Materials Literature
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Mesoporous TiO 2 thin films doped with varying amounts of cerium have been synthesized via a supramolecular-templated sol−gel route. The cerium dopant strongly affects the mesostructure, photocatalytic, and optical properties of the mesoporous TiO 2 films. At an appropriately low level of cerium doping (i.e., Ce/Ti <…
Three's company: The first genuine ternary colloidal crystal (see picture) is composed of PbSe nanocrystals of two different diameters (blue and green) and of CdSe nanocrystals (red). Electron tomography shows that the superlattice is isostructural with the atomic lattice AlMgB4.
We show that Ce(3+) can be an efficient sensitizer for Yb(3+) in the host lattice of yttrium aluminum garnet (YAG). With blue-light excitation to induce the 4f-->5d transition of Ce(3+), characteristic near-IR emission of Yb(3+) due to transition of (2)F(5/2)-->(2)F(7/2) peaking at 1030 nm is generated as a result of…
Epitaxial ultrathin Fe films on fcc Cu(001) exhibit a spin spiral (SS), in contrast to the ferromagnetism of bulk bcc Fe. We study the in-plane and out-of-plane Fermi surfaces (FSs) of the SS in 8 monolayer Fe/Cu(001) films using energy dependent soft x-ray momentum-resolved photoemission spectroscopy. We show that th…
We study the plastic yielding of disordered media using the perfectly plastic random fuse model. The yield surfaces are shown to be different from those obtained minimizing the sum of the local yield thresholds, i.e. the so-called minimum 'energy' surfaces. As a result, the global yield stress is lower than expected f…
RbFe2As2 has recently been reported to be a bulk superconductor with Tc = 2.6 K in the undoped state, in contrast to undoped BaFe2As2 with a magnetic ground state. We present here the results of the first-principles calculations of the structural, elastic and electronic properties for this newest superconductor and di…
An incommensurate modulated structure was found recently in a light group V element phosphorous in the phase P-IV stable in the pressure range 107-137 GPa. We consider configurations of the Brillouin zone and Fermi sphere within a nearly-free-electron model in order to analyze the importance of these configurations fo…
Molecular dynamics simulations have been performed to study the structural transition in bcc iron under uniaxial strain loading. We found that the transition pressures are less dependent on the crystal orientations, ∼14 GPa for [001], [011], and [111] loadings. However, the pressure interval of a mixed phase for [011]…
We show that in a quantum wire the spin-orbit interaction leads to a narrow spin resonance at low temperatures, even in the absence of an external magnetic field. Resonance absorption by linearly polarized radiation gives a dc spin current; resonance absorption by circularly polarized radiation gives a dc electric cur…
We study electron transport through a quantum interferometer with side-coupled quantum dots. The interferometer, threaded by a magnetic flux $ϕ$, is attached symmetrically to two semi-infinite one-dimensional metallic electrodes. The calculations are based on the tight-binding model and the Green's function method, wh…
Bulk crystals of zinc oxide can be grown from the melt by a Bridgman technique under pressure. This new technology using an iridium crucible shows the potential to yield large single crystals of good crystalline perfection. Crystals with diameters up to 33 mm and a length of up to 50 mm have been demonstrated. The imp…
A Monte Carlo simulation is carried out to investigate the magnetic ordering in magnets with random anisotropy (RA). Our results show peculiar similarities to recent experiments that the real part of ac susceptibility presents two peaks for weak RA and only one for strong RA regardless of glassy critical dynamics mani…
We extend the study of the Fermi surface instability of the Pomeranchuk type into systems with orbital band structures, which are common features in transition metal oxides. Band hybridization significantly shifts the spectra weight of the Landau interactions from the conventional s-wave channel to unconventional non-…
Through novel application of small-angle neutron scattering, we examined the fate of silica nanoparticles (SiO(2)NPs) during simulated primary wastewater treatment, by measuring, in real time, the colloidal behavior of SiO(2)NPs in wastewater (sewage). We examined the effects of surface functionality on SiO(2)NP fate…
In the cage: Photochemical control over biological processes is commonly achieved with caged molecules. While the first reported examples of caged compounds were small molecules, recent advances in caging technologies have enabled the photochemical regulation of oligonucleotide and protein function. This article discu…
The supercapacitive properties of nickel(II) tetraaminophthalocyanine (NiTAPc)/multi-walled carbon nanotube (MWCNT) nanocomposite films have been interrogated for the first time and found to possess a maximum specific capacitance of 981 ± 57 F g−1 (200 ± 12 mF cm−2), a maximum power density of 700 ± 1 Wkg−1, a maximum…
A low melting point soda-lime glass powder containing copper nanoparticles with high antibacterial (against gram-positive and gram-negative bacteria) and antifungal activity has been obtained. Sepiolite fibres containing monodispersed copper nanoparticles (d(50) approximately 30 +/- 5 nm) were used as the source of th…
Sophisticated helical structure has been an attractive subject due to its significance in understanding of biological self-assembly and appealing application in nanoscience. In this work, a facile route toward one-dimensional helical nanostructure is presented based on metal-cholate supramolecular self-assembly. Well-…
Phase transformation generally begins with nucleation, in which a small aggregate of atoms organizes into a different structural symmetry. The thermodynamic driving forces and kinetic rates have been predicted by classical nucleation theory, but observation of nanometer-scale nuclei has not been possible, except on ex…
We studied the electric field effect on superconductivity in atomically thin flakes of ${\text{NbSe}}_{2}$ prepared by mechanical exfoliation. We found that these ${\text{NbSe}}_{2}$ flakes are superconducting down to a thickness of a single unit cell consisting of two molecular layers of ${\text{NbSe}}_{2}$ with an o…