Materials Literature
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X-ray free-electron lasers (FELs) enable crystallographic data collection using extremely bright femtosecond pulses from microscopic crystals beyond the limitations of conventional radiation damage. This diffraction-before-destruction approach requires a new crystal for each FEL shot and, since the crystals cannot be…
We demonstrate the controlled growth of coaxial nanocables composed of GaP/ZnS core-shell structures by a facile chemical vapor deposition method. Structural analysis confirms that the cubic GaP (111) plane and wurtzite ZnS (0001) plane present close similarities in terms of hexagonal-arranged atomic configuration wit…
We investigate thermoelectric efficiency of systems with broken time-reversal symmetry under a three-terminal transport. Using a model of Aharonov-Bohm interferometer formed with three noninteracting quantum dots, we show that Carnot efficiency ${\ensuremath{\eta}}_{C}$ can be achieved when the thermopower is a symmet…
Nanoporous anodic alumina membranes (NPAMs) were produced by the two-step anodization method in sulphuric, oxalic and phosphoric acidic electrolytes displaying a hexagonally ordered spatial arrangement of pores with well controlled nanopore size distribution and low porosity. Some selected NPAMs were further modified…
Miniaturization of conventional energy sources has so far proven to be a cumbersome process. A recently developed concept of thermopower waves has shown tremendous potential to reduce the dimensions of power sources while maintaining their energy generation capabilities. We demonstrate a tremendous improvement in the…
We present a study of a transition metal oxide composite modified n-Si photoanode for efficient and stable water oxidation. This sputter-coated composite functions as a protective coating to prevent Si from photodecomposition, a Schottky heterojunction, a hole conducting layer for efficient charge separation and trans…
Guided by the analogy to Mie scattering of light on small particles, we show that the propagation of a Dirac-electron wave in graphene can be manipulated by a circular gated region acting as a quantum dot. Large dots enable electron lensing, while for smaller dots resonant scattering entails electron confinement in qu…
Photolysis of regioisomeric helical chromenes 1 and 2 leads to colored reactive intermediates. While the latter generally decay quite rapidly, they are found to be longer lived in 1 and highly persistent in 2. The remarkable stability of the otherwise fleeting transient in 2 allowed isolation and structural characteri…
Structural and dielectric properties of (1− x ) BaTiO 3 – x Bi ( Mg 1/2 Ti 1/2 ) O 3 ( x = 0.1–0.5) were investigated to understand the binary system and utilize it for high‐voltage, high energy density capacitors. The solubility limit for Bi ( Mg 1/2 Ti 1/2 ) O 3 in a BaTiO 3 perovskite was between x = 0.4 and x = 0.…
Through a series of carefully executed experiments, we discovered the prevalence of anisotropic shell growth in many upconversion NaREF4 systems caused by a combination of factors: selective adsorption of ligands on the core surface due to the core crystal structure, ligand etching, and the lattice mismatch between co…
The optical properties and electrical conductivity of highly conducting poly(3,4-ethylenedioxythiophene) (PEDOT) doped with poly(styrenesulfonate) (PSS) are reported as a function of the processing additive conditions. The addition of dimethyl sulfoxide (DMSO) increases the conductivity and modifies the dielectric res…
We study the temperature dependent dynamical processes of a Si10H16 cluster and obtain a blue shift of the Si-Si vibrational modes with transverse acoustic character and a red shift of the other vibrational modes with increasing temperature. We link this behavior to the bond length expansion and the varying sign of th…
One of the most noticeable collective motion of non-cohesive granular matter is clustering under certain conditions. In particular, when a quasi-two-dimensional monolayer of mono-disperse non-cohesive particles is vertically vibrated, a solid-liquid-like transition occurs when the driving amplitude exceeds a critical…
We demonstrate the rational solution-phase synthesis of compositional modulated telluride nanowire heterostructures containing lead telluride (PbTe) and bismuth telluride (Bi2Te3). By tuning the ratio between PbTe and Bi2Te3 through adjusting the amount of critical reactants and precursors during the synthesis, the in…
This study compares toxic effects of uncoated (20, 40, 60 and 80 nm) and OECD (Organization for Economic Co-operation and Development) standard citrate- and polyvinylpyrrolidone (PVP)-coated (10, 50, and 75 nm) silver nanoparticles (Ag-NPs) in J774A. 1 macrophage and HT29 epithelial cells. The cells were exposed to di…
We investigate the optoelectronic properties of novel graphene/FeCl3-intercalated few-layer graphene (FeCl3-FLG, dubbed graphexeter) heterostructures using photovoltage spectroscopy. We observe a prominent photovoltage signal generated at the graphene/FeCl3-FLG and graphene/Au interfaces, whereas the photovoltage at t…
Fatigue and aging of materials are, in large part, determined by the evolution of the atomic-scale structure in response to strains and perturbations. This coupling between microscopic structure and long time scales remains one of the main challenges in materials study. Focusing on a model system, ion-damaged crystall…
A comparative first-principles study of possible bismuth-related centers in TlCl and CsI crystals is performed and the results of computer modeling are compared with the experimental data. The calculated spectral properties of the bismuth centers suggest that the IR luminescence observed in TlCl:Bi is most likely caus…
Using Landau--Ginzburg--Devonshire theory and phase-field modeling, we explore the complex interplay between a structural order parameter (oxygen octahedron rotation) and polarization in Eu${}_{x}$Sr${}_{1\ensuremath{-}x}$TiO${}_{3}$ thin films. Under a biaxially tensile strain, a low-symmetry monoclinic phase with in…
We use spin density functional theory ab initio calculations to theoretically explore the possibility of achieving useful gate control over exchange coupling between cobalt clusters placed on a graphene sheet. By applying an electric field across supercells, we demonstrate that the exchange interaction is strongly dep…