Materials Literature
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Reconstructive surgery is presently struggling with the problem of infections located within implantation biomaterials. Of course, the best antibacterial protection is antibiotic therapy. However, oral antibiotic therapy is sometimes ineffective, while administering an antibiotic at the location of infection is often…
PO 4 3− polyanion-doped Li-rich layered oxides offer excellent energy density retention during long cycling due to the stronger anion bonding of PO 4 3− polyanions to transition metal cations.
The core–shell MOF templated synthesis of porous NiFe 2 O 4 @Fe 2 O 3 nanotubes that exhibit a large reversible capacity, excellent cycling stability and superior rate capability as anode materials for Li-ion batteries.
We made comparison of titanium dioxide powders obtained from three syntheses including sol‐gel and precipitation methods as well as using layered (tetramethyl)ammonium titanate as a source of TiO 2 . The obtained precursors were subjected to step annealing at elevated temperatures to transform into rutile form. The tr…
The use of a density functional theory methodology with on-site corrections (DFT + U) has been repeatedly shown to give an improved description of localised d and f states over those predicted with a standard DFT approach. However, the localisation of electrons also carries with it the problem of metastability, due to…
By utilizing the synergistic effect of poly-dopamine (PD) with functional groups and graphene oxide (GO) with a high surface area, a series of sub-nano thick PD layer coated GO (PD/GO) composites were fabricated and used for effectively decontaminating wastewater.
One pot conversion of chitin into 3A5AF opens up a new avenue for renewable, value added N-containing chemicals.
A new mesoporous MOF, Zn4O(bpdc)(btctb)(4/3) (DUT-32), containing linear ditopic (bpdc(2-); 4,4'-biphenylenedicarboxylic acid) and tritopic (btctb(3-); 4,4',4''-[benzene-1,3,5-triyltris(carbonylimino)]tris-benzoate) linkers, was synthesised. The highly porous solid has a total pore volume of 3.16 cm(3) g(-1) and a spe…
An oligothiophene derivative named DR3TBDTT with high hydrophobicity was synthesized and functioned as the hole transporting material without an ion additive. 8.8% of power conversion efficiency was obtained for CH3NH3PbI3-xClx based planar solar cells with improved stability, compared to devices using Li-TFSI doped s…
The ability to find synergic solutions is the core of scientific research and scientific advancement. This is particularly true for medicine, where multimodal imaging and theranostic tools represent the frontier research. Nanotechnology, which by its very nature is multidisciplinary, has opened up the way to the engin…
This review introduces the development and application of a multiscale approach to assess the charge mobility for organic semiconductors, which combines quantum chemistry, Kinetic Monte Carlo (KMC), and molecular dynamics (MD) simulations. This approach is especially applicable in describing a large class of organic s…
Enhanced performance for the bioelectrosynthesis of acetate from carbon dioxide is achieved with a new three-dimensional CNT-modified scaffold electrode.
The cycling performance and SEI composition of Si nano-particle anodes in electrolytes containing 5–25 wt% fluoroethyelene carbonate (FEC) and 3–6 wt% vinylene carbonate (VC) has been investigated by a combination of by electrochemical cycling, electrochemical impedance spectroscopy, IR-ATR and XPS. The incorporation…
This tutorial review details the emergence of template-directed synthesis of metal-organic materials (MOMs) with emphasis upon reports of MOMs in which the template is retained, template@MOMs, and structurally characterized. Such MOMs enable analysis of the nature of the intermolecular interactions that occur between…
The treatment of central nervous system (CNS) disease has long been difficult due to the ineffectiveness of drug delivery across the blood-brain barrier (BBB). This review summarizes important concepts of the BBB in normal versus pathophysiology and how this physical, enzymatic, and efflux barrier provides necessary p…
This tutorial review summarises recent advances in the direct supramolecular templating of metal-organic frameworks (MOFs) with hierarchical porosity across the micro- and mesoporous regimes. These are set against the important synthetic considerations that need to be addressed to ensure that strong interactions betwe…
Indene-C60 bisadduct (ICBA) is used as an electron-cascade acceptor material in poly{4,8-bis[(2-ethylhexyl)oxy]benzo[1,2-b:4,5-b′]dithiophene-2,6-diyl-alt-3-fluoro-2-[(2-ethylhexyl)carbonyl]thieno[3,4-b]thiophene-4,6-diyl} (PTB7):[6,6]-phenyl-C71-butyric-acid-methyl-ester (PC71BM) blend to fabricate ternary blend poly…
Two kinds of defects in g-C 3 N 4 caused by high temperature calcination limit the photocatalytic H 2 evolution activity. These defects are identified as amino/imino groups and controlling them will be key to improving the performance of the material for solar energy conversion.
The inorganic-organic perovskite is currently attracting a lot of attention due to its use as a light harvester in solar cells. The large absorption coefficients, high carrier mobility and good stability of organo-lead halide perovskites present good potential for their use as light harvesters in mesoscopic heterojunc…
This paper presents a thorough literature review of the powder-based electron beam additive manufacturing (EBAM) technology. EBAM, a relatively new additive manufacturing (AM) process, can produce full-density metallic parts directly from the electronic data of the designed part geometry. EBAM has gained broad attenti…