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Synthesis and characterization of new aromatic polyamides bearing crown ethers and acyclic ethylene oxide units in the pendant structure. III. Benzo‐18‐crown‐6 systems and their open‐chain counterparts

V. Calderón、Gert Schwarz、Félix C. García 等 7 位作者2006-09-20Journal of Polymer Science Part A Polymer Chemistry

Abstract We report the synthesis and characterization of 10 novel polyamides containing the benzo‐18‐crown‐6 subunit and its dipodal counterpart, along with their properties, and a comparison with homologous polyamides bearing benzo‐12‐crown‐4, benzo‐15‐crown‐5, and the corresponding dipodal systems. The anomalous pol…

Supramolecular Chemistry and ComplexesSynthetic Organic Chemistry MethodsSynthesis and properties of polymers

Modeling of Crystallization in a Blend Containing at Least One Crystallizable Component: An Analogy from Eutectic Systems

Sudhakar Balijepalli、Jerold M. Schultz2006-09-20Macromolecules

It is shown that crystalline/crystalline and crystalline/noncrystalline blends can crystallize from the melt such that both components reside in the same spherulite. The observed morphology of such systems is that of growth arms of one component separated by regions rich in the other component. For crystalline/crystal…

Polymer crystallization and propertiesMaterial Dynamics and PropertiesRheology and Fluid Dynamics Studies

Rotational Invariance and Double Frustration in the Structures of Gold Clusters Growing around the Fs-Defected MgO (100) Surface

Giovanni Barcaro、Alessandro Fortunelli2006-09-20The Journal of Physical Chemistry B

The interaction of small gold clusters (Au(n), n = 1-4, 20) and a gold monolayer with the MgO (100) surface surrounding a neutral oxygen vacancy (F(s) center) is investigated using density-functional (DF) calculations. It is found that the presence of the defect modifies the interaction of gold not only with the vacan…

Advanced Chemical Physics StudiesCatalytic Processes in Materials Sciencenanoparticles nucleation surface interactions

Precursors to stress-induced martensitic transformations and associated superelasticity: Molecular dynamics simulations and an analytical theory

Xiangdong Ding、Tetsuro Suzuki、Xiaobing Ren 等 5 位作者2006-09-20Physical Review B

Precursor phenomena are critical issues for martensitic transformation, as they provide important clues for understanding the origin of the transformation and the structure of the transformation products. Prior to temperature-induced martensitic transformation, it has been recognized for a long time that the basal pla…

High-pressure geophysics and materialsMetallic Glasses and Amorphous AlloysShape Memory Alloy Transformations

Michael addition polymerizations of difunctional amines (AA′) and triacrylamides (B3)

Ding Wang、Zhiju Zheng、Chun‐Yan Hong 等 5 位作者2006-09-20Journal of Polymer Science Part A Polymer Chemistry

Abstract Novel hyperbranched poly(amido amine)s containing tertiary amines on the backbones and acryl or secondary amines as the surface groups were successfully synthesized via the Michael addition polymerizations of a triacrylamide [1,3,5‐triacryloylhexahydro‐1,3,5‐triazine (TT)] and a difunctional amine [ n ‐butyla…

RNA Interference and Gene DeliveryChemical Synthesis and AnalysisDendrimers and Hyperbranched Polymers

Fabrication and Characterization of an Organic‐Inorganic Gradient Surface made by Polymethylsilsesquioxane (PMSQ)

Haiyun Liu、Jian Xu、Yanfang Li 等 6 位作者2006-09-20Macromolecular Rapid Communications

Abstract Summary: A simple method for the fabrication of a chemical composition gradient from organic to inorganic by the pyrolysis of a polymethylsilsesquioxane (PMSQ) thin film in a gradient temperature field is reported. The resultant chemical gradient surface demonstrates gradual changes in wettability, and slight…

Surface Modification and SuperhydrophobicityPolymer Surface Interaction StudiesSilicone and Siloxane Chemistry

Synthesis and Structural Characterization of a Series of Carboxylic Acid Modified Cerium(III) Alkoxides

Timothy J. Boyle、L.J. Tribby、S.D. Bunge2006-09-20European Journal of Inorganic Chemistry

Abstract A series of cerium alkoxides were synthesized from the reaction of Ce{N[Si(CH 3 ) 3 ] 2 } 3 and the appropriate alcohol: neopentyl alcohol [H–OCH 2 C(CH 3 ) 3 = H‐ONep], tert ‐butyl alcohol [H–OC(CH 3 ) 3 = H‐O t Bu], o ‐( tert ‐butyl)phenol {H–OC 6 H 4 [C(CH 3 ) 3 ]‐2 = H‐ o BP}, 2,6‐dimethylphenol [H–OC 6 H…

Catalytic Processes in Materials ScienceLanthanide and Transition Metal ComplexesPolyoxometalates: Synthesis and Applications

Adsorbate coverages and surface reactivity in methanol oxidation over Cu(110): An in situ photoelectron spectroscopy study

Sebastian Günther、Ling Zhou、Michael Hävecker 等 7 位作者2006-09-20The Journal of Chemical Physics

The adsorbate species present during partial oxidation of methanol on a Cu(110) surface have been investigated in the 10(-5) mbar range with in situ x-ray photoelectron spectroscopy and rate measurements. Two reaction intermediates were identified, methoxy with a C 1s binding energy (BE) of 285.4 eV and formate with a…

Advanced Chemical Physics StudiesCatalytic Processes in Materials ScienceCatalysis and Oxidation Reactions

Evolution of Polyoxoniobate Cluster Anions

R.P. Bontchev、May Nyman2006-09-20Angewandte Chemie

Eine neue Geometrie für Polyoxoniobate findet sich in {Nb24O72H9}15−, dem größten bislang bekannten Isopolyoxoniobat-Clusteranion. Die Entwicklung seiner Struktur von isolierten Lindqvist-Anionen [Nb6O19]8− und der cyclischen Pyrochloreinheit [Nb6O30] hin zum komplexen Dimer [({Nb24O72H9}{Cu(en)2(H2O)}2{Cu(en)2})2]18−…

Metal-Organic Frameworks: Synthesis and ApplicationsPolyoxometalates: Synthesis and ApplicationsChemical Synthesis and Reactions

Case for bulk nature of spectroscopic Luttinger liquid signatures observed in angle-resolved photoemission spectra ofLi0.9Mo6O17

Feng Wang、Sung‐Kwan Mo、J. W. Allen 等 10 位作者2006-09-20Physical Review B

Angle-resolved photoemission spectroscopy (ARPES) has been performed on quasi-one-dimensional ${\mathrm{Li}}_{0.9}{\mathrm{Mo}}_{6}{\mathrm{O}}_{17}$ using photon energy $h\ensuremath{\nu}=500\phantom{\rule{0.3em}{0ex}}\mathrm{eV}$. Measured band dispersions are in agreement with those from both low-photon-energy meas…

Physics of Superconductivity and MagnetismAdvanced Condensed Matter PhysicsElectronic and Structural Properties of Oxides

A novel gas-ionization sensor based on aligned multi-walled carbon nanotubes

Guohua Hui、Lili Wu、Min Pan 等 6 位作者2006-09-20Measurement Science and Technology

In this paper, we propose a novel gas-ionization sensor based on aligned multi-walled carbon nanotubes (MWNT) at normal temperature and pressure. It consists of an Al plate electrode, a plastic thin film and a MWNT electrode. Breakdown voltages and discharge currents are recorded through a peripheral detecting circuit…

Carbon Nanotubes in CompositesGas Sensing Nanomaterials and SensorsMechanical and Optical Resonators

The Effect of pH-adjusted Gold Colloids on the Formation of Gold Clusters over APTMS-coated Silica Cores

Sang-Eun Park2006-09-20Bulletin of the Korean Chemical Society

An electrostatic interaction is responsible for the attachment of gold seeds of 1-3 nm onto APTMS (3-aminopropyl trimethoxysilane)-coated silica cores in the formation of gold clusters. A surface plasmon resonance and morphology of gold clusters were significantly affected by the pH of gold colloids prepared by THPC r…

Gold and Silver Nanoparticles Synthesis and ApplicationsPolymer Surface Interaction StudiesNanocluster Synthesis and Applications

Donor−Acceptor−Donor-Type Liquid Crystal with a Pyridazine Core

Yeon Sil Park、Dohyung Kim、Hoosung Lee 等 4 位作者2006-09-20Organic Letters

[structure: see text] A new liquid crystalline material having an ethylenedioxythiophene-pyridazine-ethylenedioxythiophene (EDOT-PDZ-EDOT) core with two peripheral long alkyl chains was prepared. The designated donor-acceptor-donor (D-A-D)-type core structure induced a distinct smectic liquid crystalline phase due to…

Liquid Crystal Research AdvancementsSynthesis and Properties of Aromatic CompoundsPhotochromic and Fluorescence Chemistry

Direct Growth of Highly Organized Crystalline Carbon Nitride from Liquid-Phase Pulsed Laser Ablation

Li Yang、Paul May、Lei Yin 等 5 位作者2006-09-20Chemistry of Materials

The novel technique of liquid-phase pulsed laser ablation has been used to obtain unique, highly ordered nanostructures of crystalline carbon nitride (C 3 N 4 ) via ablation of a graphite target submerged in aqueous ammonia solution. Transmission electron microscopy (TEM) analysis shows that the morphology of the carb…

Diamond and Carbon-based Materials ResearchLaser-induced spectroscopy and plasmaLaser-Ablation Synthesis of Nanoparticles

Judd−Ofelt Intensity Parameters and Spectral Properties of Gd2O3:Eu3+Nanocrystals

Chunxu Liu、Junye Liu、Kai Dou2006-09-20The Journal of Physical Chemistry B

Three nonequivalent centers of Cs (A, B, and C) in monoclinic phase and C2 and S6 centers in cubic phase were identified in the Gd2O3:Eu3+ nanocrystals with spectral techniques. Size dependence in the spectra indicated that the excitations from both host and charge-transfer band (CTB) for the 5D0 --> 7F2 transition of…

Luminescence Properties of Advanced MaterialsQuantum Dots Synthesis And PropertiesLanthanide and Transition Metal Complexes

Sparse data structure and algorithm for the phase field method

Jason Gruber、Ning Ma、Y Wang 等 5 位作者2006-09-20Modelling and Simulation in Materials Science and Engineering

The concepts of sparse data structures and related algorithms for phase field simulations are discussed. Simulations of polycrystalline grain growth with a conventional phase field method and with sparse data structures are compared. It is shown that memory usage and simulation time scale with the number of nodes but…

Aluminum Alloy Microstructure PropertiesSolidification and crystal growth phenomenaMagnetic Properties and Applications

Impurity dimers in superconducting B-doped diamond: Experiment and first-principles calculations

Emmanuel Bourgeois、E. Bustarret、P. Achatz 等 5 位作者2006-09-20Physical Review B

On the basis of first-principles calculations and experimental secondary ion mass spectroscopy, electrical transport, and Raman measurements performed on homoepitaxial diamond, we find that at high concentrations boron atoms tend to segregate in dimers. The study of the electronic, vibrational, and electron-phonon cou…

High-pressure geophysics and materialsDiamond and Carbon-based Materials ResearchIon-surface interactions and analysis

Morphology-Tunable and Photoresponsive Properties in a Self-Assembled Two-Component Gel System

Yifeng Zhou、Miao Xu、Tao Yi 等 7 位作者2006-09-20Langmuir

Photoresponsive C3-symmetrical trisurea self-assembling building blocks containing three azobenzene groups (LC10 and LC4) at the rim were designed and synthesized. By introducing a trisamide gelator (G18), which can self-aggregate through hydrogen bonds of acylamino moieties to form a fibrous network, the mixture of L…

Supramolecular Self-Assembly in MaterialsPhotochromic and Fluorescence ChemistryPolydiacetylene-based materials and applications

Overcoming the poor short wavelength spectral response of CdS/CdTe photovoltaic modules via luminescence down‐shifting: ray‐tracing simulations

Bryce S. Richards、Keith R. McIntosh2006-09-20Progress in Photovoltaics Research and Applications

Abstract The short‐wavelength response of cadmium sulfide/cadmium telluride (CdS/CdTe) photovoltaic (PV) modules can be improved by the application of a luminescent down‐shifting (LDS) layer to the PV module. The LDS layer contains a mixture of fluorescent organic dyes that are able to absorb short‐wavelength light of…

TiO2 Photocatalysis and Solar CellsQuantum Dots Synthesis And PropertiesChalcogenide Semiconductor Thin Films