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Theoretical models for ultrashort electromagnetic pulse propagation in nonlinear metamaterials

Shuangchun Wen、Yuanjiang Xiang、Xiaoyu Dai 等 6 位作者2007-03-27Physical Review A

A metamaterial (MM) differs from an ordinary optical material mainly in that it has a dispersive magnetic permeability and offers greatly enhanced design freedom to alter the linear and nonlinear properties. This makes it possible for us to control the propagation of ultrashort electromagnetic pulses at will. Here we…

Metamaterials and Metasurfaces ApplicationsOrbital Angular Momentum in OpticsTerahertz technology and applications

Unexpected Structures of Aluminum Oxide Clusters in the Gas Phase

Marek Sierka、Jens Döbler、Joachim Sauer 等 9 位作者2007-03-27Angewandte Chemie International Edition

No family resemblance: IR photodissociation experiments and DFT optimizations implementing a genetic algorithm suggest that small aluminum oxide clusters have unusual structures in the gas phase. For example, the structure proposed for [(Al2O3)4]+ (see picture; Al black, O gray) has no features in common with bulk alu…

ZnO doping and propertiesCatalytic Processes in Materials ScienceCatalysis and Oxidation Reactions

Antiferromagnetic Interactions in Single CrystallineZn1−xCoxOThin Films

P. Sati、C. Deparis、C. Morhain 等 5 位作者2007-03-27Physical Review Letters

In a rather contradictory situation regarding magnetic data on Co-doped ZnO, we have succeeded in fabricating high-quality single crystalline Zn(1-x)Co(x)O (x=0.003-0.07) thin films. This gives us the possibility, for the first time, to examine the intrinsic magnetic properties of ZnO:Co at a quantitative level and th…

ZnO doping and propertiesGas Sensing Nanomaterials and SensorsMagnetic and transport properties of perovskites and related materials

Ultrasound‐Triggered Release from Multilayered Capsules

Bruno G. De Geest、André G. Skirtach、Arif A. Mamedov 等 7 位作者2007-03-27Small

Sound effects: Multilayered capsules, such as that shown in the SEM image, are promising vehicles for the delivery of macromolecular drugs. Ultrasonic irradiation can be used to trigger the release of encapsulated species from capsules fabricated using layer-by-layer technology. Ultrasound affects the integrity of the…

Electrospun Nanofibers in Biomedical ApplicationsPolymer Surface Interaction StudiesNanofabrication and Lithography Techniques

Pseudodiffusive magnetotransport in graphene

Elsa Prada、Pablo San-Jose、Bernhard Wünsch 等 4 位作者2007-03-27Physical Review B

Transport properties through wide and short ballistic graphene junctions are studied in the presence of arbitrary dopings and magnetic fields. No dependence on the magnetic field is observed at the Dirac point for any current cumulant, just as in a classical diffusive system, both in normal-graphene-normal and normal-…

Graphene research and applicationsQuantum and electron transport phenomenaTopological Materials and Phenomena

Magnetically Induced Field Effect in Carbon Nanotube Devices

Georgy Fedorov、Alexander Tselev、David Jiménez 等 8 位作者2007-03-27Nano Letters

Three-terminal devices with conduction channels formed by quasi-metallic carbon nanotubes (CNTs) are shown to operate as nanotube-based field-effect transistors under strong magnetic fields. The off-state conductance of the devices varies exponentially with the magnetic flux intensity. We extract the quasi-metallic CN…

Carbon Nanotubes in CompositesGraphene research and applicationsQuantum and electron transport phenomena

Synthesis and characterization of novel conducting composites of Fe3O4 nanoparticles and sulfonated polyanilines

Kakarla Raghava Reddy、Kwang‐Pill Lee、Anantha Gopalan Iyengar2007-03-27Journal of Applied Polymer Science

Abstract Surface charged iron oxide (Fe 3 O 4 ) nanoparticles were used for the synthesis of sulfonated polyaniline (SPAN)‐Fe 3 O 4 nanocomposites (SPAN/Fe 3 O 4 ‐NCs). 2,5‐diaminobenzenesulfonic acid (DABSA) and 2‐aminobenzenesulfonic acid (ABSA) were independently polymerized with aniline to form SPAN. The structure…

Supercapacitor Materials and FabricationAdvanced Sensor and Energy Harvesting MaterialsConducting polymers and applications

Preparation of nanoparticles composed of chitosan and its derivatives as delivery systems for macromolecules

Yan Sun、Ajun Wan2007-03-27Journal of Applied Polymer Science

Abstract Three different kinds of nanoparticles for paracellular transport were prepared using a simple and mild ionic‐gelation method. Sodium tripolyphosphate (TPP) as crosslinking agent was added into three kinds of solutions, which were chitosan solution, physical blending solution of chitosan, and glycidyl trimeth…

Nanocomposite Films for Food PackagingPolymer Surface Interaction StudiesAdvanced Drug Delivery Systems

Thermal Conductivity Measurements of Semitransparent Single-Walled Carbon Nanotube Films by a Bolometric Technique

Mikhail E. Itkis、Ferenc Borondics、Aiping Yu 等 4 位作者2007-03-27Nano Letters

We introduce a new technique for measurement of the thermal conductivity of ultrathin films of single-walled carbon nanotubes (SWNTs) utilizing IR radiation as heat source and the SWNT film as thermometer. The technique is applied to study the temperature dependence of the thermal conductivity of an as-prepared SWNT f…

Carbon Nanotubes in CompositesThermal properties of materialsThermal Radiation and Cooling Technologies

Electronic phase separation in manganite-insulator interfaces

L. Brey2007-03-27Physical Review B

Using a realistic microscopic model, we study the electric and magnetic properties of the interface between a half-metallic manganite and an insulator. We find that the lack of carriers at the interface attenuates the double-exchange mechanism, weakening the ferromagnetic coupling between the Mn ions. In this situatio…

Magnetic and transport properties of perovskites and related materialsAdvanced Condensed Matter PhysicsElectronic and Structural Properties of Oxides

Understanding the Insulating Phase in Colossal Magnetoresistance Manganites: Shortening of the Jahn-Teller Long-Bond across the Phase Diagram of La 1 − x Ca x MnO 3

Emil S. Božin、M. Schmidt、Adam DeConinck 等 9 位作者2007-03-27Physical Review Letters

The detailed evolution of the magnitude of the local Jahn-Teller (JT) distortion in La(1-x)Ca(x)MnO3 is obtained across the phase diagram for 0< or =x< or =0.5 from high-quality neutron diffraction data using the atomic pair distribution function method. A local JT distortion is observed in the insulating phase for al…

Magnetic and transport properties of perovskites and related materialsRare-earth and actinide compoundsAdvanced Condensed Matter Physics

Molecular microelectrostatic view on electronic states near pentacene grain boundaries

Stijn Verlaak、Paul Heremans2007-03-27Physical Review B

Grain boundaries are the most inevitable and pronounced structural defects in pentacene films. To study the effect of those structural defects on the electronic state distribution, the energy levels of a hole on molecules at and near the defect have been calculated using a submolecular self-consistent-polarization-fie…

Organic Electronics and PhotovoltaicsForce Microscopy Techniques and ApplicationsChemical and Physical Properties of Materials

Absorption Spectroscopy of Individual Single-Walled Carbon Nanotubes

Stéphane Berciaud、Laurent Cognet、Philippe Poulin 等 5 位作者2007-03-27Nano Letters

Current methods for producing single-walled carbon nanotubes (SWNTs) lead to heterogeneous samples containing mixtures of metallic and semiconducting species with a variety of lengths and defects. Optical detection at the single nanotube level should thus offer the possibility to examine these heterogeneities provided…

Carbon Nanotubes in CompositesBoron and Carbon Nanomaterials ResearchChemical and Physical Properties of Materials

Mesoscopic structures and 2D hole systems in fully field effect controlled heterostructures

R. L. Willett、M. J. Manfra、L. N. Pfeiffer 等 4 位作者2007-03-27arXiv

Two fundamental extensions to the function of previously described fully field effect two-dimensional (2D) electron heterostructures are presented: First, using the same basic heterostructure design of lithographically defined contacts overlain by both an insulating layer and top-gate employed for electron systems, ap…

Mesoscale and Nanoscale PhysicsMaterials Science

Band insulator to Mott insulator transition in a bilayer Hubbard model

S. S. Kancharla、S. Okamoto2007-03-27arXiv

The ground state phase diagram of the half-filled repulsive Hubbard model in a bilayer is investigated using cluster dynamical mean field theory. For weak to intermediate values of Coulomb repulsion $U$, the system undergoes a transition from a Mott insulating phase to a metallic phase and then onto a band insulating…

Materials ScienceStrongly Correlated Electrons

Thermogravimetric analysis of chitosan

Pengzhi Hong、Si‐Dong Li、Chunyan Ou 等 6 位作者2007-03-27Journal of Applied Polymer Science

Abstract The thermal degradation of chitosan at different heating rates B in nitrogen was studied by thermogravimetric analysis. The results indicate that the thermal degradation of chitosan in nitrogen is a one‐step reaction. The degradation temperatures increase with B . Experimentally, the initial degradation tempe…

Nanocomposite Films for Food PackagingThermal and Kinetic AnalysisAntimicrobial agents and applications

Impurity-doping-induced ferroelectricity in the frustrated antiferromagnetCuFeO2

S. Seki、Yuichi Yamasaki、Yuki Shiomi 等 6 位作者2007-03-27Physical Review B

Dielectric responses have been investigated on the triangular-lattice antiferromagnet $\mathrm{Cu}\mathrm{Fe}{\mathrm{O}}_{2}$ and its site-diluted analogs $\mathrm{Cu}{\mathrm{Fe}}_{1\ensuremath{-}x}{\mathrm{Al}}_{x}{\mathrm{O}}_{2}$ ($x=0.01$ and 0.02) with and without the application of the magnetic field. We have…

Magnetic and transport properties of perovskites and related materialsMultiferroics and related materialsAdvanced Condensed Matter Physics

ParamagneticGaN:Feand ferromagnetic(Ga,Fe)N: The relationship between structural, electronic, and magnetic properties

A. Bonanni、M. Kiecana、Clemens Simbrunner 等 13 位作者2007-03-27Physical Review B

We report on the metalorganic chemical vapor deposition of $\mathrm{GaN}:\mathrm{Fe}$ and $(\mathrm{Ga},\mathrm{Fe})\mathrm{N}$ layers on $c$-sapphire substrates and their thorough characterization via high-resolution x-ray diffraction, transmission electron microscopy (TEM), spatially resolved energy dispersive x-ray…

ZnO doping and propertiesGaN-based semiconductor devices and materialsGa2O3 and related materials

Valence-band mixing in first-principles envelope-function theory

Bradley A. Foreman2007-03-27arXiv

This paper presents a numerical implementation of a first-principles envelope-function theory derived recently by the author [B. A. Foreman, Phys. Rev. B 72, 165345 (2005)]. The examples studied deal with the valence subband structure of GaAs/AlAs, GaAs/Al(0.2)Ga(0.8)As, and In(0.53)Ga(0.47)As/InP (001) superlattices…

Materials Science

Choosing a basis that eliminates spurious solutions in k.p theory

Bradley A. Foreman2007-03-27arXiv

A small change of basis in k.p theory yields a Kane-like Hamiltonian for the conduction and valence bands of narrow-gap semiconductors that has no spurious solutions, yet provides an accurate fit to all effective masses. The theory is shown to work in superlattices by direct comparison with first-principles density-fu…

Materials Science