments and current research in bulk thermoelectric materials in which nanostructuring is a key aspect affecting thermoelectric performance. Systems based on PbTe, AgPb m SbTe 2+ m, NaPb m SbTe 2+ m, Bi 2 Te 3, and Si are given particular emphasis. To date the dramatic enhancements in…
Fluorescent carbon nanoparticles (CNPs) 2−6 nm in size with a quantum yield of about ∼3% were synthesized via nitric acid oxidation of carbon soot, and this approach can be used for milligram-scale synthesis of these water-soluble particles. These CNPs are nanocrystalline with a predominantly graphitic structure and s…
Nickel cobaltite (NiCo2O4) aerogels, synthesized with a chloride-based epoxide-driven sol–gel process, exhibit ultrahigh specific capacitances (1400 F g−1; see figure), excellent reversibility, and outstanding cycle stability, at a relatively high mass loading of 0.4 mg cm−2.
<div class="htmlview paragraph">This study aimed to evaluate the resistance of a Ti-6Al-4V alloy in creep after heat treatments. It was used a Ti-6Al-4V alloy in cylindrical bars forms, forged condition and annealing at 190 <u>°</u>C for 6 hours and cooled in air. The microstructure Ti-6Al-4V alloy w…