Materials Literature
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The first-order interaction correction to the irreducible polarization function of pristine graphene is studied at arbitrary relation between momentum and frequency. The results are used to calculate the dielectric function and the dynamical conductivity of graphene beyond the standard random-phase approximation. The…
We have developed fast responsive, colorimetric and resistive-type polymeric humidity sensors from a series of self-assembled poly(styrenesulfonate-methylbutylene) (PSS-b-PMB) block copolymers with tailored hygroscopic properties. In dry state, the PSS-b-PMB films exhibit hexagonal cylindrical morphology where hydroph…
Artificial tuning of dielectric parameters can result from interface conductivity in polycrystalline materials. In ferroelectric single crystals, it has already been shown that ferroelectric domain walls can be the source of such artificial coupling. We show here that low-temperature dielectric losses can be tuned by…
Transparent flexible graphene transistors and inverters in a coplanar-gate configuration were presented for the first time using only two materials: graphene and an ion gel gate dielectric. The novel device configuration simplifies device fabrication such that only two printing steps were required to fabricate transis…
In this report, we demonstrate a rapid and simple seeded growth method for synthesizing monodisperse, quasi-spherical, citrate-stabilized Au nanoparticles (Au NPs) via H(2)O(2) reduction of HAuCl(4). Au NPs with diameter ranging from 30 to 230 nm can be synthesized by simply adding 12 nm citrate stabilized Au NP seeds…
Carbon materials are excellent candidates for photovoltaic solar cells: they are Earth-abundant, possess high optical absorption, and maintain superior thermal and photostability. Here we report on solar cells with active layers made solely of carbon nanomaterials that present the same advantages of conjugated polymer…
Controlling ultrafast magnetization dynamics by a femtosecond laser is attracting interest both in fundamental science and industry because of the potential to achieve magnetic domain switching at ever advanced speed. Here we report experiments illustrating the ultrastrong and fully coherent light-matter coupling of a…
We report the observation of near-infrared photoluminescence from Te4(Ga2Cl7)2 and Te4(Al2Cl7)2 molecular crystals containing Te42+ polycations. The experimental and theoretical results clearly revealed that Te42+ polycation is one smart near-infrared emitter with characteristic emission peaks at 1252 and 1258 nm for…
Colloidal capsules can sustain an external osmotic pressure; however, for a sufficiently large pressure, they will ultimately buckle. This process can be strongly influenced by structural inhomogeneities in the capsule shells. We explore how the time delay before the onset of buckling decreases as the shells are made…
A current-carrying resonant nanoscale device, simulated by non-adiabatic molecular dynamics, exhibits sharp activation of non-conservative current-induced forces with bias. The result, above the critical bias, is generalized rotational atomic motion with a large gain in kinetic energy. The activation exploits sharp fe…
The active cloak comprises a discrete set of multipole sources that destructively interfere with an incident time harmonic scalar wave to produce zero total field over a finite spatial region. For a given number of sources and their positions in two dimensions it is shown that the multipole amplitudes can be expressed…
A grand challenge of nanoscience is to master the control of structure and properties in order to go beyond present day functionality. The creation of nanostructures via atom manipulation by means of a scanning probe represents one of the great achievements of the nano era. Here we build on this achievement to self-as…
Magnesium nickel hydride films have earlier been suggested for several optoelectronic applications, but the optical properties and band gap have not been firmly established. In this work, the dielectric functions and the optical band gaps of thin films of Mg2NiH4 have been determined experimentally from optical modeli…
A major challenge in the synthesis of plasmonic semiconductor nanocrystals is the ability to control localized surface plasmon resonance (LSPR) properties by varying the size, shape, and carrier density of the nanocrystal. For example, copper sulfide (Cu 2– x S) nanodisks possess two distinct LSPR modes that occur in…
Simulations are used to determine the effect of inertia on athermal shear of amorphous two-dimensional solids. In the quasistatic limit, shear occurs through a series of rapid avalanches. The distribution of avalanches is analyzed using finite-size scaling with thousands to millions of disks. Inertia takes the system…
Skipping the Odds When confined to a plane and placed in a magnetic field at low temperatures, electrons are separated by energy into the so-called Landau levels; adding an extra electron after a Landau level that has been filled is costly. In some systems, electron-electron interactions cause the appearance of sublev…
In this work, the physical and mechanical properties of bleached Eucalyptus pulp reinforced with nanofibrillated cellulose (NFC) are compared with those of traditional beaten pulp used in the making of writing/printing and offset printing papers. For this purpose, three different types of hardwood slurries were prepar…
Polylactide (PLA) is the oldest and potentially one of the most interesting and useful biodegradable man-made polymers because of its renewable origin, controlled synthesis, good mechanical properties, and inherent biocompatibility. The blending of PLA with functional nanoparticles can yield a new class of hybrid mate…
Here we report the synthesis and characterization of a BF(2)-azo complex that can be induced to isomerize without the need of deleterious UV light. The complexation of the azo group with BF(2), coupled with the extended conjugation of the N═N π-electrons, increases the energy of the n-π* transitions and introduces new…
A promising electrocatalyst prototype of low Pt mole fraction, intermetallic nanoparticles of Cu(3)Pt, has been prepared using a simple impregnation-reduction method, followed by a post heat-treatment. Two dealloying methods (electrochemical and chemical) were implemented to control the atomic-level morphology and imp…