Materials Literature
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Abstract We present a high‐throughput method for fabricating large arrays of surface‐enhanced Raman scattering (SERS) active gold dimers. Using a large‐area/low‐cost nanopatterning method in conjunction with a meniscus force deposition technique, we were able to create large arrays of uniformly spaced nanoclusters com…
At the moment two competing explanations exist for the experimental finding that net negatively charged proteins adsorb on or absorb in negatively charged polyelectrolyte brushes. One explanation is based on the possibility of charge regulation. The idea is that a protein can reverse its charge when it is in the prese…
Conducting polymer bending actuators show potential for unique manipulation devices, particularly at the microscale, given low actuation voltages, controllable manufacture, biocompatibility, and ability to operate in either air or liquid environments; however, the impracticalities of implementing feedback in these env…
BACKGROUND: Bombyx mori, the domesticated silkworm, is a well-studied model insect with great economic and scientific significance. Although more than 400 mutations have been described in silkworms, most have not been identified, especially those affecting economically-important traits. Simple sequence repeats (SSRs)…
Reported here is an extension of the nanotube longitudinal unzipping process to convert electrode-bound multiwalled carbon nanotube (MWCNT) devices into graphene nanoribbon devices. Microscopy and Raman spectroscopy were used to monitor the conversion process. The electrical properties of the devices were characterize…
In this paper, a flatness-based nonlinear control method is proposed to control a multisource/multiload electrical hybrid system (EHS). The EHS is composed of a fuel cell and a supercapacitor-bank (SCB) as the main and auxiliary sources. They supply two independent loads, connected to a dc-bus through unidirectional b…
According to the concepts of attribute axis and attribute coordinate system, porphine and 11 kinds of bridge carbon substituted porphyrins as donors and 9 common acceptors A-I have been designed and calculated at the density functional B3LYP level. The substituent effects on the molecular orbital energy levels of the…
For the investigation of the interaction of nanoparticles with biomolecules, cells, organs, and animal models there is a need for well-characterized nanoparticle suspensions. In this paper we report the preparation of monodisperse dense amorphous silica nanoparticles (SNP) suspended in physiological media that are ste…
The alpha/beta hydrolase superfamily has rapidly expanded in recent years and continues to do so at an expeditious pace. According to the ESTHER database (http://bioweb.ensam.inra.fr/ESTHER) 29000 papers have been published cataloguing 89 family groups, comprising a total of 15438 gene loci and 666 structures. This pa…
Despite their importance in many chemical processes, the relative energies of spin states of transition metal complexes have so far been haunted by large computational errors. By the use of six functionals, B3LYP, BP86, TPSS, TPSSh, M06, and M06L, this work studies nine complexes (seven with iron and two with cobalt)…
Off-axis electron holography was used to observe and quantify the magnetic microstructure of a perpendicular magnetic anisotropic (PMA) recording media. Thin foils of PMA materials exhibit an interesting up and down domain configuration. These domains are found to be very stable and were observed at the same time with…
A theoretical study of magnetic field (h) effects on single-particle spectra and transport quantities of heavy fermion metals in the paramagnetic phase is carried out. We have employed a non-perturbative local moment approach (LMA) to the asymmetric periodic Anderson model within the dynamical mean field framework. Th…
We investigated the magnetization reversal of arrays of exchange biased NiO/Ni squares with superconducting quantum interference device magnetometry and micromagnetic simulations. The edges of the squares were 0.5, 1.5, and 3.0 $μ$m long. The NiO/Ni structures exhibit vortexlike hysteresis loops and micromagnetic calc…
We present a study of the local strain effects associated with vacancy defects in strontium titanate and report the first calculations of elastic dipole tensors and chemical strains for point defects in perovskites. The combination of local and long-range results will enable determination of x-ray scattering signature…
The discovery of spin torque transfer (STT) has lead to a significant advance in the development of spintronic devices. Novel structures and materials have been studied in order to improve the performance of the magnetic tunnel junctions (MTJs) performances and understand the fundamental physics in spin torque transfe…
Metal and semiconductor nanoparticles attract much attention due to their astonishing properties and numerous possibilities for applications in sensors. Significant progress has been made on the synthesis of metal and semiconductor nanoparticles with different shapes, composition, and controllable optical and electric…
In situ high-pressure Raman spectroscopy is used to study monolayer, bilayer, and few-layer graphene samples supported on silicon in a diamond anvil cell to 3.5 GPa. The results show that monolayer graphene adheres to the silicon substrate under compressive stress. A clear trend in this behavior as a function of graph…
Upon application of a uniform strain, internal sublattice shifts within the unit cell of a noncentrosymmetric dielectric crystal result in the appearance of a net dipole moment: a phenomenon well known as piezoelectricity. A macroscopic strain gradient on the other hand can induce polarization in dielectrics of any cr…
We have systematically investigated the effect of oxidation on the structural and electronic properties of graphene based on first-principles calculations. Energetically favorable atomic configurations and building blocks are identified, which contain epoxide and hydroxyl groups in close proximity with each other. Dif…
Mesocrystals are 3D ordered nanoparticle superstructures, often with internal porosity, which receive much recent research interest. While more and more mesocrystal systems are found in biomineralization or synthesized, their potential as material still needs to be explored. It needs to be revealed, which new chemical…