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Inducing Lifshitz transition by extrinsic doping of surface bands in topological crystalline insulator Pb$_{1-x}$Sn$_{x}$Se

Ivo Pletikosić、Genda D. Gu、Tonica Valla2014-03-17arXiv

Narrow gap semiconductor Pb$_{1-x}$Sn$_{x}$Se was investigated for topologically protected surface states in its rock-salt structural phase for x=0.45, 0.23, 0.15, and 0. Angle-resolved photoelectron spectroscopy of intrinsically p-doped samples showed clear indication of two Dirac cones, eccentric about the time-reve…

Mesoscale and Nanoscale PhysicsMaterials Science

Mobility versus quality in 2D semiconductor structures

S. Das Sarma、E. H. Hwang2014-03-17arXiv

We consider theoretically effects of random charged impurity disorder on the {\it quality} of high-mobility two dimensional (2D) semiconductor structures, explicitly demonstrating that the sample mobility is not necessarily a reliable or universal indicator of the sample quality in high-mobility modulation-doped 2D Ga…

Materials ScienceMesoscale and Nanoscale Physics

Electric-Field-Modulated Nonvolatile Resistance Switching in VO2/PMN-PT(111) Heterostructures

Bowen Zhi、Guanyin Gao、Haoran Xu 等 8 位作者2014-03-17ACS Applied Materials & Interfaces

The electric-field-modulated resistance switching in VO2 thin films grown on piezoelectric (111)-0.68Pb(Mg1/3Nb2/3)O3-0.32PbTiO3 (PMN-PT) substrates has been investigated. Large relative change in resistance (10.7%) was observed in VO2/PMN-PT(111) hererostructures at room temperature. For a substrate with a given pola…

Transition Metal Oxide NanomaterialsAdvanced Memory and Neural Computing2D Materials and Applications

Ageing of the 2+1 dimensional Kardar-Parisi-Zhang model

Géza Ódor、Jeffrey Kelling、Sibylle Gemming2014-03-17arXiv

Extended dynamical simulations have been performed on a 2+1 dimensional driven dimer lattice gas model to estimate ageing properties. The auto-correlation and the auto-response functions are determined and the corresponding scaling exponents are tabulated. Since this model can be mapped onto the 2+1 dimensional Kardar…

cs.DCMaterials Sciencenlin.CGphysics.comp-phcond-mat.stat-mech

Pressure Induced Superconductivity and Structural Transitions in Ba(Fe0.9Ru0.1)2As2

Walter Uhoya、Georgiy M. Tsoi、Yogesh K. Vohra 等 5 位作者2014-03-17arXiv

High pressure electrical resistance and x-ray diffraction measurements have been performed on ruthenium-doped Ba(Fe0.9Ru0.1)2As2, up to pressures of 32 GPa and down to temperatures of 10 K, using designer diamond anvils under quasi-hydrostatic conditions. At 3.9 GPa, there is an evidence of pressure-induced supercondu…

SuperconductivityMaterials Science

Electrical switching effect of a single-unit-cell CrO2 layer on rutile TiO2 surface

Si-Da Li、Bang-Gui Liu2014-03-17arXiv

Rutile CrO2 is the most important half-metallic material with nearly 100% spin polarization at the Fermi level, and rutile TiO2 is a wide-gap semiconductor with many applications. Here we show through first-principles investigation that a single-unit-cell CrO2 layer on rutile TiO2 (001) surface is ferromagnetic and se…

Mesoscale and Nanoscale PhysicsMaterials Science

Evolving Design Rules for the Inverse Granular Packing Problem

Marc Z. Miskin、Heinrich M. Jaeger2014-03-17arXiv

If a collection of identical particles is poured into a container, different shapes will fill to different densities. But what is the shape that fills a container as close as possible to a pre-specified, desired density? We demonstrate a solution to this inverse-packing problem by framing it in the context of artifici…

Materials ScienceSoft Condensed Matter

A reentrant phenomenon in magnetic and dielectric properties of Dy2BaNiO5 and an intriguing influence of external magnetic field

Tathamay Basu、P. L. Paulose、Kartik K Iyer 等 8 位作者2014-03-17arXiv

We report that the spin-chain compound Dy2BaNiO5 recently proven to exhibit magnetoelectric coupling below its Neel temperature (T_N) of 58 K, exhibits strong frequency-dependent behavior in ac magnetic susceptibility and complex dielectric properties at low temperatures (<10K), mimicking 'reentrant' multiglass phenom…

Strongly Correlated ElectronsMaterials Science

Complex trend of magnetic order in Fe clusters on 4$d$ transition-metal surfaces

V. Sessi、F. Otte、S. Krotzky 等 9 位作者2014-03-17arXiv

We demonstrate the occurrence of compensated spin configurations in Fe clusters and monolayers on Ru(0001) and Rh(111) by a combination of X-ray magnetic circular dichroism experiments and first-principles calculations. Our results reveal complex intra-cluster exchange interactions which depend strongly on the substra…

Materials Science

Ba(Zn1-2xMnxCox)2As2: A Bulk Form Diluted Magnetic Semiconductor with n-type Carriers

Huiyuan Man、Cui Ding、Shengli Guo 等 9 位作者2014-03-17arXiv

We report the synthesis and characterization of bulk form diluted magnetic semiconductors Ba(Zn1-2xMnxCox)2As2 (0 <= x <= 0.15) with a crystal structure identical to that of 122-type Fe-based superconductors. Mn and Co co-doping into the parent compound BaZn2As2 results in a ferromagnetic ordering below TC ~ 80 K. Hal…

Strongly Correlated ElectronsMaterials Science

Proof of concept of a zinc-silver battery for the extraction of energy from a concentration difference

M. Marino、L. Misuri、A. Carati 等 4 位作者2014-03-17arXiv

The conversion of heat into current can be obtained by a process with two stages. In the first one, the heat is used for distilling a solution and obtaining two flows with different concentrations. In the second stage, the two flows are sent to an electrochemical cell that produces current by consuming the concentrati…

Chemical PhysicsMaterials Science

Spin Pumping and Inverse Spin Hall Effect in Platinum: The Essential Role of Spin-Memory Loss at Metallic Interfaces

J. -C. Rojas-Sánchez、N. Reyren、P. Laczkowski 等 10 位作者2014-03-17arXiv

Through combined ferromagnetic resonance, spin-pumping and inverse spin Hall effect experiments in Co|Pt bilayers and Co|Cu|Pt trilayers, we demonstrate consistent values of spin diffusion length $\ell_{\rm sf}^{\rm Pt}=3.4\pm0.4$ nm and of spin Hall angle $θ_{\rm SHE}^{\rm Pt}=0.051\pm0.004$ for Pt. Our data and mode…

Mesoscale and Nanoscale PhysicsMaterials Science

Perfect preferential orientation of nitrogen-vacancy defects in a synthetic diamond sample

M. Lesik、J.-P. Tetienne、A. Tallaire 等 8 位作者2014-03-17Applied Physics Letters

We show that the orientation of nitrogen-vacancy (NV) defects in diamond can be efficiently controlled through chemical vapor deposition growth on a (111)-oriented diamond substrate. More precisely, we demonstrate that spontaneously generated NV defects are oriented with a ∼97% probability along the [111] axis, corres…

Diamond and Carbon-based Materials ResearchElectronic and Structural Properties of OxidesGraphene research and applications

Introduction to Graphene-Based Nanomaterials: From Electronic Structure to Quantum Transport

Luis E. F. Foa Torres、Stephan Roche、Jean‐Christophe Charlier2014-03-17DIAL (Catholic University of Leuven)

Graphene is one of the most intensively studied materials, and has unusual electrical, mechanical and thermal properties, which provide almost unlimited potential applications. This book provides an introduction to the electrical and transport properties of graphene and other two-dimensional nanomaterials, covering ab…

Semiconductor materials and devicesGraphene research and applicationsAdvancements in Semiconductor Devices and Circuit Design

Quantum‐Dot Sensitized Solar Cells Employing Hierarchical Cu2S Microspheres Wrapped by Reduced Graphene Oxide Nanosheets as Effective Counter Electrodes

Meidan Ye、Chang Chen、Nan Zhang 等 6 位作者2014-03-17Advanced Energy Materials

Hierarchical Cu 2 S microspheres wrapped by reduced graphene oxide (RGO) nanosheets are prepared via a one‐step solvothermal process. The amount of graphene oxide used in the synthesis process has a remarkable effect on the features of Cu 2 S microspheres. Compared to Pt and Cu 2 S electrodes, RGO‐Cu 2 S electrodes sh…

Quantum Dots Synthesis And PropertiesCopper-based nanomaterials and applicationsAdvanced Photocatalysis Techniques

Hyaluronic Acid Conjugates as Vectors for the Active Targeting of Drugs, Genes and Nanocomposites in Cancer Treatment

Gloria Berlier、Paola Milla、Barbara Stella 等 4 位作者2014-03-17Molecules

Hyaluronic acid (HA) is a naturally-occurring glycosaminoglycan and a major component of the extracellular matrix. Low levels of the hyaluronic acid receptor CD44 are found on the surface of epithelial, hematopoietic, and neuronal cells; it is overexpressed in many cancer cells, and in particular in tumor-initiating c…

Nanoplatforms for cancer theranosticsNanoparticle-Based Drug DeliveryRNA Interference and Gene Delivery

Air-Stable n-Doped Colloidal HgS Quantum Dots

Kwang Seob Jeong、Zhiyou Deng、Sean Keuleyan 等 5 位作者2014-03-17The Journal of Physical Chemistry Letters

HgS nanocrystals show a strong mid-infrared absorption and a bleach of the near-infrared band edge, both tunable in energy and reversibly controlled by exposure to solution ions under ambient conditions. The same effects are obtained by applying a reducing electrochemical potential, confirming that the mid-infrared ab…

Copper-based nanomaterials and applicationsQuantum Dots Synthesis And PropertiesChalcogenide Semiconductor Thin Films

Gigantic Swelling of Inorganic Layered Materials: A Bridge to Molecularly Thin Two-Dimensional Nanosheets

Fengxia Geng、Renzhi Ma、Yasuo Ebina 等 6 位作者2014-03-17Journal of the American Chemical Society

Platy microcrystals of a typical layered material, protonated titanate, have been shown to undergo an enormous degree of swelling in aqueous solutions of various amines, including tertiary amines, quaternary ammonium hydroxides, and primary amines. Introducing these solutions expanded the crystal gallery height by up…

Advanced Photocatalysis TechniquesLayered Double Hydroxides Synthesis and ApplicationsCovalent Organic Framework Applications

Deactivation Mechanism of Potassium on the V2O5/CeO2 Catalysts for SCR Reaction: Acidity, Reducibility and Adsorbed-NOx

Yue Peng、Junhua Li、Xu Huang 等 8 位作者2014-03-17Environmental Science & Technology

A series of V2O5/CeO2 catalysts with different potassium loadings were prepared to investigate alkali deactivations for selective catalytic reduction of NOx with NH3. An alkali poisoning mechanism could be attributed to surface acidity, reducibility, and NOx adsorption/desorption behaviors. The detailed factors are as…

Catalytic Processes in Materials ScienceCatalysis and Oxidation ReactionsIndustrial Gas Emission Control

Facile Synthesis of Yolk–Shell Structured Inorganic–Organic Hybrid Spheres with Ordered Radial Mesochannels

Zhaogang Teng、Shouju Wang、Xiaodan Su 等 11 位作者2014-03-17Advanced Materials

Monodisperse yolk–shell mesoporous hybrid spheres with ordered radial mesochannels are demonstrated to be readily prepared by incubating mesostructured hybrid spheres with water. The obtained yolk–shell mesoporous spheres have inorganic–organic hybrid framework, tunable diameter, high surface area, radially oriented o…

Membrane Separation and Gas TransportMesoporous Materials and CatalysisCovalent Organic Framework Applications