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Superconducting properties ofMgCNi3films

David P. Young、Simona Moldovan、D. D. Craig 等 5 位作者2003-07-03Physical review. B, Condensed matter

We report the magnetotransport properties of thin polycrystalline films of the recently discovered nonoxide perovskite superconductor ${\mathrm{MgCNi}}_{3}.$ ${\mathrm{CNi}}_{3}$ precursor films were deposited onto sapphire substrates and subsequently exposed to Mg vapor at $700\ifmmode^\circ\else\textdegree\fi{}\math…

Rare-earth and actinide compoundsSuperconductivity in MgB2 and AlloysThermal Expansion and Ionic Conductivity

Generalized equation of phonon radiative transport

Ravi Prasher2003-07-03Applied Physics Letters

We write the equation of phonon radiative transport (EPRT) and the Boltzmann transport equation by including an in-scattering term under a relaxation time approximation. The in-scattering term contains a phase function that is exactly analogous to the phase function in the equation of radiative transport (ERT), thereb…

Numerical methods in inverse problemsThermal properties of materialsThermal Radiation and Cooling Technologies

Surface plasmon polariton modified emission of erbium in a metallodielectric grating

Jeroen Kalkman、C. Strohhöfer、Boris Gralak 等 4 位作者2003-07-03Applied Physics Letters

The spectral shape and bandwidth of the emission of Er3+ ions in silica glass around 1.5 μm is strongly modified by the presence of a silver grating. The metallodielectric grating was made by a sequence of ion implantation in silica glass, dry etching, and silver sputter deposition. Spectral enhancements are observed…

Photonic and Optical DevicesPhotonic Crystals and ApplicationsOptical Coatings and Gratings

Step Line Tension on a Metal Electrode

H. Ibach、Wolfgang Schmickler2003-07-03Physical Review Letters

The step line tension in electrochemical systems differs conceptually from the line tension on metals in the vacuum because it refers to different boundary conditions. A procedure is established for calculating the electrochemical line tension and is applied to a novel model of the interface comprising both a stepped…

Corrosion Behavior and InhibitionForce Microscopy Techniques and ApplicationsSurface and Thin Film Phenomena

Low-temperature structural and Raman studies on rare-earth gallates

D. Savytskii、L. Vasylechko、Anatoliy Senyshyn 等 8 位作者2003-07-03Physical review. B, Condensed matter

Measurements of lattice parameters and structural refinement were made for a ${\mathrm{LaGaO}}_{3},$ ${\mathrm{PrGaO}}_{3},$ ${\mathrm{NdGaO}}_{3},$ ${\mathrm{La}}_{0.34}{\mathrm{Pr}}_{0.33}{\mathrm{Nd}}_{0.33}{\mathrm{GaO}}_{3},$ and ${\mathrm{La}}_{0.63}{\mathrm{Nd}}_{0.37}{\mathrm{GaO}}_{3}$ samples by powder-diffr…

Luminescence Properties of Advanced MaterialsMagnetic and transport properties of perovskites and related materialsThermal Expansion and Ionic Conductivity

Physicochemical Properties of Fluorinated Diamond Electrodes

Sergio Ferro、Achille De Battisti2003-07-03The Journal of Physical Chemistry B

Although boron-doped diamond (BDD) is itself quite stable and chemically inert, some electrochemical applications could require further improvement, and fluorination could be one of the most promising methods. In the present paper, a characterization of diamond film electrodes surface-modified by fluorine insertion, t…

Semiconductor materials and devicesDiamond and Carbon-based Materials ResearchAnalytical Chemistry and Sensors

High-mobility thin-film transistors based on aligned carbon nanotubes

Kai Xiao、Yunqi Liu、PingAn Hu 等 6 位作者2003-07-03Applied Physics Letters

Thin-film transistors based on aligned carbon nanotubes (CNTs) were fabricated by directly growing highly ordered CNTs on silicon dioxide surface. The transistor shows a pronounced field effect. Electric transport through the aligned carbon nanotubes is dominated by the holes at room temperature. A hole mobility (μp)…

Carbon Nanotubes in CompositesDiamond and Carbon-based Materials ResearchNanowire Synthesis and Applications

Static Water Structure Detected by Heat Capacity Measurements on Aqueous Solutions of a Triple-Helical Polysaccharide Schizophyllan

Kazuto Yoshiba、Akio Teŕamoto、Naotake Nakamura 等 6 位作者2003-07-03Biomacromolecules

Heat capacity measurements were made on aqueous solutions of a triple-helical polysaccharide schizophyllan by precision adiabatic calorimetry over a wide range of concentrations 30.45-90.93 wt % at temperatures between 5 and 315 K. The heat capacity curves obtained were divided into four groups depending on the weight…

Liquid Crystal Research AdvancementsMaterial Dynamics and PropertiesSurfactants and Colloidal Systems

Laser site-selective excitation spectroscopy ofEu3+-doped yttrium aluminum garnet

Yongrong Shen、ChunMao Li、Vilma C. Costa 等 4 位作者2003-07-03Physical review. B, Condensed matter

We report the results for laser site selective excitation spectroscopy of ${\mathrm{Eu}}^{3+}$-doped yttrium aluminum garnet. We identified four primary luminescent centers (A--D) from the ${}^{7}{\stackrel{\ensuremath{\rightarrow}}{{F}_{0}}}^{5}{D}_{0}$ excitation spectra and, from the ${}^{5}{\stackrel{\ensuremath{\…

Luminescence Properties of Advanced MaterialsGlass properties and applicationsSolid State Laser Technologies

Clarification of oxygen bonding on diamond surfaces by low energy electron stimulated desorption and high resolution electron energy loss spectroscopy

A. Laikhtman、A. Lafosse、Y. Le Coat 等 5 位作者2003-07-03The Journal of Chemical Physics

In this work we correlate between O− electron stimulated desorption (ESD) from hydrogenated and bare polycrystalline diamond films exposed to thermally activated oxygen for incident electron energies in the 4–23 eV range and vibrational electron energy losses. By utilizing the previously established mechanism of low e…

Metal and Thin Film MechanicsSemiconductor materials and devicesDiamond and Carbon-based Materials Research

Through‐Space Delocalized Water‐Soluble Paracyclophane Bichromophores: New Fluorescent Optical Reporters

Janice W. Hong、Hadjar Benmansour、Guillermo C. Bazan2003-07-03Chemistry - A European Journal

Conjugated polymers and oligomers can serve as highly responsive fluorescent reporters for biosensor applications. However, their optical properties in aqueous media are highly dependent upon environmental conditions. The structure of the paracyclophane framework provides a platform for designing optical reporters tha…

Supramolecular Chemistry and ComplexesLuminescence and Fluorescent MaterialsSupramolecular Self-Assembly in Materials

Pore size distribution, survival probability, and relaxation time in random and ordered arrays of fibers

Manolis M. Tomadakis、Teri J. Robertson2003-07-03The Journal of Chemical Physics

We present a random walk based investigation of the pore size probability distribution and its moments, the survival probability and mean survival time, and the principal relaxation time, for random and ordered arrays of cylindrical fibers of various orientation distributions. The dimensionless mean survival time, pri…

Material Dynamics and PropertiesTheoretical and Computational PhysicsNMR spectroscopy and applications

Controllable optical properties of Au/SiO2 nanocomposite induced by ultrasonic irradiation and thermal annealing

Ganhua Fu、Weiping Cai、Caixia Kan 等 5 位作者2003-07-03Applied Physics Letters

Nanostructured gold/monolithic mesoporous silica assembly was synthesized by a sonochemical method. The optical absorption maximum of the as-prepared nanocomposite varies from the visible to near-infrared region, depending on the reduction rate of AuCl4− ions in solution. There exists a critical reduction rate of AuCl…

Gold and Silver Nanoparticles Synthesis and ApplicationsNonlinear Optical Materials StudiesLaser-Ablation Synthesis of Nanoparticles

Pulsation and Bouncing of a Bubble Prior to Rupture and/or Foam Film Formation

Marcel Krzan、K. Lunkenheimer、K. Małysa2003-07-03Langmuir

When a bubble rising in distilled water or in an aqueous pentanol-1 solution approached the air/water interface, rapid pulsations of its shape with a frequency of more than 1000 Hz were observed. In addition, the bubble bounced from the free surface, prior to its rupture or to the formation of a foam film. It is rathe…

Enhanced Oil Recovery TechniquesMinerals Flotation and Separation TechniquesPickering emulsions and particle stabilization

Effect of cyclic chain architecture on properties of dilute solutions of polyethylene from molecular dynamics simulations

Seung Soon Jang、Tahir Çağın、William A. Goddard2003-07-03The Journal of Chemical Physics

We have used molecular dynamics methods to investigate the effects of cyclic chain architecture on the properties of dilute solutions. In order to include solvent effects in estimating these properties, we use a van der Waals scaling factor determined for each solvent by matching to the theta condition. We predict tha…

Protein Structure and DynamicsPolymer crystallization and propertiesMaterial Dynamics and Properties

The crystal structure of methane phase III

Marcus A. Neumann、W. Press、C. Nöldeke 等 6 位作者2003-07-03The Journal of Chemical Physics

Methane is the simplest organic molecule, and like many supposedly simple molecular materials it has a rich phase diagram. While crystal structures could be determined for two of the solid phases, that of the low temperature phase III remained unsolved. Using high-resolution neutron powder diffraction and a direct-spa…

High-pressure geophysics and materialsCrystallography and molecular interactionsX-ray Diffraction in Crystallography

Determination of the interaction potential from the pair distribution function: An inverse Monte Carlo technique

N. G. Almarza、E. Lomba2003-07-03Physical review. E, Statistical physics, plasmas, fluids, and related interdisciplinary topics

In this work we present an efficient procedure to evaluate effective pair potentials compatible with "experimental" distribution functions using a Monte Carlo simulation scheme. Using computer simulation results for the pair distribution functions, we have applied the method to a Lennard-Jones fluid and to a model of…

Phase Equilibria and ThermodynamicsMaterial Dynamics and PropertiesTheoretical and Computational Physics

Influences of the surface reactions on the field emission from multiwall carbon nanotubes

Changkun Dong、Mool C. Gupta2003-07-03Applied Physics Letters

Field emission characteristics from multiwall carbon nanotubes were studied under various gas environments. The experiments on field emission revealed several surface reactions under high-vacuum operating conditions. The Fowler–Nordheim (F–N) analysis showed a field emission regime dominated by the surface adsorbents,…

Carbon Nanotubes in CompositesGraphene research and applicationsDiamond and Carbon-based Materials Research

Collapsing Cristobalitelike Structures in Silica Analogues at High Pressure

Julien Haines、C. Chateau、Jean‐Michel Léger 等 7 位作者2003-07-03Physical Review Letters

The cristobalitelike forms of the ternary silica analogues BPO4 and BAsO4 were investigated at high pressure by x-ray diffraction and theoretical methods. The behavior of these compounds represents an extreme case in which the tilt angle of the constituent tetrahedra increases in a spectacular way at high pressure res…

Zeolite Catalysis and SynthesisGlass properties and applicationsCrystal Structures and Properties

Different dynamic and static magnetic anisotropy in thin Permalloy™ films

R. Lopušnı́k、J. P. Nibarger、T. J. Silva 等 4 位作者2003-07-03Applied Physics Letters

The values of uniaxial anisotropy Hk in thin polycrystalline Permalloy™ films measured by static and dynamic methods differ by as much as a factor of 1.5. The anisotropy obtained with a pulsed inductive microwave magnetometer in 2.5 to 100 nm thick Permalloy films exhibits an additional isotropic component of 120 to 2…

Magnetic properties of thin filmsTheoretical and Computational PhysicsMagnetic Properties and Applications