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Purely hydrodynamic ordering of rotating disks at a finite Reynolds number

Yusuke Goto、Hajime Tanaka2015-01-28Nature Communications

Self-organization of moving objects in hydrodynamic environments has recently attracted considerable attention in connection to natural phenomena and living systems. However, the underlying physical mechanism is much less clear due to the intrinsically nonequilibrium nature, compared with self-organization of thermal…

Material Dynamics and PropertiesMicro and Nano RoboticsAdvanced Thermodynamics and Statistical Mechanics

Chitinase 3–Like-1 Regulates Both Visceral Fat Accumulation and Asthma-like Th2 Inflammation

Farida Ahangari、Akshay Sood、Bing Ma 等 10 位作者2015-01-28American Journal of Respiratory and Critical Care Medicine

RATIONALE: Obesity, especially truncal obesity, is a risk factor for asthma incidence, prevalence, and severity. Chitinase 3-like-1 (Chi3l1) is an evolutionarily conserved moiety that plays a critical role in antipathogen and Th2 responses. However, the mechanisms that underlie the association between asthma and obesi…

Asthma and respiratory diseasesNanocomposite Films for Food PackagingStudies on Chitinases and Chitosanases

Hybrid scaffolds based on PLGA and silk for bone tissue engineering

Faheem A. Sheikh、Hyung Woo Ju、Bo Mi Moon 等 11 位作者2015-01-28Journal of Tissue Engineering and Regenerative Medicine

Porous silk scaffolds, which are considered to be natural polymers, cannot be used alone because they have a long degradation rate, which makes it difficult for them to be replaced by the surrounding tissue. Scaffolds composed of synthetic polymers, such as PLGA, have a short degradation rate, lack hydrophilicity and…

Bone Tissue Engineering MaterialsDental Implant Techniques and OutcomesSilk-based biomaterials and applications

On how differently the quasi-harmonic approximation works for two isostructural crystals: Thermal properties of periclase and lime

Alessandro Erba、Masoud Shahrokhi、Rostam Moradian 等 4 位作者2015-01-28The Journal of Chemical Physics

Harmonic and quasi-harmonic thermal properties of two isostructural simple oxides (periclase, MgO, and lime, CaO) are computed with ab initio periodic simulations based on the density-functional-theory (DFT). The more polarizable character of calcium with respect to magnesium cations is found to dramatically affect th…

Advanced Chemical Physics StudiesHigh-pressure geophysics and materialsThermal Expansion and Ionic Conductivity

Enhanced Luminescent Properties of an Open‐Shell (3,5‐Dichloro‐4‐pyridyl)bis(2,4,6‐trichlorophenyl)methyl Radical by Coordination to Gold

Yohei Hattori、Tetsuro Kusamoto、Hiroshi Nishihara2015-01-28Angewandte Chemie International Edition

A gold(I) complex containing an open-shell luminescent (3,5-dichloro-4-pyridyl)bis(2,4,6-trichlorophenyl)methyl (PyBTM) radical was prepared. The complex showed fluorescence centered mainly on the coordinated PyBTM ligand. The photophysical and photochemical properties were positively modulated upon coordination to Au…

Metal complexes synthesis and propertiesOrganic Light-Emitting Diodes ResearchMagnetism in coordination complexes

Theory of long-lived nuclear spin states in methyl groups and quantum-rotor induced polarisation

Jean‐Nicolas Dumez、Pär Håkansson、Salvatore Mamone 等 10 位作者2015-01-28The Journal of Chemical Physics

Long-lived nuclear spin states have a relaxation time much longer than the longitudinal relaxation time T1. Long-lived states extend significantly the time scales that may be probed with magnetic resonance, with possible applications to transport and binding studies, and to hyperpolarised imaging. Rapidly rotating met…

Advanced NMR Techniques and ApplicationsSolid-state spectroscopy and crystallographyAtomic and Subatomic Physics Research

Effect of Ce addition on castability, mechanical properties and electric conductivity of Al–0.3Si–0.2Mg alloy

Hengcheng Liao、Yaxuan Liu、Cunhao Lu 等 4 位作者2015-01-28International Journal of Cast Metals Research

Effect of rare earth (RE) element cerium on castability, mechanical properties and electric conductivity of Al–0.3Si–0.2Mg alloy was investigated. With Ce addition, the fluidity of Al–0.3Si–0.2Mg alloys is increased and the hot tear sensitivity (HTS) is decreased remarkably, and the optimum Ce addition level is about…

Magnesium Alloys: Properties and ApplicationsAluminum Alloy Microstructure PropertiesAluminum Alloys Composites Properties

Three‐Dimensional Interconnected Vanadium Pentoxide Nanonetwork Cathode for High‐Rate Long‐Life Lithium Batteries

Qinyou An、Qiulong Wei、Pengfei Zhang 等 9 位作者2015-01-28Small

Three-dimensional interconnected vanadium pentoxide nanonetworks as cathodes for rechargable lithium batteries are successfully synthesized via a quick gelation followed by annealing. The interconnected structure ensures the electron transport of each unit. And their inner porous structure buffer the volume change ove…

Advancements in Battery MaterialsSupercapacitor Materials and FabricationAdvanced Battery Materials and Technologies

Ruthenium and Osmium Complexes That Bear Functional Azolate Chelates for Dye‐Sensitized Solar Cells

Yün Chi、Kuan‐Lin Wu、Tzu‐Chien Wei2015-01-28Chemistry - An Asian Journal

The preparation of sensitizers for dye-sensitized solar cells (DSSCs) represents an active area of research for both sustainability and renewable energy. Both Ru(II) and Os(II) metal sensitizers offer unique photophysical and electrochemical properties that arise from the intrinsic electronic properties, that is, the…

TiO2 Photocatalysis and Solar CellsAdvanced Photocatalysis TechniquesPolyoxometalates: Synthesis and Applications

Multicomponent superconductivity based on multiband superconductors

Y. Tanaka2015-01-28Superconductor Science and Technology

Multicomponent superconductivity is realized in multiband superconductors when an interband pairing interaction is considerably weaker than the intraband interactions. There is a new quantum phase that originates from the interband phase difference in this superconducting condensate. Firstly, we discuss the applicabil…

Physics of Superconductivity and MagnetismIron-based superconductors researchSuperconductivity in MgB2 and Alloys

Observation of Electron-Beam-Induced Phase Evolution Mimicking the Effect of the Charge–Discharge Cycle in Li-Rich Layered Cathode Materials Used for Li Ion Batteries

Ping Lu、Pengfei Yan、Eric Romero 等 6 位作者2015-01-28Chemistry of Materials

Capacity loss and voltage fade upon electrochemical charge–discharge cycling observed in lithium-rich layered cathode oxides (Li[Li x Mn y TM 1– x – y ]O 2, where TM = Ni, Co, or Fe) have recently been correlated with a gradual phase transformation featuring the formation of a surface reconstructed layer (SRL) that ev…

Advancements in Battery MaterialsAdvanced Electron Microscopy Techniques and ApplicationsElectron and X-Ray Spectroscopy Techniques

Compact femtosecond electron diffractometer with 100 keV electron bunches approaching the single-electron pulse duration limit

Lutz Waldecker、Roman Bertoni、Ralph Ernstorfer2015-01-28Journal of Applied Physics

We present the design and implementation of a highly compact femtosecond electron diffractometer working at electron energies up to 100 keV. We use a multi-body particle tracing code to simulate electron bunch propagation through the setup and to calculate pulse durations at the sample position. Our simulations show t…

Particle Accelerators and Free-Electron LasersAdvanced Electron Microscopy Techniques and ApplicationsElectron and X-Ray Spectroscopy Techniques

Highly Efficient Electronic Sensitization of Non-oxidized Graphene Flakes on Controlled Pore-loaded WO3 Nanofibers for Selective Detection of H2S Molecules

Seon‐Jin Choi、Chanyong Choi、Sang‐Joon Kim 等 7 位作者2015-01-28Scientific Reports

Tailoring of semiconducting metal oxide nanostructures, which possess controlled pore size and concentration, is of great value to accurately detect various volatile organic compounds in exhaled breath, which act as potential biomarkers for many health conditions. In this work, we have developed a very simple and robu…

Gas Sensing Nanomaterials and SensorsConducting polymers and applicationsAdvanced Chemical Sensor Technologies

A Novel and Effective Strategy for the Isolation of Adipose-Derived Stem Cells

Nicolas Bertheuil、B. Chaput2015-01-28Plastic & Reconstructive Surgery

Sir: We read with great interest the article entitled “A Novel and Effective Strategy for the Isolation of Adipose-Derived Stem Cells: Minimally Manipulated Adipose-Derived Stem Cells for More Rapid and Safe Stem Cell Therapy” by Raposio et al.1 Foremost, we want to congratulate the authors for this work and this inte…

Mesenchymal stem cell researchElectrospun Nanofibers in Biomedical ApplicationsTissue Engineering and Regenerative Medicine

Melting and Crystallization of Silicate Systems Relevant to Thermal Barrier Coating Damage

Elisa M. Zaleski、Charlotte Ensslen、Carlos G. Levi2015-01-28Journal of the American Ceramic Society

The melting and crystallization behaviors of model calcium–magnesium–alumino‐silicate ( CMAS ) compositions relevant to the degradation of thermal barrier coatings ( TBC s) were investigated. A primary goal was to establish a baseline for studies on CMAS reactions with TBC materials, reported separately, and their pot…

Advanced ceramic materials synthesisGlass properties and applicationsHigh-Temperature Coating Behaviors

XFEL diffraction: developing processing methods to optimize data quality

Nicholas K. Sauter2015-01-28Journal of Synchrotron Radiation

Serial crystallography, using either femtosecond X-ray pulses from free-electron laser sources or short synchrotron-radiation exposures, has the potential to reveal metalloprotein structural details while minimizing damage processes. However, deriving a self-consistent set of Bragg intensities from numerous still-crys…

Advanced Electron Microscopy Techniques and ApplicationsEnzyme Structure and FunctionAdvanced X-ray Imaging Techniques

Influence of boron diffusion on the perpendicular magnetic anisotropy in Ta|CoFeB|MgO ultrathin films

Jaivardhan Sinha、M. Gruber、M. Kodzuka 等 7 位作者2015-01-28Journal of Applied Physics

We have studied structural and magnetic properties of Ta|CoFeB|MgO heterostructures using cross-section transmission electron microscopy (TEM), electron energy loss spectrum (EELS) imaging, and vibrating sample magnetometry. From the TEM studies, the CoFeB layer is found to be predominantly amorphous for as deposited…

Magnetic properties of thin filmsZnO doping and propertiesMagnetic Properties of Alloys

1,5,9-Triaza-2,6,10-triphenylboracoronene: BN-Embedded Analogue of Coronene

Gang Li、Wei‐Wei Xiong、Peiyang Gu 等 9 位作者2015-01-28Organic Letters

A novel BN-fused coronene derivative 1,5,9-triaza-2,6,10-triphenylboracoronene (1) has been successfully synthesized in one step from 2,3,6,7,9,10-hexamethoxy-1,5,9-triamino-triphenylene. Compound 1 has been investigated using photophysical, electrochemical, and molecular simulation methods. Interestingly, three pheny…

Luminescence and Fluorescent MaterialsSynthesis and Properties of Aromatic CompoundsOrganoboron and organosilicon chemistry

Role of B diffusion in the interfacial Dzyaloshinskii-Moriya interaction in Ta/Co20Fe60B20/MgO nanowires

Roberto Lo Conte、E. Martı́nez、Aleš Hrabec 等 14 位作者2015-01-28Physical Review B

We report on current-induced domain wall motion in $\mathrm{Ta}/\mathrm{C}{\mathrm{o}}_{20}\mathrm{F}{\mathrm{e}}_{60}{\mathrm{B}}_{20}/\mathrm{MgO}$ nanowires. Domain walls are observed to move against the electron flow when no magnetic field is applied, while a field along the nanowires strongly affects the domain w…

Magnetic properties of thin filmsMetallic Glasses and Amorphous AlloysMagnetic Properties and Applications

Enzyme-Free Electrochemical Immunosensor Based on Host–Guest Nanonets Catalyzing Amplification for Procalcitonin Detection

Wen‐Jun Shen、Ying Zhuo、Ya-Qin Chai 等 6 位作者2015-01-28ACS Applied Materials & Interfaces

An enzyme-free electrochemical immunosensor based on the host-guest nanonets of N,N-bis(ferrocenoyl)-diaminoethane/β-cyclodextrins/poly(amidoamine) dendrimer-encapsulated Au nanoparticles (Fc-Fc/β-CD/PAMAM-Au) for procalcitonin (PCT) detection has been developed in this study. The signal probe was constructed as follo…

Advanced biosensing and bioanalysis techniquesElectrochemical sensors and biosensorsConducting polymers and applications