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Inelastic transport in molecular spin valves

N. Jean、S. Sanvito2005-11-23arXiv

We present a study of the effects of inelastic scattering on the transport properties of various nanoscale devices, namely H$_2$ molecules sandwiched between Pt contacts, and a spin-valve made by an organic molecule attached to model half-metal ferromagnetic current/voltage probes. In both cases we use a tight-binding…

Mesoscale and Nanoscale PhysicsMaterials Science

Hydrogenation of Single-Walled Carbon Nanotubes

Anton Nikitin、Hirohito Ogasawara、Dan C. Mann 等 8 位作者2005-11-23Physical Review Letters

Towards the development of a useful mechanism for hydrogen storage, we have studied the hydrogenation of single-walled carbon nanotubes with atomic hydrogen using core-level photoelectron spectroscopy and x-ray absorption spectroscopy. We find that atomic hydrogen creates C-H bonds with the carbon atoms in the nanotub…

Carbon Nanotubes in CompositesGraphene research and applicationsHydrogen Storage and Materials

Porosity and Mechanical Properties of Mesoporous Thin Films Assessed by Environmental Ellipsometric Porosimetry

Cédric Boissière、David Grosso、Sophie Lepoutre 等 6 位作者2005-11-23OpenAlex

Mesoordered silica thin films with cubic structures were prepared by evaporation induced self-assembly (EISA) with two types of structuring agent (CTAB and block copolymer F127). A complete and accurate description of these films was obtained by combining 2D-SAXS analyses, variable angle spectroscopic ellipsometry, an…

Mesoporous Materials and CatalysisBlock Copolymer Self-AssemblyAerogels and thermal insulation

Ferroelectric and Piezoelectric Properties of Fine‐Grained Na 0.5 K 0.5 NbO 3 Lead‐Free Piezoelectric Ceramics Prepared by Spark Plasma Sintering

Jing‐Feng Li、Ke Wang、Bo‐Ping Zhang 等 4 位作者2005-11-23OpenAlex

Lead‐free piezoelectric ceramics have received attention because of increasing interest in environmental protection. Niobate ceramics such as NaNbO 3 and KNbO 3 have been studied as promising Pb‐free piezoelectric ceramics, but their sintering densification is fairly difficult. In the present study, highly dense Na 0.…

Ferroelectric and Piezoelectric MaterialsMultiferroics and related materialsAcoustic Wave Resonator Technologies

Study of Biodegradable Polylactide/Poly(butylene adipate-co-terephthalate) Blends

Long Jiang、Michael P. Wolcott、Jinwen Zhang2005-11-23OpenAlex

Both polylactide (PLA) and poly(butylene adipate-co-terephthalate) (PBAT) are biodegradable polymers. They are thermoplastics which can be processed using most conventional polymer processing methods. PLA is high in strength and modulus (63 MPa and 3.4 GPa, respectively) but brittle (strain at break 3.8%) while PBAT i…

Polymer crystallization and propertiesbiodegradable polymer synthesis and propertiesAdditive Manufacturing and 3D Printing Technologies

Quantum Spin Hall Effect in Graphene

C. L. Kane、E. J. Melé2005-11-23OpenAlex

We study the effects of spin orbit interactions on the low energy electronic structure of a single plane of graphene. We find that in an experimentally accessible low temperature regime the symmetry allowed spin orbit potential converts graphene from an ideal two-dimensional semimetallic state to a quantum spin Hall i…

Graphene research and applicationsQuantum and electron transport phenomenaTopological Materials and Phenomena

Luminescence Quenching of Eu(III) Carboxylates by Cu(II) in a Composite Polymer Xerogel Film†

Beatriz C. Barja、Amanda Remorino、Pedro F. Aramendı́a2005-11-22Photochemistry and Photobiology

Three Eu(III) luminescent compounds were separately entrapped in a xerogel porous silica matrix and finely ground particles of it were deposited on a glass support with polyvinylacetate (PVAc) as a binder to build a thin film sensor. These 3 devices were immersed in aqueous solutions of Cu(II) and the content of this…

Molecular Sensors and Ion DetectionLanthanide and Transition Metal ComplexesAnalytical Chemistry and Sensors

Coalescence in semiconcentrated emulsions in simple shear flow

Alexander V. Korobko、Dirk van den Ende、W.G.M. Agterof 等 4 位作者2005-11-22The Journal of Chemical Physics

The coalescence frequency in emulsions containing droplets with a low viscosity (viscosity ratio approximately 0.005) in simple shear flow has been investigated experimentally at several volume fractions of the dispersed phase (2%-14%) and several values of the shear rate (0.1-10 s(-1)). The evolution of the size dist…

Surfactants and Colloidal SystemsInnovative Microfluidic and Catalytic Techniques InnovationPickering emulsions and particle stabilization

Aggregated nanoparticle structures prepared by thermal decomposition of poly(vinyl)-N-pyrrolidone/Ag nanoparticle composite films

L. Rast、Andrei Stanishevsky2005-11-22Applied Physics Letters

Silver nanoparticle layers were fabricated using spin coating and rapid thermal processing of poly(vinyl)-N-pyrrolidone/Ag nanoparticle composite thin films on glass. Fast thermal degradation of the polymeric matrix at 420°C results in spontaneous aggregation of Ag nanoparticles, accompanied by strong enhancement and…

Gold and Silver Nanoparticles Synthesis and ApplicationsNanomaterials and Printing TechnologiesNonlinear Optical Materials Studies

Analysis of Interactions with Mitochondrial mRNA Using Mutant Forms of Yeast NAD+-Specific Isocitrate Dehydrogenase

Sondra L. Anderson、Anping Lin、Lee McAlister-Henn2005-11-22Biochemistry

Yeast NAD(+)-specific isocitrate dehydrogenase (IDH) is an allosterically regulated tricarboxylic acid cycle enzyme that has been shown to bind specifically and with high affinity to 5'-untranslated regions of yeast mitochondrial mRNAs. The absence of IDH has been shown to result in reduced expression of mitochondrial…

RNA Research and SplicingEnzyme Structure and FunctionBiochemical and Molecular Research

Nucleation and size distribution of nucleus during induction period of polyethylene crystallization

Narayan Chandra Das、Masamichi Hikosaka、Kiyoka Okada 等 5 位作者2005-11-22The Journal of Chemical Physics

The crystallization process from supercooled melt results in the formation of nanosize nuclei in the earlier stage (induction period) through subsequent attachment or detachment of repeating unit to nuclei. The size distribution of nucleus f(N(j),t) in the induction period of nucleation process from the melts has not…

Carbon Nanotubes in CompositesPolymer crystallization and properties

Absolute determination of inelastic mean-free paths and surface excitation parameters by absolute reflection electron energy loss spectrum analysis

T. Nagatomi、Kenta Goto2005-11-22Applied Physics Letters

An analytical approach was proposed for simultaneously determining an inelastic mean-free path (IMFP) and a surface excitation parameter (SEP) with absolute units by the analysis of an absolute experimental reflection electron energy loss spectrum. The IMFPs and SEPs in Ni were deduced for electrons of 300 to 3000 eV.…

Semiconductor materials and devicesX-ray Spectroscopy and Fluorescence AnalysisElectron and X-Ray Spectroscopy Techniques

Kinetic parameters of crystallization in glassy Se100–xSbx alloys

N. Mehta、M. Zulfequar、A. Kumar2005-11-22physica status solidi (a)

Abstract Differential scanning calorimetry (DSC) has been performed at different heating rates under non‐isothermal conditions to study the crystallization kinetics of glassy Se 100– x Sb x (2 ≤ x ≤ 10) alloys. The crystallization kinetics have been studied using four different methods of analysis of the non‐isotherma…

Phase-change materials and chalcogenidesThermal and Kinetic AnalysisChemical Thermodynamics and Molecular Structure

High-temperature orbital, charge, and structural phase transitions in the cation-ordered manganitesTbBaMn2O6andYBaMn2O6

A. J. Williams、J. Paul Attfield、Simon A. T. Redfern2005-11-22Physical Review B

The high-temperature structures and phase transitions of the cation-ordered manganite perovskites $\mathrm{Tb}\mathrm{Ba}{\mathrm{Mn}}_{2}{\mathrm{O}}_{6}$ and $\mathrm{Y}\mathrm{Ba}{\mathrm{Mn}}_{2}{\mathrm{O}}_{6}$ have been studied by powder neutron diffraction and differential scanning calorimetry. $\mathrm{Tb}\ma…

Ferroelectric and Piezoelectric MaterialsMagnetic and transport properties of perovskites and related materialsThermal Expansion and Ionic Conductivity

Quasi-Static and Dynamic Buckling of Thin Cylindrical Shape-Memory Shells

Sia Nemat‐Nasser、Jeom Yong Choi、Jon Isaacs 等 4 位作者2005-11-22Journal of Applied Mechanics

To investigate the buckling behavior of thin and relatively thick cylindrical shape-memory shells, uniaxial compression tests are performed at a 295K initial temperature, using the CEAM/UCSD’s modified split Hopkinson bar systems and an Instron hydraulic testing machine. The quasi-static buckling response of the shell…

Shape Memory Alloy TransformationsHigh-Velocity Impact and Material BehaviorStructural Analysis and Optimization

Observation of Magnetic Ripple and Nanowidth Domains in a Layered Ferromagnet

Toru Asaka、T. Kimura、Takuro Nagai 等 7 位作者2005-11-22Physical Review Letters

We investigated ferromagnetic domain structures on nanometer to micrometer scale for single crystals of a layered ferromagnet, La(2-2x)Sr(1+2x)Mn2O7 (0.32 < or = x < or = 0.40), as functions of x and temperature by means of Lorentz electron microscopy. We have succeeded in observing the evolution of magnetic ripple st…

Magnetic and transport properties of perovskites and related materialsMultiferroics and related materialsAdvanced Condensed Matter Physics

Dielectric relaxation processes in water mixtures of tripropylene glycol

K. Grzybowska、A. Grzybowski、Sebastian Pawlus 等 5 位作者2005-11-22The Journal of Chemical Physics

Broadband dielectric measurements for anhydrous tripropylene glycol (3PG) and 96, 92, 84, 80, 74, 71, and 68 wt % 3PG-water mixtures are performed in the frequency range of 10(-2)-10(7) Hz and in the temperature range of 123-243 K. We examined the effect of adding water into anhydrous 3PG on relaxation dynamics. Apart…

Material Dynamics and PropertiesThermodynamic properties of mixturesSpectroscopy and Quantum Chemical Studies

How Does Surface Modification Aid in the Dispersion of Carbon Nanofibers?

Jian Zhao、Dale W. Schaefer、Donglu Shi 等 8 位作者2005-11-22The Journal of Physical Chemistry B

Small-angle light scattering is used to assess the dispersion behavior of vapor-grown carbon nanofibers suspended in water. These data provide the first insights into the mechanism by which surface treatment promotes dispersion. Both acid-treated and untreated nanofibers exhibit hierarchical morphology consisting of s…

Carbon Nanotubes in CompositesGraphene research and applicationsNanopore and Nanochannel Transport Studies

Aging in a free-energy landscape model for glassy relaxation

Gregor Diezemann2005-11-22The Journal of Chemical Physics

The aging properties of a simple free-energy landscape model for the primary relaxation in supercooled liquids are investigated. The intermediate scattering function and the rotational correlation functions are calculated for the generic situation of a quench from a high temperature to below the glass transition tempe…

Material Dynamics and PropertiesTheoretical and Computational PhysicsAdvanced Physical and Chemical Molecular Interactions

Surface-detached V-shaped yoke of obliquely bonded magnetostrictive strips for high transduction of ultrasonic torsional waves

Chan Il Park、Woochul Kim、Seung Hyun Cho 等 4 位作者2005-11-22Applied Physics Letters

When slender magnetostrictive strips that are obliquely bonded on the surface of a pipe are subjected to a time-varying magnetic field, the strips deform mechanically because of the magnetostrictive effect and in turn, ultrasonic torsional waves are generated in the pipe. If the magnetic flux density in the strips can…

Structural Health Monitoring TechniquesUltrasonics and Acoustic Wave PropagationMagnetic Properties and Applications