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Preparations and Characterizations of Bichromophoric Systems Composed of a Ruthenium Polypyridine Complex Connected to a Difluoroborazaindacene or a Zinc Phthalocyanine Chromophore

Fabrice Odobel、Hervé Zabri2005-07-08Inorganic Chemistry

This paper describes the synthesis of a new series of molecules composed of a ruthenium cation liganded by a chloro or a thiocyanato, a 4,4'-(diethoxycarbonyl)-2,2'-bipyridine, and a 2,2':6',2' '-terpyridine substituted in its 4' position by a difluoroborazaindacene or a zinc phthalocyanine. A set of conditions are re…

Organic Light-Emitting Diodes ResearchPorphyrin and Phthalocyanine ChemistryLuminescence and Fluorescent Materials

Electronic and structural properties of SnO under pressure

N. E. Christensen、A. Svane、E. L. Peltzer y Blancá2005-07-08Physical Review B

Pressure-induced changes in the electronic and structural properties of tin monoxide are examined by means of ab initio density-functional calculations. Also, the pressure shifts of the ${A}_{1g}$ and ${E}_{g}$ zone-center phonon modes are derived. The results are compared to recent experimental high-pressure data as…

ZnO doping and propertiesGas Sensing Nanomaterials and SensorsElectronic and Structural Properties of Oxides

Araneoid Egg Case Silk: A Fibroin with Novel Ensemble Repeat Units from the Black Widow Spider, Latrodectus hesperus

Xiaoyi Hu、Barbara A. Lawrence、Kristin Kohler 等 8 位作者2005-07-08Biochemistry

Araneoid spiders use specialized abdominal glands to manufacture up to seven different protein-based silks/glues that have diverse physical properties. The fibroin sequences that encode egg case fibers (cover silk for the egg case sac) and the secondary structure of these threads have not been previously determined. I…

Antimicrobial Peptides and ActivitiesSilk-based biomaterials and applicationsSpider Taxonomy and Behavior Studies

Blends of poly(ethylene terephthalate) and poly(butylene terephthalate)

G. Aravinthan、D. D. Kale2005-07-08Journal of Applied Polymer Science

Abstract Commercial grade poly(ethylene terephthalate), (PET, intrinsic viscosity = 0.80 dL/g) and poly(butylene terephthalate), (PBT, intrinsic viscosity = 1.00 dL/g) were melt blended over the entire composition range using a counterrotating twin‐screw extruder. The mechanical, thermal, electrical, and rheological p…

Polymer crystallization and propertiesPolymer Nanocomposites and Propertiesbiodegradable polymer synthesis and properties

Ultrafast carrier dynamics in ZnO nanorods

Chi‐Kuang Sun、Shih-Ze Sun、Kung‐Hsuan Lin 等 7 位作者2005-07-08Applied Physics Letters

Free exciton and above-band-gap free carrier dynamics in ZnO nanorods have been investigated at room temperature with a femtosecond transient transmission measurement. Following the photoexcitation of above-band-gap free carriers, an extremely fast external thermalization time on the order of 200 fs can be observed. U…

ZnO doping and propertiesGaN-based semiconductor devices and materialsPerovskite Materials and Applications

Cyclohexane‐Based Low Molecular Weight Hydrogelators: A Chirality Investigation

Arianna Friggeri、Cornelia van der Pol、Kjeld J. C. van Bommel 等 7 位作者2005-07-08Chemistry - A European Journal

Seven new 1,3,5-cyclohexyltricarboxamide-phenylalanine derivatives were synthesized in order to investigate the effect of the amino acid chirality on the gelating properties of these small molecules in water. Gelation tests have shown that enantiomerically pure homochiral 1,3,5-cyclohexyltricarboxamide-L-phenylalanine…

Lipid Membrane Structure and BehaviorGlycosylation and Glycoproteins ResearchSupramolecular Self-Assembly in Materials

Hydrostatic pressure control of the magnetostructural phase transition inGd5Si2Ge2single crystals

César Magén、L. Morellón、P. A. Algarabel 等 11 位作者2005-07-08Physical Review B

Magnetic and structural properties of single crystalline ${\mathrm{Gd}}_{5}{\mathrm{Si}}_{2}{\mathrm{Ge}}_{2}$ under hydrostatic pressure have been characterized by using magnetization, linear thermal expansion, and compressibility measurements. A strong dependence of Curie temperature on pressure, $d{T}_{C}∕dP=+4.8\p…

Magnetic and transport properties of perovskites and related materialsCrystal Structures and PropertiesAdvanced Condensed Matter Physics

Sub‐10 nm High‐Aspect‐Ratio Patterning of ZnO Using an Electron Beam

Mohammad S. M. Saifullah、K. R. V. Subramanian、Dae Joon Kang 等 7 位作者2005-07-08Advanced Materials

An electron-beam-sensitive zinc naphthenate resist is used to pattern ZnO. Features as small as 7 nm and with an aspect ratio of ∼ 9 can be patterned. Size reduction to ∼ 5 nm is observed when these patterns are heat treated to give crystalline ZnO (see Figure). The functionality of ZnO is confirmed via photoluminesce…

ZnO doping and propertiesCopper-based nanomaterials and applicationsElectronic and Structural Properties of Oxides

Amphoteric doping of carbon nanotubes by encapsulation of organic molecules: Electronic properties and quantum conductance

Vincent Meunier、Bobby G. Sumpter2005-07-08The Journal of Chemical Physics

In order to investigate and optimize the electronic transport processes in carbon nanotubes doped with organic molecules, we have performed large-scale quantum electronic structure calculations coupled with a Green's function formulation for determining the quantum conductance. Our approach is based on an original sch…

Carbon Nanotubes in CompositesGraphene research and applicationsMolecular Junctions and Nanostructures

Ballistic thermal and electrical conductance measurements on individual multiwall carbon nanotubes

Elisabetta Brown、Ling Hao、John Gallop 等 4 位作者2005-07-08Applied Physics Letters

We report thermal measurements on individual carbon nanotubes using a temperature sensing scanned microscope probe. An arc-grown bundle of multiwalled nanotubes (MWNTs) is mechanically attached to a thermal probe. The heat flow down individual MWNTs is recorded as a function of the temperature difference across them.…

Carbon Nanotubes in CompositesThermal properties of materialsMechanical and Optical Resonators

Effect of Supercritical Gas on Crystallization of Linear and Branched Polypropylene Resins with Foaming Additives

Hani E. Naguib、Chul B. Park、Seungwon Song2005-07-08Industrial & Engineering Chemistry Research

The thermal behaviors of linear and branched polypropylene (PP) with foaming additives were investigated using a normal and a high-pressure differential scanning calorimeter (DSC). Specifically, the effects of material branching, dispersed additives, cooling rates, and dissolved blowing agents on the crystallization t…

Polymer crystallization and propertiesbiodegradable polymer synthesis and propertiesPolymer Foaming and Composites

Quantitative Prediction of Long-Term Failure of Polycarbonate

E. T. J. Klompen、Tom A. P. Engels、van Lca Lambèrt Breemen 等 6 位作者2005-07-08Macromolecules

Time-to-failure of polymers, and the actual failure mode, are influenced by stress, temperature, processing history, and molecular weight. We show that long-term ductile failure under constant load is governed by the same process as short term ductile failure at constant rate of deformation. Failure proves to originat…

Polymer crystallization and propertiesRheology and Fluid Dynamics StudiesElectrostatic Discharge in Electronics

Thermally stable visible-blind diamond photodiode using tungsten carbide Schottky contact

Meiyong Liao、Yasuo Koide、José Alvarez2005-07-08Applied Physics Letters

We have developed a thermally stable, deep-ultraviolet (DUV) photodiode using tungsten carbide (WC) Schottky and Ti/WC ohmic contacts for a boron-doped homoepitaxial p-diamond epilayer. Effects of thermal annealing in an argon ambient on the electrical and photoresponse properties were investigated. Annealing at tempe…

Semiconductor materials and devicesDiamond and Carbon-based Materials ResearchNanowire Synthesis and Applications

Influence of the Rare‐Earth Element on the Mechanical Properties of RE–Mg‐Bearing Silicon Nitride

R. L. Satet、Michael J. Hoffmann2005-07-08Journal of the American Ceramic Society

Silicon nitride bulk ceramics with varying compositions of the grain boundary phase but similar grain sizes were developed, which allows to analyze the influence of the grain boundary chemistry on mechanical properties. Micrographs of the crack path reveal a much weaker interface when the rare‐earth element in the gra…

Advanced ceramic materials synthesisMetal and Thin Film MechanicsBoron and Carbon Nanomaterials Research

Plasmon hybridization in nanoshell dimers

Daniel Brandl、Chris Oubre、Peter Nordlander2005-07-08The Journal of Chemical Physics

We extend the plasmon hybridization method to investigate the plasmon modes of metallic nanoshell dimers. The formalism is also generalized to include the effects of dielectric backgrounds. It is shown that the presence of dielectrics shifts the plasmon resonances of the individual nanoparticles to lower energies and…

Gold and Silver Nanoparticles Synthesis and ApplicationsPlasmonic and Surface Plasmon ResearchNonlinear Optical Materials Studies

Preparation of Exfoliated Polyester/Clay Nanocomposites

Tsung‐Yu Tsai、Chii‐Horng Li、Chiung‐Hsin Chang 等 6 位作者2005-07-08Advanced Materials

Poly(ethylene terephthalate) (PET)/clay nanocomposites are prepared by intercalation of a catalyst precursor and an organic modifier, followed by the polymerization of monomers between the adjacent clay layers. The mechanical properties, thermal deformation temperature, anti-UV-radiation properties, CO2 gas-barrier pr…

Polymer crystallization and propertiesPolymer Nanocomposites and Propertiesbiodegradable polymer synthesis and properties

Application of rice husk ash as fillers in the natural rubber industry

Wanvimon Arayapranee、Nuchanat Na‐Ranong、Garry L. Rempel2005-07-08Journal of Applied Polymer Science

Abstract Rice husk ash (RHA) obtained from agricultural waste, by using rice husk as a power source, is mainly composed of silica and carbon black. A two‐stage conventional mixing procedure was used to incorporate rice husk ash into natural rubber. For comparison purposes, two commercial reinforcing fillers, silica an…

Concrete and Cement Materials ResearchPolymer Nanocomposites and PropertiesInnovative concrete reinforcement materials

Electrode and grain-boundary effects on the conductivity of CaCu3Ti4O12

Lei Zhang2005-07-08Applied Physics Letters

The ac conductivity of CaCu3Ti4O12 (CCTO) ceramics was studied in the temperature range 173<T<443K. The dc conductivities containing the components of electrodes (σe) and grain boundaries (σgb) were measured, from which a thermal activation energies of ∼0.54eV was inferred. Different behaviors of dielect…

Ferroelectric and Piezoelectric MaterialsMicrowave Dielectric Ceramics SynthesisDielectric properties of ceramics

Highest conductivity oxide SrMoO3 grown by a floating-zone method under ultralow oxygen partial pressure

Ichiro Nagai、Naoki Shirakawa、S. Ikeda 等 6 位作者2005-07-08Applied Physics Letters

Single crystals of a highly conductive oxide SrMoO3 have been grown by a floating-zone method under argon atmosphere with ultralow oxygen partial pressure p(O2)∼10−25atm. The obtained single crystals of SrMoO3 reveal quite low resistivity at 300 K ρ(300K)=5.1μΩcm, which is the lowest to date in the values of ρ(300K) o…

Magnetic and transport properties of perovskites and related materialsAdvanced Condensed Matter PhysicsElectronic and Structural Properties of Oxides

High‐Yield Synthesis of Single‐Crystal Nanosprings of ZnO

Pu Gao、Zhong Lin Wang2005-07-08Small

Pre-growth pressure control in a solid–vapor process leads to the synthesis of single-crystal ZnO nanosprings at high yield (>50 %). This study demonstrates the possibility of synthesizing nanosprings (see image) of high purity and at high yield, and makes systematic understanding of the properties and exploration of…

ZnO doping and propertiesGas Sensing Nanomaterials and SensorsGa2O3 and related materials