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Separate Crystallization and Cocrystallization of Poly(L‐lactide) in the Presence of L‐Lactide‐Based Copolymers With Low Crystallizability, Poly(L‐lactide‐co‐glycolide) and Poly(L‐lactide‐co‐D‐lactide)

Hideto Tsuji、Kohji Tashiro、Leevameng Bouapao 等 4 位作者2012-09-14Macromolecular Chemistry and Physics

Abstract Poly( L ‐lactide) (PLLA) and poly( L ‐lactide‐ co ‐glycolide) (78/22)0 [P(LLA‐GA)] were phase‐separated in PLLA/P(LLA‐GA) blends, forming independent domains and thence crystallizing separately. The crystallization of PLLA was not disturbed or delayed by the presence of P(LLA‐GA) and vice versa. PLLA and poly…

biodegradable polymer synthesis and propertiesMicroplastics and Plastic PollutionAdditive Manufacturing and 3D Printing Technologies

Spin-lattice coupling in the frustrated antiferromagnet ZnCr2Se4probed by ultrasound

V. Felea、S. Yasin、A. Günther 等 10 位作者2012-09-14Physical Review B

Ultrasound and magnetization studies of the frustrated spinel ZnCr${}_{2}$Se${}_{4}$ are performed as a function of temperature and magnetic field up to 14 T. In zero field, the sound velocity and attenuation reveal significant anomalies at the antiferromagnetic transition at ${T}_{N}\ensuremath{\approx}$ 21 K indicat…

Magnetic and transport properties of perovskites and related materialsMultiferroics and related materialsAdvanced Condensed Matter Physics

Modification of the Green Fluorescent Protein Chromophore with Large Aromatic Moieties: Photophysical Study and Solid‐State Emission

Guangxi Huang、Guanxin Zhang、Yishi Wu 等 6 位作者2012-09-14Asian Journal of Organic Chemistry

Abstract Green fluorescent protein (GFP)‐like chromophores 1 – 5 , in which the p ‐hydroxylphenyl group is substituted with large aromatic moieties, were synthesized and their crystal structures were determined. Compared with that of p ‐hydroxybenzylideneimidazolinone (GFP chromophore), the fluorescence spectra of 1 –…

Advanced Fluorescence Microscopy TechniquesLuminescence and Fluorescent MaterialsSupramolecular Self-Assembly in Materials

Improvement of the thermal properties of poly(3‐hydroxybutyrate) (PHB) by low molecular weight polypropylene glycol (LMWPPG) addition

Juan Pedro Bretas Roa、Patrícia Santiago de Oliveira Patricio、Rodrigo Lambert Oréfice 等 4 位作者2012-09-14Journal of Applied Polymer Science

Abstract In this work, blends of poly(3‐hydroxybutyrate) (PHB) with 5, 10, 15, and 20 wt % low molecular weight poly(propylene glycol) (LMWPPG) have been prepared and characterized by scanning electron microscopy (SEM), Fourier transform infrared (FTIR) with attenuated total reflectance (ATR) accessory and simultaneou…

Polymer crystallization and propertiesbiodegradable polymer synthesis and propertiesCarbon dioxide utilization in catalysis

Small and Stable Phosphorylcholine Zwitterionic Quantum Dots for Weak Nonspecific Phagocytosis and Effective Tat Peptide Functionalization

Xiangsheng Liu、Huiguang Zhu、Qiao Jin 等 6 位作者2012-09-14Advanced Healthcare Materials

Facile surface modification of quantum dots (QDs) to make them water-soluble, small, stable, antibiofouling, and functional is crucial for their biological applications. This study demonstrates a simple ligand-exchange reaction to convert hydrophobic CdSe/ZnS QDs into water-soluble QDs using amphiphilic, zwitterionic…

Advanced biosensing and bioanalysis techniquesQuantum Dots Synthesis And PropertiesNanocluster Synthesis and Applications

How Structure-Related Collapse Mechanisms Determine Nanoscale Inhomogeneities in Thermoresponsive Polymers

Dennis Kurzbach、Martina Schömer、Valerie S. Wilms 等 5 位作者2012-09-14Macromolecules

Continuous wave electron paramagnetic resonance (CW EPR) spectroscopy on the amphiphilic spin probe TEMPO in solutions of selectively chosen functional, thermoresponsive poly(propylene oxide) (PPO)- and poly(ethylene oxide) (PEO)-based copolymers of both linear and branched structure is used to elucidate their host–gu…

Advanced Polymer Synthesis and CharacterizationConducting polymers and applicationsPolymer Surface Interaction Studies

Dispersion of magnetic nanoparticles in a polymorphic liquid crystal

Maksym F. Prodanov、Максим А. Колосов、Alexander I. Krivoshey 等 8 位作者2012-09-14Liquid Crystals

In order to enhance the phase stability of dispersions of magnetic nanoparticles (NPs) in a polymorphic liquid crystal, new ligands have been designed consisting of a terphenyl-based liquid crystalline core. The most stable dispersions were obtained with 7 nm super-paramagnetic Fe3O4 NPs decorated with the new ligands…

Liquid Crystal Research AdvancementsSurfactants and Colloidal SystemsCharacterization and Applications of Magnetic Nanoparticles

Energy spectrum and Landau levels in bilayer graphene with spin–orbit interaction

Francisco Mireles、John Schliemann2012-09-14New Journal of Physics

We present a theoretical study of the band structure and Landau levels in bilayer graphene at low energies in the presence of a transverse magnetic field and Rashba spin–orbit interaction in the regime of negligible trigonal distortion. Within an effective low-energy approach the (Löwdin partitioning theory), we deriv…

Graphene research and applicationsQuantum and electron transport phenomenaTopological Materials and Phenomena

Molecular Dynamics Simulations and Structural Descriptors of Radioisotope Glass Vectors for In Situ Radiotherapy

Jamieson K. Christie、Antonio Tilocca2012-09-14The Journal of Physical Chemistry B

The low solubility (high durability) of yttrium aluminosilicate (YAS) glass is one of its most important properties for use in in situ radiotherapy. Simple parameters, such as silica or yttria content or network connectivity, are not sufficient to rationalize the dependence of the solubility on the glass composition o…

Luminescence Properties of Advanced MaterialsGlass properties and applicationsNuclear materials and radiation effects

Synthesis of Chlorin-Sensitized Near Infrared-Emitting Lanthanide Complexes

Johanna Laakso、Geraldine A. Rosser、Csongor Szíjjártó 等 5 位作者2012-09-14Inorganic Chemistry

Lanthanide (Yb(3+), Nd(3+)) complexes equipped with red-absorbing hydroporphyrin (chlorin) antennae were synthesized and characterized. The syntheses are scalable, highly modular, and enable the introduction of different chlorins functionalized with a single reactive group (COOH or NH(2)). Absorption maxima were depen…

Molecular Sensors and Ion DetectionLanthanide and Transition Metal ComplexesSulfur Compounds in Biology

Improved Dehydrogenation Properties of Ti-Doped LiAlH4: Role of Ti Precursors

Placidus B. Amama、John T. Grant、Patrick J. Shamberger 等 5 位作者2012-09-14The Journal of Physical Chemistry C

The dehydrogenation properties of LiAlH 4 doped with different Ti precursors (Ti, TiO 2, and TiCl 3 ) via ball milling are investigated. The results not only show significant decreases in the decomposition temperatures ( T dec ) and activation energies ( E A ) of the first two dehydrogenation reaction steps of LiAlH 4…

Hydrogen Storage and MaterialsAmmonia Synthesis and Nitrogen ReductionSuperconductivity in MgB2 and Alloys

First-Principles Calculations of Clean and Defected ZnO Surfaces

Nunzio Roberto D’Amico、Giovanni Cantele、D. Ninno2012-09-14The Journal of Physical Chemistry C

We report on a theoretical study of the nonpolar ZnO (101̅0) and (112̅0) surfaces carried out in the framework of density functional theory, aiming to elucidate the thermodynamic and kinetic stability of the clean surface against the formation and diffusion of oxygen vacancies. At variance with other oxide materials a…

ZnO doping and propertiesGas Sensing Nanomaterials and SensorsElectronic and Structural Properties of Oxides

Highly Doped Carbon Nanotubes with Gold Nanoparticles and Their Influence on Electrical Conductivity and Thermopower of Nanocomposites

Kyungwho Choi、Choongho Yu2012-09-14PLoS ONE

Carbon nanotubes (CNTs) are often used as conductive fillers in composite materials, but electrical conductivity is limited by the maximum filler concentration that is necessary to maintain composite structures. This paper presents further improvement in electrical conductivity by precipitating gold nanoparticles onto…

Carbon Nanotubes in CompositesAdvanced Sensor and Energy Harvesting MaterialsConducting polymers and applications

Chiral Self-Assembly of Designed Amphiphiles: Optimization for Nanotube Formation

Thomas G. Barclay、Kristina T. Constantopoulos、Wei Zhang 等 5 位作者2012-09-14Langmuir

Four amphiphiles with L-aspartic acid headgroups (Asp) and a diphenyldiazenyl group (Azo) contained within the hydrophobic tails were designed and synthesized for self-assembly into helically based nanotubes. The amphiphiles of the form R'-{4-[(4-alkylphenyl)diazenyl]phenoxy}alkanoyl-L-aspartic acid (where R' is 10 or…

Lipid Membrane Structure and BehaviorSupramolecular Self-Assembly in MaterialsPolydiacetylene-based materials and applications

Synthesis, structure, and properties of chiral liquid crystal monomers and polymers based on menthol

Jianshe Hu、Dan Li、Wenchang Zhang 等 4 位作者2012-09-14Journal of Polymer Science Part A Polymer Chemistry

Abstract To study structure–mesomorphism relationships of the monomers and polymers based on menthol, four new chiral monomers ( M 1 – M 4 ) and the corresponding homopolymers ( P 1 – P 4 ) with menthyl group were synthesized. Their chemical structures, formula, phase behavior, and thermal stability were characterized…

Liquid Crystal Research AdvancementsPhotochromic and Fluorescence ChemistryMolecular spectroscopy and chirality

Impact of dynamic orbital correlations on magnetic excitations in the normal state of iron-based superconductors

Wei-Cheng Lee、Weicheng Lv、J. M. Tranquada 等 4 位作者2012-09-14Physical Review B

We show here that orbital degrees of freedom produce a distinct signature in the magnetic excitation spectrum of iron-based superconductors above the magnetic ordering temperature. Because ${d}_{xz}$ and ${d}_{yz}$ orbitals are strongly connected with Fermi surface topology, the nature of magnetic excitations can be m…

Rare-earth and actinide compoundsCorporate Taxation and AvoidanceIron-based superconductors research

Molecular dynamics simulation on interacting and mechanical properties of polylactic acid and attapulgite(100) surface

Su‐Qin Zhou、Xiao‐Chun Cheng、Yeling Jin 等 5 位作者2012-09-14Journal of Applied Polymer Science

Abstract The method of molecular dynamics (MD) simulations was used to investigate the interaction between the PLA and the attapulgite, and the influence of the temperature on the mechanical properties of the PLA and the PLA‐attapulgite. After the PLA blends the attapulgite, the structures and properties of the PLA an…

Polymer crystallization and propertiesbiodegradable polymer synthesis and propertiesMicroplastics and Plastic Pollution

Production of copolyesters of 3-hydroxybutyrate and medium-chain-length 3-hydroxyalkanoates by E. coli containing an optimized PHA synthase gene

Xue Gao、Xiao-Xi Yuan、Zhenyu Shi 等 8 位作者2012-09-14Microbial Cell Factories

BACKGROUND: Microbial polyhydroxyalkanoates (PHA) are biopolyesters consisting of diverse monomers. PHA synthase PhaC2Ps cloned from Pseudomonas stutzeri 1317 is able to polymerize short-chain-length (scl) 3-hydroxybutyrate (3HB) monomers and medium-chain-length (mcl) 3-hydroxyalkanoates (3HA) with carbon chain length…

biodegradable polymer synthesis and propertiesCatalysis for Biomass ConversionCarbon dioxide utilization in catalysis

Electrostatic interactions between Janus particles

Joost de Graaf、Niels Boon、Marjolein Dijkstra 等 4 位作者2012-09-14The Journal of Chemical Physics

In this paper we study the electrostatic properties of "Janus" spheres with unequal charge densities on both hemispheres. We introduce a method to compare primitive-model Monte Carlo simulations of the ionic double layer with predictions of (mean-field) nonlinear Poisson-Boltzmann theory. We also derive practical Derj…

Surfactants and Colloidal SystemsPickering emulsions and particle stabilizationElectrostatics and Colloid Interactions

Orientational interactions in block copolymer melts: Self-consistent field theory

Wei Zhao、Thomas P. Russell、Gregory M. Grason2012-09-14The Journal of Chemical Physics

We study the phase behavior of diblock copolymer melts with one block possessing orientation-dependent segmental interactions using self-consistent field theory. A generalized coarse-grained description is introduced based on the local (polar) orientational order parameter and K, an effective Frank elastic constant fo…

Theoretical and Computational PhysicsRheology and Fluid Dynamics StudiesBlock Copolymer Self-Assembly