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Cation-Directed Synthesis of Tungstosilicates. 1. Syntheses and Structures of K10A-α-[SiW9O34]·24H2O, of the Sandwich-Type Complex K10.75[Co(H2O)6]0.5[Co(H2O)4Cl]0.25A-α-[K2{Co(H2O)2}3(SiW9O34)2]·32H2O and of Cs15[K(SiW11O39)2]·39H2O

Nathalie Laronze、Jérôme Marrot、Gilbert Hervé2003-08-16Inorganic Chemistry

The influence of the nature of alkali metal cations on the structure of the species obtained from the trivacant precursor A-alpha-[SiW(9)O(34)](10-) has been studied. Starting from the potassium salt 1, K(10)A-alpha-[SiW(9)O(34)].24H(2)O, the sandwich-type complex 2, K(10.75)[Co(H(2)O)(6)](0.5)[Co(H(2)O)(4)Cl](0.25)A-…

Metal-Organic Frameworks: Synthesis and ApplicationsPolyoxometalates: Synthesis and ApplicationsChemical Synthesis and Characterization

Structures and Fragmentations of Small Silicon Oxide Clusters by ab Initio Calculations

Wen-Cai Lu、Cai‐Zhuang Wang、Vân Hà Nguyễn 等 6 位作者2003-08-16The Journal of Physical Chemistry A

The structures, energies, and fragmentation stabilities of silicon oxide clusters Si m O n, with m = 1−5, n = 1, 2 m + 1, are studied systematically by ab initio calculations. New structures for nine clusters are found to be energetically more favorable than previously proposed structures. Using the ground state struc…

ZnO doping and propertiesCatalytic Processes in Materials ScienceSemiconductor materials and devices

Controlled Grafting of Well-Defined Polymers on Hydrogen-Terminated Silicon Substrates by Surface-Initiated Atom Transfer Radical Polymerization

W. H. Yu、E. T. Kang、K. G. Neoh 等 4 位作者2003-08-16The Journal of Physical Chemistry B

Controlled grafting of well-defined polymer brushes on the hydrogen-terminated Si(100) substrates (the Si−H substrate) was carried out via the surface-initiated atom transfer radical polymerization (ATRP). Surface initiators were immobilized on the Si−H substrates in three consecutive steps: (i) coupling of an ω-unsat…

Polymer Surface Interaction StudiesMolecular Junctions and NanostructuresForce Microscopy Techniques and Applications

Loading the Multilayer Dextran Sulfate/Protamine Microsized Capsules with Peroxidase

Н. Г. Балабушевич、Olga P. Tiourina、Dmitry Volodkin 等 5 位作者2003-08-16Biomacromolecules

Stable polyelectrolyte capsules were produced by the layer-by-layer (LbL) assembling of biodegradable polyelectrolytes, dextran sulfate and protamine, on melamine formaldehyde (MF) microcores followed by the cores decomposition at low pH. The mean diameter of the capsules at pH 3-5 was 8.0 +/- 0.2 microm, which is mor…

Electrospun Nanofibers in Biomedical ApplicationsPolymer Surface Interaction StudiesDendrimers and Hyperbranched Polymers

Synthesis of Organic One-Dimensional Nanomaterials by Solid-Phase Reaction

Huibiao Liu、Yuliang Li、Shengqiang Xiao 等 11 位作者2003-08-16Journal of the American Chemical Society

The synthesis of anthracene (AN) nanowires and perylene (PY) nanorods on the basis of solid-phase organic reactions under controlled conditions is discussed, and the structures are confirmed by SEM, TEM, and XRD. The dimension-dependent emission properties of the AN nanowires and PY nanorods is observed. This approach…

Carbon Nanotubes in CompositesGraphene research and applicationsFullerene Chemistry and Applications

Microdomain Morphology in an ABC 3-Miktoarm Star Terpolymer: A Study by Energy-Filtering TEM and 3D Electron Tomography

Kazuhiro Yamauchi、Keiko Takahashi、Hirokazu Hasegawa 等 12 位作者2003-08-16Macromolecules

ADVERTISEMENT RETURN TO ISSUEPREVCommunication to the...Communication to the EditorNEXTMicrodomain Morphology in an ABC 3-Miktoarm Star Terpolymer: A Study by Energy-Filtering TEM and 3D Electron TomographyKazuhiro Yamauchi, Keiko Takahashi, Hirokazu Hasegawa, Hermis Iatrou, Nikos Hadjichristidis, Takeshi Kaneko, Yuki…

Block Copolymer Self-AssemblyElectron and X-Ray Spectroscopy TechniquesSurface and Thin Film Phenomena

Frequency Dependence of Superconducting Cavity Q and Magnetic Breakdown Field

Mario Rabinowitz2003-08-16arXiv

A theoretical explanation is given to account for the unexpected observation that L- and S-band Nb superconducting cavities were found to have lower Q and lower magnetic breakdown field than those of the higher X-band frequencies. Both effects can be related to the trapping of magnetic flux in the cavity walls. The fr…

Materials ScienceSuperconductivity

Kinetic Self-Assembly of Metals on Co-polymer Templates

Ajay Gopinathan2003-08-16arXiv

In this work we seek to understand some of the fundamental processes that govern self-assembly at the nanoscale in the context of the formation of metallic structures on patterned co-polymer templates. To this end we focus on the experiments conducted by Lopes {\it et al} (Nature, 2001), where morphologies resulting f…

Materials ScienceSoft Condensed Matter

TEMPO-Mediated Oxidation of Cellulose III

Denilson da Silva Perez、Suzelei Montanari、Michel R. Vignon2003-08-16OpenAlex

Various cellulose samples converted into cellulose III by two different ammonia treatments, either liquid or gaseous, were reacted with catalytic amounts of 2,2,6,6-tetramethylpiperidine-1-oxyl radical (TEMPO), sodium hypochlorite, and sodium bromide in water. A substantial increase in the reactivity of cellulose III…

Advanced Cellulose Research StudiesEnzyme-mediated dye degradationLignin and Wood Chemistry

Wetting on Hydrophobic Rough Surfaces: To Be Heterogeneous or Not To Be?

Abraham Marmur2003-08-16OpenAlex

Equilibrium wetting on rough surfaces is discussed in terms of the “competition” between complete liquid penetration into the roughness grooves and entrapment of air bubbles inside the grooves underneath the liquid. The former is the homogeneous wetting regime, usually described by the Wenzel equation. The latter is t…

Surface Modification and SuperhydrophobicityFluid Dynamics and Heat TransferFluid Dynamics and Thin Films

Second Harmonic Generation from YAl3(BO3)4-Containing Glass-Ceramics Prepared by Thermal Poling of Y2O3–Al2O3–B2O3Glasses

Yoshitsugu Yamamoto、Tadanori Hashimoto、Hiroyuki Nasu 等 4 位作者2003-08-15Japanese Journal of Applied Physics

Transparent glass-ceramics containing YAl 3 (BO 3 ) 4 crystals were prepared by thermal poling of the Y 2 O 3 –Al 2 O 3 –B 2 O 3 glasses. Second harmonic generation could be measured from both the glass-ceramics prepared with/without applied voltage, however, intensity is markedly enhanced in the samples prepared with…

Luminescence Properties of Advanced MaterialsGlass properties and applicationsPhotorefractive and Nonlinear Optics

Mg-rich wolfeite, (FeII,Mg)2(PO4)(OH): structure refinement and Raman spectroscopic data

Uwe Kolitsch2003-08-15Acta Crystallographica Section E Structure Reports Online

Mg-rich wolfeite [diiron(II) hydro­xide phosphate], (FeII,Mg)2(PO4)(OH), from the Big Fish River area, Yukon Territory, Canada, is isotypic with its MnII-dominant analogue triploidite. The framework structure contains edge- and corner-sharing, distorted MO4(OH) and MO4(OH)2 (M = FeII or FeII,Mg) polyhedra linked by fa…

Crystal Structures and PropertiesChemical Synthesis and CharacterizationX-ray Diffraction in Crystallography

Synthesis of 2,5-Bis[(3,4-ethylenedioxy)thien-2-yl]- 3-Substituted Thiophenes

Michael F. Pepitone、K. Eaiprasertsak、Stephen S. Hardaker 等 4 位作者2003-08-15Organic Letters

[reaction: see text] Synthesis of 2,5-bis[(3,4-ethylenedioxy)thien-2-yl]-3-substituted thiophene monomers afforded compounds with blue emission characteristics and having a quantum yield of 3-5%. Cyclic voltammetry was employed to investigate the electrochemical behavior of the four monomers reported here. Polymer fil…

Organic Electronics and PhotovoltaicsOrganic Light-Emitting Diodes ResearchConducting polymers and applications

Water vapor effects on the cyclic oxidation resistance of alumina forming alloys

K. Onal、M.C. Maris-Sida、G. H. Meier 等 4 位作者2003-08-15Materials at High Temperatures

Water vapor is present in most environments in which alloys are used at elevated temperatures and there are papers in the literature that show water vapor usually has adverse effects on the oxidation resistance of alloys. However, the exact effect of water vapor is dependent on the particular alloy under consideration…

Advanced ceramic materials synthesisHigh-Temperature Coating BehaviorsIntermetallics and Advanced Alloy Properties

Microstructural evidence for counter-diffusion of aluminum and oxygen during the growth of alumina scales

V.K. Tolpygo、David R. Clarke2003-08-15Materials at High Temperatures

A novel, two-stage oxidation experiment is described that enables the outward diffusion of cations in alumina scales during high-temperature oxidation to be analyzed on the basis of microstructural changes in the surface morphology of the scale. Using this technique, observations of aluminum out-diffusion along α-Al2O…

Advanced ceramic materials synthesisCatalytic Processes in Materials ScienceHigh-Temperature Coating Behaviors

Microwave Dielectric Properties of Bi2(Zn1/3Ta2/3)2O7Polymorphs

Hee Bum Hong、Dong‐Wan Kim、Kug Sun Hong2003-08-15Japanese Journal of Applied Physics

Polymorphic phases of Bi 2 (Zn 1/3 Ta 2/3 ) 2 O 7 pyrochlore were studied. A metastable monoclinic structure was observed at temperatures below 950°C. This low-temperature phase possesses highly temperature-stable characteristics in the microwave frequency range (5–7 GHz) with a temperature coefficient of resonant fre…

Microwave Dielectric Ceramics SynthesisNuclear materials and radiation effects

Light Polarization by Cholesteric Layers

Nina P. M. Huck、Ilja Staupe、Alexandre Thirouard 等 4 位作者2003-08-15Japanese Journal of Applied Physics

A cholesteric liquid crystal layer acts as a Bragg reflector for one circular polarization at normal incidence. At oblique incidence the situation is more complex. We investigated, both numerically and experimentally, the optical behavior of a cholesteric liquid crystal layer by illuminating the layer at normal and ob…

Liquid Crystal Research AdvancementsPhotonic Crystals and ApplicationsOptical Polarization and Ellipsometry

HOUDINI: A New Approach to Computer-Based Structure Generation

A. Korytko、Kenneth Schulz、Mark S. Madison 等 4 位作者2003-08-15Journal of Chemical Information and Computer Sciences

A new method of structure generation called convergent structure generation has been developed to address limitations of earlier methods. The features of the program (HOUDINI) based on this method include the following: a single integrated representation of the collective substructural information; the use of parallel…

Computational Drug Discovery MethodsCrystallization and Solubility StudiesMachine Learning in Materials Science

Structural Evidence for the Charge Disproportionation of Fe 4+ in BaFeO 3-δ

Kazuhiro Mori、Takashi Kamiyama、Hisao Kobayashi 等 6 位作者2003-08-15Journal of the Physical Society of Japan

A weak distortion of a [FeO 6 ] octahedron was observed in hexagonal BaFeO 2.91 at around 180 K by neutron powder diffraction. The occurrence of a weak distortion is consistent with the results of Mössbauer measurements, which indicated a decrease in the Fe 4+ concentration below 170 K. We strongly suggest that the we…

High-pressure geophysics and materialsMultiferroics and related materialsAdvanced Condensed Matter Physics