Materials Literature
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Comprehensive low-temperature specific-heat data $C(T,H)$ of ${\mathrm{Na}}_{0.35}{\mathrm{CoO}}_{2}\ifmmode\cdot\else\textperiodcentered\fi{}1.3\phantom{\rule{0.3em}{0ex}}{\mathrm{H}}_{2}\mathrm{O}$ with temperature $T$ down to $0.6\phantom{\rule{0.3em}{0ex}}\mathrm{K}$ and the magnetic field $H$ up to $8\phantom{\ru…
This work presents the development of a wettability switching membrane device using the surface roughness effect. We designed and fabricated a roughness switchable membrane device, consisting of a thin poly(dimethylsiloxane) (PDMS) membrane bonded on the top of a rough PDMS substrate. A thin (less than 2 µm) PDMS memb…
A simple method has been developed to produce SERS-active metal surfaces. Six metal surfaces (cadmium, nickel, gold, iron, copper, and silver) have been prepared on an aluminum foil underlayment by chemical reduction and strong surface-enhanced Raman signals have been observed for pyridine species on these surfaces. T…
Recently we have reported on the growth of an exciting new class of hybrid nanostructured carbon materials, coupling nanosized diamond with single-walled carbon nanotubes. The inner structures were shown to be single-walled C nanotubes or bundles of single-walled nanotubes up to 15 μm long, and the outer deposit consi…
The selective reduction of NO with NH(3) catalyzed by isolated VO(x) species grafted onto TiO(2) (anatase) is studied by means of periodic density functional calculations. NH(3) is adsorbed molecularly by the bare support both as a Lewis-bonded complex at (101) 5-fold coordinated Ti sites, and as a H-bonded complex at…
Abstract Rheological, thermomechanical, and morphological properties of blends of two different epoxy resins with hydroxyl functionalized hyperbranched polymers have been studied. The hydroxyl functionalized hyperbranched polymers used in this work had different generation number and different number of terminal group…
Positron annihilation spectroscopy has been used to study the vacancy-type defects produced in films grown by metalorganic chemical vapor deposition on different sapphire orientations. Zn vacancies are the defects controlling the positron annihilation spectra at room temperature. Close to the interface (<500nm) the…
The synthesis of large-pore micelle-templated silica (MTS) materials as discrete spheres by pseudomorphic synthesis solves the double challenge: enlarging the pore size of MTS beyond the diameter of the micelles and controlling the morphology and the size of the particles. The pseudomorphic transformation of silica be…
Hollow polyhedra and cubes of nanostructured Cu(2)O particles have been synthesized by reduction of CuSO(4) with ascorbate acid in the solution phase. The nanostructures were obtained when the cetyltrimethylammonium (CTAB) concentration ranged from 0 to 0.03 M in the presence of NaOH. Structural characterizations, by…
We report on the correlation between the electrical behavior and valence band spectra of undoped and Al-doped ZnO films, obtained by using x-ray photoelectron spectroscopy. Although Al-doping can induce a conductivity increase of two orders of magnitude, we show that the gap persists and there is no semiconductor–meta…
Reliable diffusion coefficients, D, for the diffusion of perchlorate anions into polypyrrole films during polymeric oxidation were obtained from chronoamperometric results. Two different models were used to calculate D: the Cottrell equation and the electrochemically stimulated conformational relaxation (ESCR) model.…
CdS multipod-based structures, such as flowerlike microstructures, tetrapod-like microrods, and long branched nanowires, were selectively prepared by atmospheric pressure thermal evaporation of CdS nanoparticles without the use of a catalyst. The morphologies could be well controlled by simply adjusting the deposition…
Gold clusters adsorbed with CO, Au(m)(CO)(n) (-) (m=2-5; n=0-7), were studied by photoelectron spectroscopy (PES). The first few CO adsorptions were observed to induce significant redshifts to the PES spectra relative to pure gold clusters. For each Au cluster, a critical CO number (n(c)) was observed, beyond which th…
The apatite La 10 - x □ x (Ge 5.5 Al 0.5 O 24 )O 2.75 - 1.5 x (10 − x = 9.80, 9.75, 9.67, 9.60, 9.50, and 9.40) series has been prepared and the single phase existence range has been established, 9.75 ≥ 10 − x ≥ 9.45. The hexagonal crystal structures of La 9.5 □ 0.5 (Ge 5.5 Al 0.5 O 24 )O 2 have been determined at roo…
Thermosensitive micelles and vesicles in water were prepared using narrowly distributed polystyrene- b -poly( N -isopropylacrylamide) (PS- b -PNIPAM) diblock copolymers, and the conformational changes of PNIPAM blocks in the coronas of micelles and vesicles were investigated by a combination of static and dynamic lase…
Views Icon Views Article contents Figures & tables Video Audio Supplementary Data Peer Review Share Icon Share Twitter Facebook Reddit LinkedIn Tools Icon Tools Reprints and Permissions Cite Icon Cite Search Site Citation A. E. Pap, K. Kordás, G. Tóth, J. Levoska, A. Uusimäki, J. Vähäkangas, S. Leppävuori, T. F. Georg…
Out of the blue: Photoinduced magnetism in polymeric “Prussian Blue” analogues is a well understood phenomenon that can even occur near room temperature. The lessons learned are now being transferred to the synthesis of molecular cyanide-bridged single-molecule magnets (see picture; Mo yellow, C black, N blue, Cu purp…
Using time-resolved $1s$-$2p$ excitonic Lyman spectroscopy, we study the orthoexciton-to-paraexcitons transfer, following the creation of a high density population of ultracold $1s$ orthoexcitons by resonant two-photon excitation with femtosecond pulses. An observed fast exciton-density dependent conversion rate is at…
We analyze the scaling of avalanche precursors in the three dimensional random fuse model by numerical simulations. We find that both the integrated and non-integrated avalanche size distributions are in good agreement with the results of the global load sharing fiber bundle model, which represents the mean-field limi…
An understanding of osteoblast response to surface topography is essential for successful bone tissue engineering applications. Alumina has been extensively used as a substrate for bone tissue constructs. However, current techniques do not allow precise surface topography and orientation of the material. In this resea…