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Efficient organic-inorganic hybrid Schottky solar cell: The role of built-in potential

Yawen Zhu、Tao Song、Fute Zhang 等 5 位作者2013-03-18Applied Physics Letters

The organic-inorganic hybrid Schottky solar cells based on solution processed poly(3,4-ethlenedioxythiophene):poly(styrenesulfonate) (PEDOT:PSS) in combination with silicon offer the merits of simple fabrication process and potential low cost. Here, we demonstrate that the work function (WF) of PEDOT:PSS films plays a…

Organic Electronics and PhotovoltaicsConducting polymers and applicationsSemiconductor materials and interfaces

Highly Fluorescent and Stable Quantum Dot-Polymer-Layered Double Hydroxide Composites

Seungho Cho、Jungheon Kwag、Sanghwa Jeong 等 5 位作者2013-03-18Chemistry of Materials

We report a designed strategy for a synthesis of highly luminescent and photostable composites by incorporating quantum dots (QDs) into layered double hydroxide (LDH) matrices without deterioration of a photoluminescence (PL) efficiency of the fluorophores during the entire processes of composite formations. The QDs s…

Luminescence Properties of Advanced MaterialsQuantum Dots Synthesis And PropertiesLayered Double Hydroxides Synthesis and Applications

Can Surface Plasmon Fields Provide a New Way to Photosensitize Organic Photoreactions? From Designer Nanoparticles to Custom Applications

J. C. Scaiano、Kevin G. Stamplecoskie2013-03-18The Journal of Physical Chemistry Letters

In this Perspective, we explore the opportunities that plasmon excitation may offer for the practitioners in organic chemistry. Beyond the interesting physical properties and lively colors of colloidal solutions of noble metal nanostructures, excitation of plasmon transitions can trigger a variety of processes, from t…

Gold and Silver Nanoparticles Synthesis and ApplicationsPhotochromic and Fluorescence ChemistryNanocluster Synthesis and Applications

Observation of suppressed terahertz absorption in photoexcited graphene

Alex Frenzel、Chun Hung Lui、Wenjing Fang 等 8 位作者2013-03-18Applied Physics Letters

When light is absorbed by a semiconductor, photoexcited charge carriers enhance the absorption of far-infrared radiation due to intraband transitions. We observe the opposite behavior in monolayer graphene, a zero-gap semiconductor with linear dispersion. By using time domain terahertz (THz) spectroscopy in conjunctio…

Graphene research and applicationsPhotonic Crystals and ApplicationsThermal Radiation and Cooling Technologies

Substituent Group Variations Directing the Molecular Packing, Electronic Structure, and Aggregation-Induced Emission Property of Isophorone Derivatives

Zheng Zheng、Zhipeng Yu、Mingdi Yang 等 8 位作者2013-03-18The Journal of Organic Chemistry

A series of new isophorone derivatives (1-5), incorporating the heterocyclic ring or aza-crown-ether group, with large Stokes shifts (>140 nm), have been synthesized and characterized. 1-4 display aggregation-induced emission behaviors, while dye 5 is highly emissive in solution but quenched in the solid state. It was…

Molecular Sensors and Ion DetectionNanoplatforms for cancer theranosticsLuminescence and Fluorescent Materials

Responsive Janus Composite Nanosheets

Haili Yang、Fuxin Liang、Xing Wang 等 10 位作者2013-03-18Macromolecules

A general approach is proposed to synthesize Janus polymer/inorganic composite nanosheets. Onto the amine-group-terminated side of the Janus inorganic nanosheets, initiators are covalently bonded. By a favorable grafting from initiator-terminated side, responsive polymers, for example PDEAEMA and PNIPAM, are synthesiz…

Advanced Polymer Synthesis and CharacterizationSurfactants and Colloidal SystemsPickering emulsions and particle stabilization

Development of stress-induced curved actuators for a tunable THz filter based on double split-ring resonators

Yu‐Sheng Lin、You Qian、Fusheng Ma 等 6 位作者2013-03-18Applied Physics Letters

Using stress-induced curved cantilevers to form double split-ring resonator (DSRR) in three-dimensional configuration, an electrically tunable microelectromechanical system (MEMS) based out-of-plane metamaterials THz filter is experimentally demonstrated and characterized. While the achieved tunable range for the reso…

Metamaterials and Metasurfaces ApplicationsMicrowave Engineering and WaveguidesAcoustic Wave Resonator Technologies

Role of graphene defects in corrosion of graphene-coated Cu(111) surface

I. Własny、P. Dąbrowski、Maciej Rogala 等 8 位作者2013-03-18Applied Physics Letters

Protection of Cu(111) surface by chemical vapor deposition graphene coating is investigated. The X-ray photoemission spectroscopy results do not reveal any signs of corrosion on graphene-coated Cu(111), and suggest perfect protection of copper surface against interaction with atmospheric gases. However, the scanning t…

Graphene research and applicationsDiamond and Carbon-based Materials ResearchIon-surface interactions and analysis

Tunable Carrier Type and Density in Graphene/PbZr0.2Ti0.8O3 Hybrid Structures through Ferroelectric Switching

Christoph Baeumer、Steven P. Rogers、Ruijuan Xu 等 5 位作者2013-03-18Nano Letters

Bidirectional interdependency between graphene doping level and ferroelectric polarization is demonstrated in graphene/PbZr0.2Ti0.8O3 hybrid structures. The polarization of the PbZr0.2Ti0.8O3 can be effectively switched with graphene electrodes and can in turn alter carrier type and density in the graphene. A complete…

Graphene research and applicationsFerroelectric and Piezoelectric MaterialsMultiferroics and related materials

Interplay of Octahedral Tilts and Polar Order in BiFeO3 Films

Young‐Min Kim、Amit Kumar、Alison Hatt 等 12 位作者2013-03-18Advanced Materials

Heterointerface stabilization of a distinct nonpolar BiFeO3 phase occurs simultaneously with changes in octahedral tilts. The resulting phase arises via suppression of polarization by a structural order parameter and can thus be identified as anti-ferroelectric (Fe displacements - bottom panel). The phase is metastabl…

Ferroelectric and Piezoelectric MaterialsMultiferroics and related materialsDielectric properties of ceramics

Theoretical Studies of the Adsorption of CO and C on Ni(111) and Ni/CeO2(111): Evidence of a Strong Metal–Support Interaction

Javier Carrasco、Laura Barrio、Ping Liu 等 5 位作者2013-03-18The Journal of Physical Chemistry C

The catalytic CO methanation reaction on Ni/CeO 2 (111) systems is known to depend on Ni coverage: at medium and large coverages, Ni/CeO 2 (111) surfaces are able to catalyze methane production, whereas at small coverage they become efficient catalysts for the water–gas shift reaction. Electronic structure, geometries…

Catalytic Processes in Materials ScienceCatalysts for Methane ReformingCatalysis and Oxidation Reactions

Charge carrier relaxation model in hopping system

Nianduan Lu、Ling Li、Pengxiao Suna 等 4 位作者2013-03-18arXiv

The relaxation phenomena of charge carriers in hopping system have been demonstrated and investigated theoretically. An analytical model describing the charge carrier relaxation is proposed based on the hopping transport theory. The relation between the material disorder, electric field and temperature and the relaxat…

Materials Science

Temperature control of local magnetic anisotropy in multiferroic CoFe/BaTiO3

Tuomas H. E. Lahtinen、Sebastiaan van Dijken2013-03-18Applied Physics Letters

This paper reports on the temperature evolution of local elastic interactions between ferromagnetic CoFe films and ferroelectric BaTiO3 substrates. Polarization microscopy measurements indicate that growth-induced stripe domains in the CoFe films are preserved and strengthened during cooling and heating through the st…

Ferroelectric and Piezoelectric MaterialsMultiferroics and related materialsMagnetic Properties and Synthesis of Ferrites

Coupling and induced depinning of magnetic domain walls in adjacent spin valve nanotracks

J. Sampaio、L. O'Brien、D. Petit 等 9 位作者2013-03-18arXiv

The magnetostatic interaction between magnetic domain walls (DWs) in adjacent nanotracks has been shown to produce strong inter-DW coupling and mutual pinning. In this paper, we have used electrical measurements of adjacent spin-valve nanotracks to follow the positions of interacting DWs. We show that the magnetostati…

Materials Science

New Dirac points and multiple Landau level crossings in biased trilayer graphene

Maksym Serbyn、Dmitry A. Abanin2013-03-18Physical Review B

Recently a new high-mobility Dirac material, trilayer graphene, was realized experimentally. The band structure of $ABA$-stacked trilayer graphene consists of a monolayer-like and a bilayer-like pair of bands. Here we study electronic properties of $ABA$-stacked trilayer graphene biased by a perpendicular electric fie…

Graphene research and applicationsQuantum and electron transport phenomenaTopological Materials and Phenomena

Determination of the magnetization profile of Co/Mg periodic multilayers by magneto-optic Kerr effect and X-ray magnetic resonant reflectivity

Philippe Jonnard、K. Le Guen、Jean-Michel André 等 11 位作者2013-03-18arXiv

The resonant magnetic reflectivity of Co/Mg multilayers around the Co L2,3 absorption edge is simulated then measured on a specifically designed sample. The dichroic signal is obtained when making the difference between the two reflectivities measured with the magnetic field applied in two opposite directions parallel…

Materials Science

Nonlinear Surface Resistance of YBa2Cu3O7-x Superconducting Thin Films on MgO Substrates in Dielectric Resonator at Ultra High Frequencies

Dimitri O. Ledenyov2013-03-18arXiv

The nonlinear surface resistance Rs of the YBa2Cu3O7-x superconducting thin films on the MgO substrates was researched in the Hakki-Coleman dielectric resonator at the microwave signal powers from -18 dBm to +30 dBm at the ultra high frequency of 25 GHz in the range of temperatures from 12 K to 85 K. The dependences o…

Mesoscale and Nanoscale PhysicsMaterials ScienceSuperconductivitynlin.CDphysics.ins-det

Symmetrical laws of structure of helicoidally-like biopolymers in the framework of algebraic topology. III. Nature of the double and relations between the alpha helix and the various forms of DNA structures

M. I. Samoylovich、A. L. Talis2013-03-18arXiv

In the frameworks of algebraic topology α-helix and different DNA-conformations are determined as the local latticed packing, confined by peculiar minimal surfaces which are similar to helicoids. These structures are defined by Weierstrass representation and satisfy to a zero condition for the instability index of the…

Materials Science

Quantum states of muons in fluorides

J. S. Möller、D. Ceresoli、T. Lancaster 等 5 位作者2013-03-18arXiv

Muon-spin relaxation (μSR) is a sensitive probe of magnetism, but its utility can be severely limited by the lack of knowledge of the muon implantation site and the extent to which the muon perturbs its host. We demonstrate systematically that these problems can be addressed accurately using electronic-structure calcu…

Materials ScienceStrongly Correlated Electrons

Origin of the superior conductivity of perovskite Ba(Sr)SnO3

Heng-Rui Liu、Ji-Hui Yang、H. J. Xiang 等 5 位作者2013-03-18Applied Physics Letters

ASnO3 (A = Ba, Sr) are unique perovskite oxides in that they have superior electron conductivity despite their wide optical band gaps. Using first-principles band structure calculations, we show that the small electron effective masses, thus, good electron conductivity of ASnO3 can be attributed to the large size of S…

Machine Learning in Materials ScienceElectronic and Structural Properties of OxidesChemical and Physical Properties of Materials