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Fourier transform Raman spectrum andab initio and density functional computations of the vibrational spectrum, molecular geometry, atomic charges and some molecular properties of the anticarcinogenic drug 5-fluorouracil

V. K. Rastogi、Vaibhav Jain、R.A. Yadav 等 5 位作者2000-01-01Journal of Raman Spectroscopy

FT Raman study of 5-fluorouracil, an anticarcinogenic drug, was carried out. Ab initio and density functional computations of the vibrational spectrum, the molecular geometry, the atomic charges, the total energy, the zero point energy, the rotational constants, the room temperature entropy, (translational, rotational…

Metal complexes synthesis and propertiesNonlinear Optical Materials ResearchInorganic and Organometallic Chemistry

CeNixOy and CeAlzNixOy solids studied by electron microscopy, XRD, XPS and depth sputtering techniques

Anne Ponchel、A. D’Huysser、Carole Lamonier 等 4 位作者2000-01-01Physical Chemistry Chemical Physics

Mixed oxides based on nickel, cerium and aluminum, effective in the catalytic hydrogenation of unsaturated compounds, were prepared by a coprecipitation route and studied by XRD, TEM, XPS and ion sputtering techniques. The CeNixOy mixed oxides (0⩽x⩽1) can be described as a mixture of nickel oxide and ceria modified by…

Catalytic Processes in Materials ScienceCatalysis and Hydrodesulfurization StudiesCatalysis and Oxidation Reactions

Self-sedimented diatom mats as agents of exceptional fossil preservation in the Oligocene Florissant lake beds, Colorado, United States

Ian C. Harding、Loraine S. Chant2000-01-01Geology

Research Article| March 01, 2000 Self-sedimented diatom mats as agents of exceptional fossil preservation in the Oligocene Florissant lake beds, Colorado, United States Ian C. Harding; Ian C. Harding 1School of Ocean and Earth Science, University of Southampton, European Way, Southampton SO14 3ZH, UK Search for other…

Geology and Paleoclimatology ResearchPaleontology and Stratigraphy of FossilsDiatoms and Algae Research

Influence of the counter ions and ligands on structures of silver(I) helicates with di-Schiff bases containing imidazole groups

Shiping Yang、Xiao‐Ming Chen、Liang‐Nian Ji2000-01-01Journal of the Chemical Society Dalton Transactions

Five complexes, [Ag6(bmimen)5(MeCN)][CF3SO3]6·H2O 1, [Ag7(bmimen)6][ClO4]7·MeCN 2, [Ag2(bmimen)2][NO3]2· 0.5H2O 3, [Ag3(bmimpn)2][CF3SO3]34 and [Ag3(bmimpn)2]n[NO3]3n5, were obtained by self-assembly of AgX (X = CF3SO3−, ClO4− or NO3−) with bmimen and bmimpn (bmimen = 1,2-bis[(1-methyl-2-imidazolyl)methyleneamino]etha…

Metal-Organic Frameworks: Synthesis and ApplicationsMetal complexes synthesis and propertiesMagnetism in coordination complexes

Polybis(4-azabenzimidazolato)-iron(II) and -cobalt(II). 3-D single diamond-like framework materials which exhibit spin canting and ferromagnetic ordering at low temperatures †

Steven J. Rettig、Víctor Sánchez‐Mendieta、Alan Storr 等 5 位作者2000-01-01Journal of the Chemical Society Dalton Transactions

The direct reaction between ferrocene and an excess of molten 4-azabenzimidazole yielded amber-green crystals of polybis(4-azabenzimidazolato)iron(II), 1. Single crystal X-ray diffraction studies revealed tetrahedrally coordinated iron ions linked by single imidazolate bridges and forming a 3-D single diamond-like (di…

Metal-Organic Frameworks: Synthesis and ApplicationsMagnetism in coordination complexesLanthanide and Transition Metal Complexes

Ni/SiO2 catalyst with hierarchical pore structure prepared by phase separation in sol–gel process

Norifumi Nakamura、Ryōji Takahashi、Satoshi Sato 等 5 位作者2000-01-01Physical Chemistry Chemical Physics

Silica-supported nickel catalysts with both macropores and mesopores were prepared in an alkoxide-derived sol–gel process in the presence of poly(ethylene oxide) (PEO) with an average molecular weight of 100000. In this process, the interconnected macroporous morphology is formed when transitional structures of spinod…

Catalytic Processes in Materials ScienceMesoporous Materials and CatalysisCatalysis and Oxidation Reactions

Photometathesis activity and thermal stability of two types of mesoporous silica materials, FSM-16 and MCM-41

Yoshitaka Inaki、Hisao Yoshida、Kôichi Kimura 等 6 位作者2000-01-01Physical Chemistry Chemical Physics

The metathesis reaction of propene under photoirradiation was performed over two types of mesoporous silica materials, FSM-16 and MCM-41, and amorphous silica evacuated at high temperature. The activity increased with increasing evacuation temperature, and moreover, prehydration treatment before evacuation influenced…

Zeolite Catalysis and SynthesisMesoporous Materials and CatalysisPolyoxometalates: Synthesis and Applications

Stability and electronic property investigations of the graphitic C3N4 system showing an orthorhombic unit cell

Maurizio Mattesini、Samir F. Matar、J. Étourneau2000-01-01Journal of Materials Chemistry

Recently, Alves et al. have suggested a new orthorhombic lattice system as a possible form for the graphitic C3N4 model structure. For this new phase, some modifications in the electronic properties are expected with respect to the hexagonal variety previously proposed by Teter and Hemley. A theoretical investigation…

Advancements in Battery MaterialsGraphene research and applicationsBoron and Carbon Nanomaterials Research

Drape Analysis using Imaging Techniques

D. Robson、Christina C. Long2000-01-01Clothing and Textiles Research Journal

Many textile properties have traditionally been assessed using subjective methods dependent upon one or more of the human senses. It is generally accepted that these methods can be unreliable, and the development of more reliable and consistent objective measurement systems is a key objective for textile scientists. I…

Textile materials and evaluationsColor Science and ApplicationsIndustrial Vision Systems and Defect Detection

Influence of Water Composition and Substrate on Electrochemical Scaling

R. Jaouhari、A. Benbachir、A. Guenbour 等 6 位作者2000-01-01Journal of The Electrochemical Society

Scaling of gold, bronze, and stainless steel was investigated in synthetic fresh and seawater. It is shown that the calcium carbonate precipitation rate increased from stainless steel, to bronze and then to gold whatever the composition of the scaling water. The morphology of the deposited scale depended on the substr…

Corrosion Behavior and InhibitionHydrogen embrittlement and corrosion behaviors in metalsElectrodeposition and Electroless Coatings

Spectroscopic characterisation of MoO3/TiO2 deNOx-SCR catalysts: Redox and coordination properties

Lorenzo Dall’Acqua、Isabella Nova、Luca Lietti 等 6 位作者2000-01-01Physical Chemistry Chemical Physics

MoO3/TiO2 catalysts prepared by impregnation of anatase with ammonium heptamolybdate have been investigated with the aim of understanding their redox chemistry and the coordination state of surface active species. Adsorption of ammonia has been followed by FTIR and by EPR on thermally treated, partially reduced sample…

Catalytic Processes in Materials ScienceCatalysis and Hydrodesulfurization StudiesCatalysis and Oxidation Reactions

Thermal degradation of biomedical polyurethanes?A kinetic study using high-resolution thermogravimetry

La�rcio Gomes Lage、Yoshio Kawano2000-01-01Journal of Applied Polymer Science

The kinetics of thermal degradation of polyurethanes (PUR) has been studied by means of high-resolution and constant heating rate thermogravimetry (TG), under nitrogen and synthetic air atmospheres. The high-resolution TG provided a way to increase resolution with decreasing the time of data acquisition. In this mode,…

Polymer crystallization and propertiesEnergetic Materials and CombustionThermal and Kinetic Analysis

Electron transfer reaction and demetalation of phthalocyanines

J. Kossanyi、Driss Chahraoui2000-01-01International Journal of Photoenergy

An electron‐transfer reaction takes place in the ground state between phthalocyanines (as electron‐donors) and pyrylium cations (as electron‐acceptors) in polar solvents, reaction which leads to the phthalocyanine radical‐cations as evidenced by its absorption spectra identical to the one of the species formed by elec…

Porphyrin and Phthalocyanine Chemistry

pH-dependent reversible polymers formed from cyclic sugar- and aromatic boronic acid-based bolaamphiphiles

Ikuo Nakazawa、Suda Sakae、Mitsutoshi Masuda 等 5 位作者2000-01-01Chemical Communications

Glucuronamide-based bolaamphiphiles are found to form a reversible, linear polymolecular array, via a boronate ester linkage attached to the 1,2-positions of the pyranose or furanose ring, upon complexation with an aromatic boronic acid-based homologue in aqueous solutions.

biodegradable polymer synthesis and propertiesConnective tissue disorders researchSupramolecular Self-Assembly in Materials

Synchrotron chemical crystallography

W. Clegg2000-01-01Journal of the Chemical Society Dalton Transactions

Recent years have seen a considerable development in the availability of single-crystal diffraction facilities with synchrotron radiation for use in non-biological crystallography, with access to several suitable beam-lines around the world. These can markedly extend the range of materials for which a full crystal str…

Crystallography and molecular interactionsEnzyme Structure and FunctionX-ray Diffraction in Crystallography

Increased intracellular drug accumulation and complete chemosensitization achieved in multidrug-resistant solid tumors by co-administering valspodar(PSC 833) with sterically stabilized liposomal doxorubicin

Rajesh Krishna、Maryse St‐Louis、Lawrence D. Mayer2000-01-01International Journal of Cancer

We have previously demonstrated that liposome encapsulation of doxorubicin (DOX) can alleviate adverse interactions with non-encapsulated DOX and the cyclosporine multidrug-resistant (MDR) modulator Valspodar. We have now investigated the behavior of different liposomal DOX formulations in MDA435LCC6/MDR-1 human breas…

Nanoparticle-Based Drug DeliveryDrug Transport and Resistance MechanismsNeonatal Health and Biochemistry

Interaction of ethylbenzene and styrene with iron oxide model catalyst films at low coverages: A NEXAFS study

Yvonne Joseph、Mario Wühn、Arno Niklewski 等 7 位作者2000-01-01Physical Chemistry Chemical Physics

The adsorption of ethylbenzene and styrene on well ordered epitaxial iron oxide model catalyst films with different stoichiometries was investigated using near-edge X-ray absorption fine structure spectroscopy (NEXAFS). On the iron-terminated Fe3O4(111) and α-Fe2O3(0001) surfaces chemisorption of ethylbenzene and styr…

Iron oxide chemistry and applicationsElectron and X-Ray Spectroscopy TechniquesSurface and Thin Film Phenomena

Ionic elastomer based on carboxylated nitrile rubber: infrared spectral analysis

U?K Mandal2000-01-01Polymer International

Carboxylated nitrile rubber (XNBR) neutralized by metal oxide forms an ionic elastomer (ionomer) due to formation of ionic clusters by the metal carboxylated salt. Cluster formation in carboxylated nitrile rubber by metal oxide, mainly zinc oxide (ZnO), has been studied by infrared analyses. Two modes of plasticizatio…

Polymer Nanocomposites and PropertiesDielectric materials and actuators

Diamond Growth Mechanisms in Various Environments

A. Gicquel、François Silva、Khaled Hassouni2000-01-01Journal of The Electrochemical Society

The goal of this study was to improve our understanding of diamond growth reactors. Direct relationships were set up between key parameters at a microscale level and diamond film characteristics. The coupled action of plasma variables, such as microwave power density, substrate temperature, and percentage of methane,…

Metal and Thin Film MechanicsDiamond and Carbon-based Materials ResearchElectronic and Structural Properties of Oxides

Characterization of Eu-Doped Y[sub 2]O[sub 3] Nanoparticles Prepared in Nonionic Reverse Microemulsions in Relation to Their Application for Field Emission Display

Myung-Han Lee、Seong‐Geun Oh、Sung Yi 等 8 位作者2000-01-01Journal of The Electrochemical Society

Characterization of Eu‐Doped Y 2 O 3 Nanoparticles Prepared in Nonionic Reverse Microemulsions in Relation to Their Application for Field Emission Display, Lee, Myung Han, Oh, Seong Geun, Yi, Sung Chul, Seo, Do Seok, Hong, Jin Pyo, Kim, Chae Ok, Yoo, Young Kil, Yoo, Jae Soo

Luminescence Properties of Advanced MaterialsPerovskite Materials and ApplicationsPolyoxometalates: Synthesis and Applications