Materials Literature
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PURPOSE: To design low peak and integrated power simultaneous multislice excitation radiofrequency pulses with transmit field inhomogeneity compensation in high field MRI. THEORY AND METHODS: The "interleaved greedy and local optimization" algorithm for small-tip-angle spokes pulses is extended to design multiband (MB…
A new colorimetric probe has been developed for the detection and estimation of Pd(II) at sub-nanomolar concentrations. The probe consisted of rhodamine (signaling unit), which was linked with a bis-picolyl moiety (binding site) through a phenyl ring. Pd(II) induced opening of the spirolactam ring of the probe with th…
Abstract An important challenge in asymmetric cascade reactions is solving the intrinsic incompatibility of two types of distinct organometallic complexes that participate in a one‐pot reaction. Herein, we develop an organoruthenium‐/organopalladium‐bifunctionalized periodic mesoporous organosilica and realize one‐pot…
By screening the possible range of isoreticular isomers, the structure of copper paddle-wheel-based metal–organic frameworks with nbo-b topology can be predicted and the formation of different phases can be rationalized.
The gravity-driven flow of a thin liquid film down a uniformly heated vertical fiber is considered. This is an unstable open flow that exhibits rich dynamics including the formation of droplets, or beads, driven by a Rayleigh-Plateau mechanism modified by the presence of gravity as well as the variation of surface ten…
This work describes an efficient synthetic method for creating ladder-type, oligomeric donor monomers with fused thienobenzothiophene structures. These monomers are copolymerized with fluorinated thieno[3,4- b ]thiophene ester to form a series of polymers which are investigated as donor materials in polymer/fullerene…
We report the synthesis, characterization, redox behavior, and n-channel organic field-effect (OFET) characteristics of a new class of thieno[3,2-b]thiophene-diketopyrrolopyrrole-based quinoidal small molecules 3 and 4. Under ambient atmosphere, solution-processed thin-film transistors based on 3 and 4 exhibit maximum…
The enzyme flavocytochrome c3 (fcc3), which catalyzes hydrogenation across a C═C double bond (fumarate to succinate), is used to carry out the fuel-forming reaction in an artificial photosynthesis system. When immobilized on dye-sensitized TiO2 nanoparticles, fcc3 catalyzes visible-light-driven succinate production in…
The area of smart textiles has recently attracted more and more attention. One of the challenges in this domain is the development of textile sensors, such as textile electrodes, pressure sensors, elongation sensors, etc., mostly containing conductive yarn and/or conductive coating. One possibility to build a textile…
Death Receptor 5 (DR5) is a pro-apoptotic cell-surface receptor that is a potential therapeutic target in cancer. Despite the potency of DR5-targeting agents in preclinical models, the translation of these effects into the clinic remains disappointing. Herein, we report an alternative approach to exploiting DR5 tumor…
Ni(OH)2 nanoparticles are demonstrated to be cost-efficient alternatives to Pt co-catalysts for enhancing the visible-light photocatalytic H2 evolution activity of red phosphorous (P) when deposited onto its surface. Ni(OH)2-modified red P exhibits 1.12 times higher photocatalytic activity for H2 evolution than that o…
The produced mechanical work at tensile drawing is converted into heat almost completely and the polymer temperature rises. The temperature rise at adiabatic drawing for different polymers is 20-100°C. To determine the temperature of PET during neck propagation, micro-particles with pre-determined melt surface were du…
In this paper, the structural, elastic, and electronic properties of RIn3 and RSn3 (R = Sm, Eu, Gd) compounds have been investigated using the full potential linearized augmented plane wave plus local orbital method within the density functional theory. The structural properties are investigated using the LDA, GGA, an…
Abstract Solar‐light‐driven H2 production in water with a [NiFeSe]‐hydrogenase (H2ase) and a bioinspired synthetic nickel catalyst (NiP) in combination with a heptazine carbon nitride polymer, melon (CNx), is reported. The semibiological and purely synthetic systems show catalytic activity during solar light irradiati…
Angular resolved photoemission spectroscopy in combination with ab initio calculations show that trace amounts of carbon doping of the Bi_{2}Se_{3} surface allows the controlled shift of the Dirac point within the bulk band gap. In contrast to expectation, no Rashba-split two-dimensional electron gas states appear. Th…
The occurrence of active water transport (net transport against a free energy gradient) in photosynthetic organisms has been debated for several decades. Here, active water transport is considered in terms of its roles, where it is found, and the mechanisms by which it could occur. First there is a brief consideration…
This paper presents a semirigid (SR) bonnet tool which has the advantages of high efficiency and determinacy for material removal on optical elements and also has the potential to be used on aspheric optics. It consists of three layers: a metal sheet, a rubber membrane, and a polishing pad, from inside to outside. It…
Wavelet‐based de‐noising is used to separate partial discharge (PD) signals from the noises resulting from measurement circuits or the surrounding environment. PD de‐noising by using the wavelet shrinkage method is capable of separating the noise component to some extent, but the selection of the wavelet base has a re…
This paper proposes a novel high-performance control scheme with hysteresis compensator and disturbance observer for high-precision motion control of a nanopositioning stage driven by a piezoelectric stack actuator (PSA). In the developed control scheme, a real-time inverse hysteresis compensator (IHC) with the modifi…
Chaperone-mediated autophagy (CMA) is involved in wild-type α-synuclein degradation in Parkinson's disease (PD), and LAMP2A and Hsc 70 have recently been indicated to be deregulated by microRNAs. To recognize the regularory role of miR-320a in CMA and the possible role in α-synuclein degradation, in the present study,…