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A theoretical analysis of Ballistic Electron Emission Microscopy: k-space distributions and spectroscopy

P. L. de Andres、K. Reuter、F. J. Garcia-Vidal 等 5 位作者1997-10-09arXiv

We analyze BEEM experiments. At low temperatures and low voltages, near the threshold value of the Schottky barrier, the BEEM current is dominated by the elastic component. Elastic scattering by the lattice results in the formation of focused beams and narrow lines in real space. To obtain the current injected in the…

Materials Science

Stabilized Spin-Polarized Jellium Model and Odd-Even Alternations in Jellium Metal Clusters

M. Payami、N. Nafari1997-10-09arXiv

In this paper, we have considered the mechanical stability of a jellium system in the presence of spin degrees of freedom and have generalized the stabilized jellium model, introduced by J. P. Perdew, H. Q. Tran, and E. D. Smith [Phys. Rev. B42, 11627 (1990)], to a spin-polarized case. By applying this generalization…

Materials Sciencephysics.atm-clusChemical Physics

Dynamic Local Distortions in Ferroelectrics

H. Krakauer、R. Yu、C. -Z. Wang 等 5 位作者1997-10-09arXiv

Molecular-dynamics simulations of KNbO$_3$ reveal preformed dynamic chain-like structures, present even in the paraelectric phase, that are related to the softening of phonon branches over large regions of the Brillouin zone. The phase sequence of ferroelectric transitions is correctly reproduced, showing that the fir…

Materials Science

Luminescence spectroscopy of atomic zinc in rare-gas solids. I

Veronica A. Bracken、P. Gürtler、John G. McCaffrey1997-10-08The Journal of Chemical Physics

Steady-state and time-resolved luminescence spectroscopy of atomic zinc isolated in thin film samples of the solid rare gases, prepared by the cocondensation of zinc vapor with argon, krypton, and xenon has been recorded at 6.3 K using synchrotron radiation. Pairs of emission bands result from photoexcitation of the s…

Advanced Chemical Physics StudiesLuminescence Properties of Advanced MaterialsInorganic Fluorides and Related Compounds

Dynamics of polyisoprene in star block copolymers confined in microstructures: A dielectric spectroscopy study

George Floudas、Stella Paraskeva、Nikos Hadjichristidis 等 6 位作者1997-10-08The Journal of Chemical Physics

Dielectric spectroscopy has been employed to study selectively the local and global dynamics of polyisoprene (PI) in three microphase separated star diblock copolymers (SI)4, where PI and polystyrene (PS) form the core and corona, respectively. The thermally induced order-to-disorder transition (ODT) has been identifi…

Material Dynamics and PropertiesRheology and Fluid Dynamics StudiesBlock Copolymer Self-Assembly

Fluctuation theory of diblock copolymer/homopolymer blends and its effects on the Lifshitz point

L. Kielhorn、M. Muthukumar1997-10-08The Journal of Chemical Physics

We have considered the stability of lamellar, cylindrical, and spherical morphologies of a ternary melt system of A homopolymers, B homopolymers, and AB diblock copolymers in the weak segregation limit. We have extended the mean field analysis by including composition fluctuations in a one-loop self-consistent approxi…

Theoretical and Computational PhysicsRheology and Fluid Dynamics StudiesBlock Copolymer Self-Assembly

Realistic grand canonical Monte Carlo surface simulation: application to Ar(111)

Franck Celestini、Daniele Passerone、Furio Ercolessi 等 4 位作者1997-10-08arXiv

Most realistic, off-lattice surface simulations are done canonically--- conserving particles. For some applications, however, such as studying the thermal behavior of rare gas solid surfaces, these constitute bad working conditions. Surface layer occupancies are believed to change with temperature, particularly at pre…

Materials Science

Manifestation of quantum chaos on scattering techniques: application to low-energy and photo-electron diffraction intensities

P. L. de Andres、J. A. Vergés1997-10-08arXiv

Intensities of LEED and PED are analyzed from a statistical point of view. The probability distribution is compared with a Porter-Thomas law, characteristic of a chaotic quantum system. The agreement obtained is understood in terms of analogies between simple models and Berry's conjecture for a typical wavefunction of…

chao-dynMaterials Sciencecond-mat.stat-mechnlin.CD

Electric field effects in STM imaging

Kurt Stokbro、Ulrich Quaade、Francois Grey1997-10-08arXiv

We present a high voltage extension of the Tersoff-Hamann theory of STM images, which includes the effect of the electric field between the tip and the sample. The theoretical model is based on first principles electronic structure calculations and has no adjustable parameters. We use the method to calculate theoretic…

Materials Science

The selection of mechanical actuators based on performance indices

John E. Huber、N.A. Fleck、M. F. Ashby1997-10-08OpenAlex

A method is presented for selecting the type of actuator best suited to a given task, in the early stages of engineering design. The selection is based on matching performance characteristics of the actuator, such as force and displacement, to the requirements of the given task. The performance characteristics are est…

Shape Memory Alloy TransformationsAeroelasticity and Vibration ControlTopology Optimization in Engineering

ChemInform Abstract: Highly Efficient Epoxidation of Olefins Using Aqueous H2O2 and Catalytic Methyltrioxorhenium/Pyridine: Pyridine‐Mediated Ligand Acceleration.

Joachim Rudolph、K. Laxmi Reddy、Jay P. Chiang 等 4 位作者1997-10-07ChemInform

Abstract ChemInform is a weekly Abstracting Service, delivering concise information at a glance that was extracted from about 100 leading journals. To access a ChemInform Abstract of an article which was published elsewhere, please select a “Full Text” option. The original article is trackable via the “References” opt…

Porphyrin and Phthalocyanine ChemistryPolyoxometalates: Synthesis and ApplicationsOxidative Organic Chemistry Reactions

Photovoltaic effects from porous Si

B. Ünal、S. C. Bayliss1997-10-07Journal of Physics D Applied Physics

The photovoltaic (PV) effects from sandwiched porous silicon (PS), fabricated using electrochemical etching processes, have been investigated. Contacts were made by bonding to semi-transparent coatings of Au via a secondary supportive Al contact. The contribution of the PV effects from the junctions of the metal (Au)/…

Semiconductor materials and devicesSilicon Nanostructures and PhotoluminescenceNanowire Synthesis and Applications

Oscillatory Instability, Limit Cycle, and Transition to Doublets in Directional Solidification

Marc Georgelin、Alain Pocheau1997-10-06Physical Review Letters

An oscillatory instability is experimentally evidenced in directional solidification of nominally pure succinonitrile in a unity P\'eclet number regime. It involves long-time oscillations of both cell width and cell tip position in a nearly phase quadrature and at a wavelength equal to twice the cell spacing. The inst…

Solidification and crystal growth phenomenaNonlinear Dynamics and Pattern FormationFluid Dynamics and Thin Films

Reduced bias growth of pure-phase cubic boron nitride

Dmitri Litvinov、Roy Clarke1997-10-06Applied Physics Letters

We report results on an improved growth process for cubic boron nitride (c-BN) films. The films are deposited on a dc-biased silicon substrate using ion-assisted sputtering. First, we grow a BN template layer at a bias voltage which maximizes the sp3 content. After this template layer attains a thickness of ∼500 Å, co…

Metal and Thin Film MechanicsDiamond and Carbon-based Materials ResearchBoron and Carbon Nanomaterials Research

Antiferromagnetic Resonance in the Linear Chain Conducting PolymersRbC60andCsC60

A. Jánossy、N. M. Nemes、T. Fehér 等 6 位作者1997-10-06Physical Review Letters

Antiferromagnetic resonance has been observed in powders of the conducting alkali fulleride linear polymers, ${\mathrm{RbC}}_{60}$ and ${\mathrm{CsC}}_{60}$, at high frequencies (75, 150, and 225 GHz). This is proof for an antiferromagnetically ordered ground state and shows that these systems are not spin glasses. Th…

Magnetism in coordination complexesFullerene Chemistry and ApplicationsOrganic and Molecular Conductors Research

Increased radiative lifetime of rare earth-doped zinc oxyhalide tellurite glasses

David L. Sidebottom、Michael A. Hruschka、B. G. Potter 等 4 位作者1997-10-06Applied Physics Letters

We have investigated the structural and optical properties of rare earth-doped zinc tellurite glasses modified by the substitution of ZnF2. Raman and phonon sideband spectroscopies were employed to characterize changes in the glass structure as well as to probe vibrational behavior in the immediate vicinity of the rar…

Luminescence Properties of Advanced MaterialsGlass properties and applicationsOptical properties and cooling technologies in crystalline materials

Electromechanical properties of SrBi2Ta2O9 thin films

Andréi L. Kholkin、K.G. Brooks、N. Setter1997-10-06Applied Physics Letters

Weak field piezoelectric coefficient and strain were investigated in ferroelectric SrBi2Ta2O9 (SBT) thin films by means of optical interferometry. Though the maximum polarization and dielectric constant were small enough (7 μC/cm2 and 150, respectively), the piezoelectric coefficient attained 17 pm/V under the dc elec…

Ferroelectric and Piezoelectric MaterialsUltrasonics and Acoustic Wave PropagationAcoustic Wave Resonator Technologies

Suppression of ferroelectric polarization by an adjustable depolarization field

Charles T. Black、C. E. Farrell、Thomas J. Licata1997-10-06Applied Physics Letters

We have measured the effect of a depolarizing field on the properties of a ferroelectric capacitor. By systematically adjusting the amount of charge available to compensate the polarization, we can control the strength of the field inside the ferroelectric. We find that even a few percent of uncompensated polarization…

Ferroelectric and Piezoelectric MaterialsMultiferroics and related materialsAcoustic Wave Resonator Technologies

Theory of Size-Dependent Resonance Raman Scattering from Carbon Nanotubes

Ernst Richter、K. R. Subbaswamy1997-10-06Physical Review Letters

Raman scattering from single-walled carbon nanotubes is examined in detail theoretically and compared with experiments. Within a simple tight-binding model the Raman matrix elements are evaluated explicitly, and the shape of the resonance in the scattered intensity due to interband electronic transitions is derived. T…

Carbon Nanotubes in CompositesGraphene research and applicationsMechanical and Optical Resonators

Slater model applied to polarization graded ferroelectrics

J. V. Mantese、Norman W. Schubring、Adolph L. Micheli 等 7 位作者1997-10-06Applied Physics Letters

Ferroelectric thin films of BaxSr1−xTiO3 with compositional gradients normal to the growth surface have been formed by the successive deposition and annealing of films having step-variable Ba to Sr ratios. By suitably tailoring the magnitude and sense of the gradient in Ba to Sr ratio, directional potentials can be bu…

Ferroelectric and Piezoelectric MaterialsMultiferroics and related materialsAcoustic Wave Resonator Technologies