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Hydrothermal synthesis, structure, and sorption properties of the new microporous ferric molybdenum phosphates [(CH3)4N]2(NH4)2[Fe2Mo12O30(H2PO4)6(HPO4)2].nH2O and [(CH3)4N]2Na4[Fe3Mo12O30(HxPO4)8].nH2O

Linda A. Meyer、Robert C. Haushalter1993-04-01Inorganic Chemistry

ADVERTISEMENT RETURN TO ISSUEPREVArticleNEXTHydrothermal synthesis, structure, and sorption properties of the new microporous ferric molybdenum phosphates [(CH3)4N]2(NH4)2[Fe2Mo12O30(H2PO4)6(HPO4)2].nH2O and [(CH3)4N]2Na4[Fe3Mo12O30(HxPO4)8].nH2OLinda A. Meyer and Robert C. HaushalterCite this: Inorg. Chem. 1993, 32,…

Metal-Organic Frameworks: Synthesis and ApplicationsPolyoxometalates: Synthesis and ApplicationsChemical Synthesis and Characterization

Evaluating the Large Electromigration Resistance of Copper Interconnects Employing a Newly Developed Accelerated Life‐Test Method

T. Nitta、Tadahiro Ohmi、T. Hoshi 等 7 位作者1993-04-01Journal of The Electrochemical Society

An accelerated electromigration life‐test method has been developed to evaluate the large electromigration resistance of Cu interconnects in a very short period of test time. The essence of the acceleration technique employed here is to use stress current more than 10 7 A/cm 2 and to utilize the self‐heating of the te…

Electronic Packaging and Soldering Technologies3D IC and TSV technologiesCopper Interconnects and Reliability

Phase equilibria in block copolymer-homopolymer mixtures

A. N. Semenov1993-04-01Macromolecules

Phase equilibria in block copolymer (AB) + homopolymer (A) blends are considered theoretically in the strong segregation limit. The effect of homopolymer molecular weight is analyzed. In particular, the following are shown: (i) Long enough A-homopolymer chains (N(h) much greater than N(hc)) are incompatible with stret…

Polymer crystallization and propertiesAdvanced Polymer Synthesis and CharacterizationBlock Copolymer Self-Assembly

Preform permeability predictions by self‐consistent method and finite element simulation

Alexander L. Berdichevsky、Zhong Cai1993-04-01Polymer Composites

Abstract The self‐consistent method and finite element simulations have been used to estimate the permeability of an aligned fiber bundle. The self‐consistent method gives out formulas for both longitudinal and transverse permeabilities as functions of the fiber volume fraction. The finite element simulation presents…

High voltage insulation and dielectric phenomenaEpoxy Resin Curing ProcessesAerosol Filtration and Electrostatic Precipitation

Binding Mechanism of 2,4‐Dichlorophenoxyacetic Acid by Organo‐Clays

M.C. Hermosı́n、J. Cornejo1993-04-01Journal of Environmental Quality

Abstract The interaction of the herbicide 2,4‐dichlorophenoxyacetic acid (2,4‐D) with decylammonium‐montmorillonite (C10M) and decylammonium‐vermiculite (C10V) was studied by measuring 2,4‐D adsorption at different pH levels, and by preparing herbicide‐organic clay complexes which were characterized by x‐ray diffracti…

Pesticide and Herbicide Environmental StudiesClay minerals and soil interactions

Microstructural and chemical properties of ceria-supported rhodium catalysts reduced at 773 K

S. Bernal、F.J. Botana、José J. Calvino 等 8 位作者1993-04-01The Journal of Physical Chemistry

ADVERTISEMENT RETURN TO ISSUEPREVArticleNEXTMicrostructural and chemical properties of ceria-supported rhodium catalysts reduced at 773 KS. Bernal, F. J. Botana, J. J. Calvino, M. A. Cauqui, G. A. Cifredo, A. Jobacho, J. M. Pintado, and J. M. Rodriguez-IzquierdoCite this: J. Phys. Chem. 1993, 97, 16, 4118–4123Publicat…

Electrocatalysts for Energy ConversionCatalytic Processes in Materials ScienceNanomaterials for catalytic reactions

Biodegradability and mechanical properties of poly-(beta-hydroxybutyrate-co-beta-hydroxyvalerate)-starch blends

Bruce A. Ramsay、Vincent Langlade、Pierre J. Carreau 等 4 位作者1993-04-01Applied and Environmental Microbiology

Wheat starch granules and poly-(beta-hydroxybutyrate-co-beta-hydroxyvalerate) [P(HB-co-HV), (19.1 mol% HV)] were blended at 160 degrees C. Increasing the starch content from 0 to 50% (wt/wt) decreased the tensile strength of P(HB-co-HV) from 18 MPa to 8 MPa and diminished flexibility as Young's modulus increased from…

biodegradable polymer synthesis and propertiesElectrospun Nanofibers in Biomedical ApplicationsCarbon dioxide utilization in catalysis

Nickel carbonyl [Ni(CO)4] and iron carbonyl [Fe(CO)5]: molecular structures in the solid state

Dario Braga、Fabrizia Grepioni、A.G. Orpen1993-04-01Organometallics

ADVERTISEMENT RETURN TO ISSUEPREVArticleNEXTNickel carbonyl [Ni(CO)4] and iron carbonyl [Fe(CO)5]: molecular structures in the solid stateDario Braga, Fabrizia Grepioni, and A. Guy OrpenCite this: Organometallics 1993, 12, 4, 1481–1483Publication Date (Print):April 1, 1993Publication History Published online1 May 2002…

Metal complexes synthesis and propertiesMagnetism in coordination complexesInorganic and Organometallic Chemistry

Mechanisms and Kinetics of Reaction‐Bonded Aluminum Oxide Ceramics

Suxing Wu、Dietmar Holz、Nils Claussen1993-04-01Journal of the American Ceramic Society

Reaction‐bonded Al 2 O 3 (RBAO) ceramics were fabricated starting from mechanically alloyed Al 2 O 3 /Al, Al 2 O 3 / Al/ZrO 2 , and Al 2 O 3 /Al/ZrO 2 /Zr mixtures. Isopressed compacts were heat‐treated in air up to 1550°C. Reaction‐bonding mechanisms, kinetics, and the influence of ZrO 2 and Zr additions are investig…

Concrete and Cement Materials ResearchAdvanced ceramic materials synthesisAluminum Alloys Composites Properties

Autoactivation of catalytic (C alpha) subunit of cyclic AMP-dependent protein kinase by phosphorylation of threonine 197.

Robert A. Steinberg、Robert D. Cauthron、Marina M. Symcox 等 4 位作者1993-04-01Molecular and Cellular Biology

We recently found, using cultured mouse cell systems, that newly synthesized catalytic (C) subunits of cyclic AMP-dependent protein kinase undergo a posttranslational modification that reduces their electrophoretic mobilities in sodium dodecyl sulfate (SDS)-polyacrylamide gels and activates them for binding to a Sepha…

Enzyme Structure and FunctionBiochemical and Molecular ResearchBiotin and Related Studies

2,2′‐Bipyrimidineoxalatocopper(II) Complexes: From the Mononuclear Complex to the 2D Sheetlike Polymer

Giovanni De Munno、Miguel Julve、F. Nicolò 等 7 位作者1993-04-01Angewandte Chemie International Edition in English

An unusual two-dimensional mesh of CuII ions is found in complex 1(see picture); the metal atoms are bridged by oxalato (ox) and bipyrimidine (bpym) ligands to form ringshaped hexamers. Variable-temperature magnetic susceptibility measurements indicate that antiferromagnetic coupling between the Cu atoms occurs.

Metal-Organic Frameworks: Synthesis and ApplicationsMagnetism in coordination complexesLanthanide and Transition Metal Complexes

Are the equilibrium concentrations of carbon monoxide and hydrogen exceeded during the oxidation of methane over a nickel/ytterbium oxide catalyst?

D. P. Dissanayake、Michael P. Rosynek、Jack H. Lunsford1993-04-01The Journal of Physical Chemistry

ADVERTISEMENT RETURN TO ISSUEPREVArticleNEXTAre the equilibrium concentrations of carbon monoxide and hydrogen exceeded during the oxidation of methane over a nickel/ytterbium oxide catalyst?Dhammike Dissanayake, Michael P. Rosynek, and Jack H. LunsfordCite this: J. Phys. Chem. 1993, 97, 15, 3644–3646Publication Date…

Electrocatalysts for Energy ConversionCatalytic Processes in Materials ScienceCatalysis and Oxidation Reactions

Experimental/theoretical studies of the paramagnetic 52/53-electron triangular metal [Ni3(.eta.5-C5H5)3(.mu.3-S)2]n series (n = 1+, 0) containing weak metal-metal bonding interactions: Fenske-Hall MO analysis of the trimetal-antibonding frontier orbitals involved in the reversible redox-generated change in nickel-sulfur Ni3S2 core geometry

Terry E. North、James B. Thoden、Brock Spencer 等 4 位作者1993-04-01Organometallics

ADVERTISEMENT RETURN TO ISSUEPREVArticleNEXTExperimental/theoretical studies of the paramagnetic 52/53-electron triangular metal [Ni3(.eta.5-C5H5)3(.mu.3-S)2]n series (n = 1+, 0) containing weak metal-metal bonding interactions: Fenske-Hall MO analysis of the trimetal-antibonding frontier orbitals involved in the reve…

Magnetism in coordination complexesInorganic Chemistry and MaterialsInorganic Fluorides and Related Compounds

Synthesis, Resolution and Kinetics of Electron Self-Exchange of High-Spin Manganese(II)/(III) Cage Complexes

PA Anderson、II Creaser、Christopher Dean 等 9 位作者1993-04-01Australian Journal of Chemistry

The ligand sarcophagine ( sar = 3,6,10,13,16,19-hexaazabicyclo[6.6.6] icosane ) rapidly reacts with [ Mn (OH2)6]2+ to form the nearly colourless [ Mn ( sar )]2+ ion, which can readily be oxidized to the bright orange [Mn ( sar )]3+ ion (E°'+0.53 V v. n.h.e. in 0.1 mol l-1 CF3SO3H at 295 K). A single-crystal structure…

Metal complexes synthesis and propertiesMagnetism in coordination complexesLanthanide and Transition Metal Complexes

Why Direct Tension Test Specimens Break Flexing to the Side

Zdeněk P. Bažant、Luigi Cedolin1993-04-01Journal of Structural Engineering

Contrary to the traditional view, unnotched direct tension test specimens of quasi‐brittle materials that exhibit post‐peak strain softening do not deform symmetrically. After passing the peak load, the equilibrium path bifurcates and the secondary postbifurcation branch represents flexing to the side. The bifurcation…

Fatigue and fracture mechanicsElasticity and Material ModelingHigh-Velocity Impact and Material Behavior

Indentation Crack Initiation and Propagation in Tempered Glass

Rajan Tandon、Robert E. Cook1993-04-01Journal of the American Ceramic Society

Indentation crack initiation and propagation in tempered glass surfaces are examined and the results compared to those in annealed and in ion‐exchange‐strengthened glasses. The presence of surface compression due to tempering inhibits median crack initiation during the loading cycle of the indentation and depresses th…

Dental materials and restorationsAdvanced ceramic materials synthesisAdvanced Surface Polishing Techniques

The layered ternary germanium tellurides ZrGeTe4, HfGeTe4, and TiGeTe6: structure, bonding, and physical properties

Arthur Mar、James A. Ibers1993-04-01Journal of the American Chemical Society

ADVERTISEMENT RETURN TO ISSUEPREVArticleNEXTThe layered ternary germanium tellurides ZrGeTe4, HfGeTe4, and TiGeTe6: structure, bonding, and physical propertiesArthur Mar and James A. IbersCite this: J. Am. Chem. Soc. 1993, 115, 8, 3227–3238Publication Date (Print):April 1, 1993Publication History Published online1 May…

2D Materials and ApplicationsCrystal Structures and PropertiesInorganic Chemistry and Materials

Competitive and noncompetitive reversible binding processes

Noam Agmon1993-04-01Physical review. E, Statistical physics, plasmas, fluids, and related interdisciplinary topics

This work treats many-body aspects in an idealized class of reversible binding problems involving a static binding site with many diffusing point particles. In the noncompetitive limit, where no restriction exists on the number of simultaneously bound particles, the problem reduces to reversible aggregation. In the co…

Material Dynamics and PropertiesTheoretical and Computational PhysicsStochastic processes and statistical mechanics

Platinum Sulfide by XPS

J. Dembowski、L. Marosi、Martin Essig1993-04-01Surface Science Spectra

It is known from crystallographic investigations that there are two distinct Pt–S modifications, PtS and PtS2 [see R. Collins, R. Kaner, P. Russo, A. Wold, and D. Avignant, Inorg. Chem. 18, 727 (1979); A. Finley, D. Schleich, J. Ackerman, S. Soled, and A. Wold, Mater. Res. Bull. 9, 1655 (1974); S. Soled, A. Wold, and…

Electron and X-Ray Spectroscopy TechniquesSurface and Thin Film PhenomenaAdvanced Materials Characterization Techniques

CuCl by XPS

R. P. Vasquez1993-04-01Surface Science Spectra

X-ray photoemission measurements of high purity CuCl are presented. XPS studies of Cu compounds have been motivated in this laboratory by the need to identify species on high temperature superconductor surfaces which have been chemically etched [see R. P. Vasquez, M. C. Foote, and B. D. Hunt, J. Appl. Phys. 66, 4866 (…

Electron and X-Ray Spectroscopy TechniquesX-ray Diffraction in CrystallographySurface and Thin Film Phenomena