Materials Literature
按标题、摘要、年份、主题和来源检索公开元数据。结果保留作者、摘要、分类与原始来源链接。
A method of solving the time-dependent Schrödinger equation is presented, in which a finite region of space is treated explicitly, with the boundary conditions for matching the wave-functions on to the rest of the system replaced by an embedding term added on to the Hamiltonian. This time-dependent embedding term is d…
An electric current flowing around a loop produces a magnetic field and hence a magnetic flux through the loop. The ratio of the magnetic flux to the electric current is called the (magnetic) self inductance. Can there be a dual situation with a magnetic current flowing around a loop and producing an electric field an…
We generalize our recent work on the optical bistability of thin films of molecular aggregates [J. Chem. Phys. 127, 164705 (2007); arXiv:0707.1264v1 [cond-mat.dis-nn]] by accounting for the optical transitions from the one-exciton manifold to the two-exciton manifold as well as the exciton-exciton annihilation of the…
Angle-resolved photoemission spectroscopy data for the bilayer manganite ${\mathrm{La}}_{1.2}{\mathrm{Sr}}_{1.8}{\mathrm{Mn}}_{2}{\mathrm{O}}_{7}$ show that, upon lowering the temperature below the Curie point, a coherent polaronic metallic ground state emerges very rapidly with well-defined quasiparticles which track…
Soft and hard X-ray photoelectron spectroscopy (PES) has been performed for one of the heavy fermion system CeRu$_2$Si$_2$ and a $4f$-localized ferromagnet CeRu$_2$Ge$_2$ in the paramagnetic phase. The three-dimensional band structures and Fermi surface (FS) shapes of CeRu$_2$Si$_2$ have been determined by soft X-ray…
We report the propagation of highly nonlinear solitary waves in heterogeneous, periodic granular media using experiments, numerical simulations, and theoretical analysis. We examine periodic arrangements of particles in experiments in which stiffer/heavier beads (stainless steel) are alternated with softer/lighter one…
Specially shaped gold nanoparticles have intrigued considerable attention becausethey usually possess high-sensitivity surface-enhanced Raman scattering (SERS) and thusresult in large advantages in trace biodetermination. In this article, starch-capped goldnanoparticles with hexagon and boot shapes were prepared throu…
Abstract Recent progress of colloidal chemistry in the synthesis of multimaterial nanostructures incorporating transition‐metal oxides is reviewed. Attention is focused on the emerging class of hybrid nanocrystals (HNCs), in which domains of different materials are interconnected through inorganic junctions in defined…
The impact of electronic correlation in nanoscale junctions, e.g. formed by single molecules, is analyzed using the single-impurity Anderson model. Numerically exact Quantum Monte Carlo calculations are performed to map out the orbital filling, linear response conductance and spectral function as a function of the Cou…
Graphene grown epitaxially on SiC has been proposed as a material for carbon-based electronics. Understanding the interface between graphene and the SiC substrate will be important for future applications. We report the ability to image the interface structure beneath single-layer graphene using scanning tunneling mic…
Charge impurities in graphene can host an infinite family of Rydberg-like resonance states of massless Dirac particles. These states, appearing for supercritical charge, are described by Bohr-Sommerfeld quantization of collapsing classical trajectories that descend on point charge, in analogy to the hydrogenic Rydberg…
We explore the electronic properties of finite-length graphene nanoribbons as well as graphene nanodisks with various sizes and shapes in quest of metallic ones. For this purpose, it is sufficient to search zero-energy states. We find that no zero-energy states exist in finite-length zigzag nanoribbons though all infi…
Marilyn Monroe knew that "diamonds are a girl's best friend" but, in the meantime, many chemists have realized that they are also extremely attractive objects in contemporary chemistry. The chemist's diamonds are usually quite small (herein: nanometer-sized "diamondoids") and as a result of their unique structure are…
Through the use of various layer-by-layer polyelectrolyte (PE) coating schemes, such as the common poly(diallyldimethylammonium chloride)-poly(4-styrenesulfonic acid) (PDADMAC-PSS) system, the mammalian cellular uptake of gold nanorods can be tuned from very high to very low by manipulating the surface charge and func…
The conductivity of graphene samples with various levels of disorder is investigated for a set of specimens with mobility in the range of $1--20\ifmmode\times\else\texttimes\fi{}{10}^{3}\text{ }\text{ }{\mathrm{cm}}^{2}/\mathrm{V}\text{ }\mathrm{sec}$. Comparing the experimental data with the theoretical transport cal…
Three novel zinc(II) phthalocyanines substituted with one or two 3,4,5-tris(3,6,9-trioxadecoxy)benzoxy group(s) have been prepared and spectroscopically characterized. These compounds are highly soluble and remain nonaggregated in N,N-dimethylformamide. Upon excitation, they exhibit a relatively weak fluorescence emis…
This paper reports an investigation of the impact of temperature-dependent electrical and thermal conductivities (as governed by the classical Weidemann?Franz?Lorenz law) on the thermal response of nickel?chromium (nichrome) alloy cylinders. The relationship between the conductivities and temperature for nichrome is s…
Hydroxypropyl chitosan (HPCS), a water-soluble chitosan derivate, was modified by introducing photoreactive azide groups (4-azidobenzoic acid, Az-) to the amino groups of HPCS, resulting in a photocrosslinkable Az-HPCS. Novel porous chitosan scaffolds thus were fabricated by ultraviolet (UV) light irradiation of Az-HP…
Abstract The use of an accelerator based on diisopropyl xanthogen polysulfide (DIXP) to formulate bromobutyl elastomer (BIIR‐DIXP) compositions for sealing medical devices was published in the Journal of Applied Polymer Science (Ohbi, D. S.; Pureval, T. S.; Shah, T.; Siores, E. 2007, 106, 526). In this publication, a…
Despite widespread zirconium use ranging from nuclear technology to antiperspirants, important aspects of its solvation chemistry, such as the nature of small zirconium(IV) hydroxy cluster ions in aqueous solution, are not known due to the complexity of the zirconium aqueous chemistry. Using a combination of Car-Parri…