Materials Literature
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Computer simulations of (i) a [C12mim][Tf2N] film of nanometric thickness squeezed at kbar pressure by a piecewise parabolic confining potential reveal a mesoscopic in-plane density and composition modulation reminiscent of mesophases seen in 3D samples of the same room-temperature ionic liquid (RTIL). Near 2D confine…
In recent years, cellulose-based materials have attracted significant attention. To broaden the application areas for cellulose, polymers are often grafted to/from the surface to modify its properties. This study applies ARGET (activators regenerated by electron transfer) ATRP (atom transfer radical polymerization) wh…
The quantum corrections to the energies of the $\ensuremath{\Gamma}$ point optical phonon modes (Kohn anomalies) in graphene nanoribbons (NRs) are investigated. We show theoretically that the longitudinal optical (LO) modes undergo a Kohn anomaly effect, while the transverse optical (TO) modes do not. In relation to R…
In this paper we investigate the statistical behavior of an annealed continuous damage model. For different model variations we study distributions of times to failure and compare these results with the classical case of metastable nucleation in statistical mechanics. We show that our model has a tuning parameter whic…
The structure and evolution of grain boundaries underlies the nature of polycrystalline materials. Here we describe an experimental apparatus and light reflection technique for measuring disorder at grain boundaries in optically clear material, in thermodynamic equilibrium. The approach is demonstrated on ice bicrysta…
A new method to implement an asymmetrical two-dimensional magnetic lattice is proposed. The asymmetrical two-dimensional magnetic lattice can be created by periodically distributing magnetic minima across the surface of magnetic thin film where the periodicity can be achieved by milling $n\times n$ square holes on the…
Dynamic loadings produce high stress waves leading to the spallation of ductile materials such as aluminum, copper, magnesium or tantalum. The main mechanism used herein to explain the change of the number of cavities with the stress rate is nucleation inhibition, as induced by the growth of already nucleated cavities…
The hybrid nonlocal Euler-Bernoulli beam model is applied for the bending, buckling, and vibration analyzes of micro/nanobeams. In the hybrid nonlocal model, the strain energy functional combines the local and nonlocal curvatures so as to ensure the presence of small length-scale parameters in the deflection expressio…
Multilayer polyelectrolyte capsules made by layer-by-layer assembly of oppositely charged biodegradable polyelectrolytes were filled with a model of a nonactive prodrug, a self-quenched fluorescence-labeled protein. After capsule uptake by living cells, the walls of the capsules were actively degraded and digested by…
Nanocomposite thermoelectric materials have attracted much attention recently due to experimental demonstrations of improved thermoelectric properties over those of the corresponding bulk material. In order to better understand the reported data and to gain insight into transport in nanocomposites, we use the Boltzman…
The application of nanotechnology to medicine termed as 'nanomedicine' is recognised as an emerging field with enormous potential for developing new therapeutic concepts. A range of nanoscale materials have been explored in the last few years for drug delivery to address the problems associated with conventional drug…
Fungal cellobiohydrolases act at liquid-solid interfaces. They have the ability to hydrolyze cellulose chains of a crystalline substrate because of their two-domain structure, i.e. cellulose-binding domain and catalytic domain, and unique active site architecture. However, the details of the action of the two domains…
The negatively charged nitrogen-vacancy defect in diamond is an important atomic-scale structure that can be used as a qubit in quantum computing and as a marker in biomedical applications. Its usefulness relies on the ability to optically excite electrons between well-defined gap states, which requires a clear and de…
Full integration of graphene into conventional device circuitry would require a reproducible large scale graphene synthesis that is compatible with conventional thin film technology. We report the synthesis of large scale single layer graphene directly onto an evaporated copper film. A novel fabrication method was use…
In this paper, we report an investigation into the continuous crystallization of a model active pharmaceutical ingredient (API) using a continuous oscillatory baffled crystallizer (COBC). The results show that continuous crystallization offers significant advantages in terms of process, operation and costs, and delive…
We report a facile, high yielding synthetic method for preparing truly monodisperse Au(38)(SC(2)H(4)Ph)(24) nanoclusters. The synthetic approach involves two main steps: first, glutathionate (-SG) protected polydisperse Au(n) clusters (n ranging from 38 to approximately 102) are synthesized by reducing Au(I)-SG in ace…
Abstract Polypyrrole (PPy) was doped with the azocalix[4]arene [(5,11,17,23‐tetrakis[( p ‐carboxyphenyl)azo]25,26,27,28‐tetrahydroxycalix[4]arene)] host species. PPy/azocalix[4]arene salts were characterized by FTIR, TGA, SEM, X‐ray diffraction, and conductivity measurements. The properties of PPy were investigated in…
High optical quality, well end leg faceted ZnO microtetrapods sustaining lasing modes with quality factors of 2500–3000 have been grown by carbothermal chemical vapor deposition. It is shown that lasing is due to longitudinal Fabry–Pérot modes in individual tetrapod legs and the analysis of the wavelength position of…
The Exo-Planet Imaging Camera and Spectrograph for the future 42 m European-Extremely Large Telescope will enable direct images and spectra for both young and old Jupiter-mass planets in the infrared. To achieve the required contrast, several coronagraphic concepts—to remove starlight—are under investigation: conventi…
We demonstrate a polarizer-free electro-optical switch using dye-doped liquid crystal (LC) gels. The mechanism of dye-doped LC gels mainly involves the combination of polymer scattering and dye absorption. However, the domain size of polymer networks, dye concentration, LC concentration, and fabrication process can al…