Materials Literature
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The electrical and structural characteristics of SmTiO3/SrTiO3/SmTiO3 and GdTiO3/SrTiO3/GdTiO3 heterostructures are compared. Both types of structures contain narrow SrTiO3 quantum wells, which accommodate a confined, high-density electron gas. As shown previously [Phys. Rev. B 86, 201102(R) (2012)] SrTiO3 quantum wel…
Less-defective colloidal crystals can be used as photonic crystals. To this end, colloidal epitaxy was proposed in 1997 as a method to reduce the stacking defects in the colloidal crystals. In this method, face-centered cubic (fcc) (001) stacking is forced by a template. In fcc (001) stacking, in contract to fcc {111}…
Modern theory of the orbital magnetization is applied to the series of prototype insulating perovskite transition metal oxides (orthorhombic YTiO${}_{3}$, LaMnO${}_{3}$, and YVO${}_{3}$, as well as monoclinic YVO${}_{3}$), carrying a net ferromagnetic (FM) moment in the ground state. For these purposes, we use an effe…
Recent advances in nanoscale science and technology provide possibilities to directly self-assemble and integrate functional circuit elements within the wiring scheme of devices with potentially unique architectures. Electroionic resistive switching circuits comprising highly interconnected fractal electrodes and meta…
We demonstrate a new method to measure absorption coefficients in any family of nanowires, provided they are grown on a substrate having considerable difference in permittivity with the nanowire-air matrix. In the case of high crystal quality, strain-free GaN nanowires, grown on Si (111) substrates with a density of ~…
The charge ordering (CO) transition in polycrystalline La1/3Sr2/3MnO3 has been studied by measuring the resistivity, magnetization and transverse ultrasonic velocity. At about 235K, a conspicuous increase in resistivity was observed, while the magnetization shows a cusp structure, corresponding to an antiferromagnetic…
The present paper gives a review of our recent progress and latest results for novel linear-algebraic algorithms and its application to large-scale quantum material simulations or electronic structure calculations. The algorithms are Krylov-subspace (iterative) solvers for generalized shifted linear equations, in the…
Planar auxetic structures have the potential to impact on a wide range of applications from deployable and morphing structures to space-filling composite and medical treatments. The ability to fabricate auxetics from smart materials greatly enhances this facility by building in controllable actuation and deployment. A…
The increasing application of engineered nanomaterials (ENMs) in consumer and medical products has motivated the development of single-particle inductively coupled plasma mass spectrometry (spICP-MS) for characterizing nanoparticles under realistic environmental exposure conditions. Recent studies have established a s…
Significant elemental segregation is shown to exist within individual hollow silver-gold (Ag-Au) bimetallic nanoparticles obtained from the galvanic reaction between Ag particles and AuCl4(-). Three-dimensional compositional mapping using energy dispersive X-ray (EDX) tomography within the scanning transmission electr…
Cellulose microfibrils physically bound together by soft hemicellulose chains form the scaffolding that makes plant cell walls strong. Inspired by this architecture, we designed biomimetic thermoreversible hydrogel networks based on reinforcing cellulose nanocrystals (CNC) and thermoresponsive methylcellulose (MC). Up…
This study demonstrates a facile, mild and environmentally-friendly sustainable (soft processing) approach for the efficient electrochemical exfoliation of graphite using a sodium hydroxide/hydrogen peroxide/water (NaOH/H2O2/H2O) system that can produce high-quality, anodic few-layer graphene nanosheets in 95% yield a…
The rapid development of deep‐UV (DUV) all‐solid‐state laser sources greatly depends on the good performance of the nonlinear optical (NLO) crystals used for harmonic generation. In this work, the potential prospects for NLO borate crystals are investigated from the point of view of their structure–property relationsh…
Self-assembled α-Fe2O3 mesocrystals/graphene nanohybrids have been successfully synthesized and have a unique mesocrystal porous structure, a large specific surface area, and high conductivity. Mesocrystal structures have recently attracted unparalleled attention owing to their promising application in energy storage…
In this study, we investigated the effect of nZVI on plant root elongation in Arabidopsis thaliana and showed, for the first time, that nZVI enhanced root elongation by inducing OH radical-induced cell wall loosening. Exposure of plants to 0.5 g/L nZVI enhanced root elongation by 150-200% over that in the control, and…
Two-dimensional (2D) nanomaterials, such as graphene and transition metal chalcogenides, show many interesting dimension-related materials properties. Inspired by the development of 2D inorganic nanomaterials, single-layered covalent organic frameworks (sCOFs), featuring atom-thick sheets and crystalline extended orga…
A scalable method to produce exfoliated and functionalized boron nitride sheets is described. The procedure involves the high temperature treatment of commercially obtained hexagonal boron nitride followed by hydrolysis. A mechanism of formation is proposed and analysis by XRD, FTIR, FESEM, TEM, AFM, XPS, TGA, and Ram…
Poly(lactic acid) (PLA) is one of the most promising alternatives for petrochemical-based plastics. Crystallization mediation provides the simplest and most practical approach for enhancing the properties of PLA. Here, recent advances in understanding the relationship between crystalline structure and properties of PL…
Mesoporous cobalt oxide (Co3O4) nanosheet electrode arrays are directly grown over flexible carbon paper substrates using an economical and scalable two-step process for supercapacitor applications. The interconnected nanosheet arrays form a three-dimensional network with exceptional supercapacitor performance in stan…
Small-molecule fluorophores manifest the ability of chemistry to solve problems in biology. As we noted in a previous review (Lavis, L. D.; Raines, R. T. ACS Chem. Biol. 2008, 3, 142-155), the extant collection of fluorescent probes is built on a modest set of "core" scaffolds that evolved during a century of academic…