Materials Literature
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The static and dynamic properties of 2- and 3-dimensional dispersions of strongly interacting colloidal spheres are examined. Quasi-2-dimensional dispersions of particles interacting by long range electrostatic and dipolar magnetic forces, respectively, are investigated using Brownian dynamics computer simulations wit…
Abstract The aim of this work is to evaluate routes to upgrade recycled engineering plastics, especially mixed plastics with acrylonitrile–butadiene–styrene copolymers (ABS) as the major component. A core‐shell impact modifier was successfully used to improve the impact strength of blends of ABS and ABS/polycarbonate…
We achieved separate detection of the components of 10 ppm of a benzene, toluene, and o-xylene mixture gas by using mesoporous silica powder incorporated in our microfluidic device. The device consists of concentration and detection cells formed of 3 cm x 1 cm Pyrex plates. We first introduced the mixture gas into the…
Abstract The graft copolymerization of acrylamide–methylacrylate comonomers was carried out using ceric ammonium nitrate as initiator in the presence of nitric acid at 25 ± 1°C. The effects of feed molarity, feed composition, reaction time, and temperature on graft yield (% G ) and other grafting parameters were inves…
The Raman spectra of tetragonal CaMoO 4 (scheelite structure, C 4h 6 space group) have been measured in the temperature range 12–1300 K. At high temperatures, the frequency and linewidth of all Raman-active phonons vary almost linearly with temperature, indicating that the three-phonon decay processes are dominant ove…
Studies on a large number of compositions among the ferromagnetic self-doped manganites, La 1−x MnO 3 , show that the ferromagnetic Curie temperature increases with x and reaches a maximum value for x = 1/7. T c remains independent of x for x ≥ 1/7 and the maximum value of the magnetization is obtained for x = 1/8. Th…
We shall discuss the following phenomena found in various colloidal systems in shear flow. We recently observed shear-banding in suspensions of fd-virus in a cylindrical shear cell. Small angle light scattering experiments revealed that the shear-banding transition is preceded by a relatively fast process (minutes) of…
We show that crystals of molecular nanomagnets can exhibit giant magnetic relaxation due to the Dicke superradiance of electromagnetic waves. Rigorous theory is presented that combines superradiance with the Landau-Zener effect.
Two-dimensional electromagnetic crystals formed by rectangular lattices of thin ideally conducting cylinders periodically loaded by bulk reactive impedances are considered. An analytical theory of dispersion and reflection from this medium is presented. The consideration is based on the local field approach. The trans…
The Hamiltonian of the wurtzite quantum rods with an ellipsoidal boundary is given after a coordinate transformation. The energies, wave functions, and transition possibilities are obtained as functions of the aspect ratio e with the same method we used on spherical dots. With an overall consideration of both the tran…
Abstract A radiofrequency air plasma has been used to incorporate new functionalities at the surface of cycloolefin polymers (Zeonex® and Topas®), polymethyl methacrylate (PMMA), styrene–acrylonitrile copolymer (SAN), and polystyrene (PS). The main goals with the plasma treatment of the different plastics were to hydr…
The diesel particulate filters (DPFs) technology has impressively advanced especially during the last years, driven by the interest in the reduction of automobile particulate emissions. This paper is concerned with the effect of NO 2 as an active oxidation agent in the regeneration process of the soot accumulated in t…
A quarter of a century ago, Chemical Communications published a seminal paper called “Synthesis of Electrically Conducting Organic Polymers: Halogen Derivatives of Polyacetylene, (CH)x”. A new field of chemistry was born.
We demonstrate bulk synthesis of highly crystalline beta-gallium oxide tubes, nanowires, and nanopaintbrushes using molten gallium and microwave plasma containing a mixture of monatomic oxygen and hydrogen. Gallium oxide nanowires were 20-100 nm thick and tens to hundreds of micrometers long. Transmission electron mic…
A purification algorithm for expanding the single-particle density matrix in terms of the Hamiltonian operator is proposed. The scheme works with a predefined occupation and requires less than half the number of matrix-matrix multiplications compared to existing methods at low (<10%) and high (>90%) occupancy. The exp…
We study the properties of a polycarbonate melt near a nickel surface as a model system for the interaction of polymers with metal surfaces by employing a multiscale modeling approach. For bulk properties, a suitably coarse-grained bead-spring model is simulated by molecular dynamics methods with model parameters dire…
Time-resolved synchrotron small-angle X-ray scattering (SAXS) studies were performed to investigate the unseeded formation and growth of colloidal calcium carbonate particles. Equimolar aqueous solutions of CaCl 2 ·2H 2 O and Na 2 CO 3 were rapidly mixed in a stopped-flow apparatus, and SAXS data were recorded using a…
We have studied the coefficient of restitution, $η$, in normal collisions of a non-rotating sphere on a massive plate for a range of material parameters, impact velocity and sphere size. The measured coefficient of restitution does not monotonically vary with velocity. This effect is due to dynamics that occur during…
This paper presents a nonlinear, robust control algorithm for accurate positioning of a single degree of freedom rotary manipulator actuated by Shape Memory Alloy (SMA). A model for an SMA actuated manipulator is presented. The model includes nonlinear dynamics of the manipulator, a constitutive model of Shape Memory…
The miscibility and phase behavior of two stereoisomer forms of poly(lactide) (PLA: poly (L-lactide) (PLLA) and poly(DL-lactide) (PDLLA)) blends with poly(epsilon-caprolactone)-b-poly(ethylene glycol) (PCL-b-PEG) and PCL-b-monomethoxy-PEG (PCL-b-MPEG) block copolymers have been investigated by differential scanning ca…