Materials Literature
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In an ideal graphene sheet charge carriers behave as two-dimensional (2D) Dirac fermions governed by the quantum mechanics of massless relativistic particles. This has been confirmed by the discovery of a half-integer quantum Hall effect in graphene flakes placed on a SiO2 substrate. The Dirac fermions in graphene, ho…
Microbial polyhydroxyalkanoates (PHA) were proposed for the first time as a new type of biofuel. In this paper, poly-R-3-hydroxybutyrate (PHB) and medium chain length PHA (mcl PHA) were, respectively, esterified to become R-3-hydroxybutyrate methyl ester (3HBME) and medium chain length hydroxyalkanoate methyl ester (3…
The Weighted Burgers Vector (WBV) is defined here as the sum, over all types of dislocations, of [(density of intersections of dislocation lines with a map) x (Burgers vector)]. Here we show that it can be calculated, for any crystal system, solely from orientation gradients in a map view, unlike the full dislocation…
Fibrin is a natural biopolymer involved in the coagulation cascade. It acts as a reservoir for growth factors, cells, and enzymes during wound healing and provides a scaffold for the synthesis of extracellular matrix. Thus, the use of fibrin has expanded in recent years from traditional use as a sealant for surgical a…
We studied the impurity scattering on the $\ifmmode\pm\else\textpm\fi{}s$-wave superconductor (SC), with realistic parameters for the Fe pnictide SCs. Using the $\mathcal{T}$-matrix method, generalized for the two bands, we found that the strong scattering limit of impurities forms an off-centered resonance state insi…
With their increased use, engineered nanomaterials (ENMs) will enterthe environment where they may be altered by bacteria and affect bacterial processes. Metallic ENMs, such as CdSe quantum dots (QDs), are toxic due to the release of dissolved heavy metals, but the effects of cadmium ions versus intact QDs are mostly…
The electronic structure and physical properties of the pnictide compound families RE OFeAs ( RE =La, Ce, Pr, Nd, Sm), A Fe 2 As 2 ( A =Ca, Sr, Ba, Eu), LiFeAs and FeSe are quite similar. Here, we focus on the members of the A Fe 2 As 2 family whose sample composition, quality and single-crystal growth are more contro…
The occurrence of high-temperature superconductivity, and the competition with magnetism, in stoichiometric and doped LaFeAsO and isostructural iron oxypnictides is raising many fundamental questions about the electronic structure and magnetic interactions in this class of materials. There are now sufficient experimen…
Neutron scattering measurements were performed to investigate magnetic excitations in a single-crystal sample of the ternary iron arsenide ${\text{BaFe}}_{2}{\text{As}}_{2}$, a parent compound of a recently discovered family of Fe-based superconductors. In the ordered state, we observe low energy spin-wave excitations…
Abstract Novel nanowall arrays of hydrous manganese dioxide MnO 2 · 0.5H 2 O are deposited onto cathodic substrates by the potentiostatic method from a mixed aqueous solution of manganese acetate and sodium sulfate. The deposition is induced by a change of local pH resulting from electrolysis of H 2 O, and hierarchica…
This manuscript describes the accurate deposition of carbon on the surface of ZnO nanorods by a simple, microwave-assisted method and the studies on the cytotoxicity and photocatalytic activity of the C/ZnO hybrids. For the coating of carbon, the surface of the preformed ZnO nanorods were first modified by amino group…
Abstract 1‐longitudinal optical (LO) phonons in free‐standing mixed Cd 1− x Zn x S nanocrystals, synthesized using chemical precipitation, are investigated using Raman spectroscopy. As expected for the nanocrystals, the 1‐LO modes are found to appear at slightly lower wavenumbers than those in the bulk mixed crystals…
We have grown lead iron niobate thin films with composition Pb(Fe1/2Nb1/2)O3 (PFN) on (0 0 1) SrTiO3 substrates by pulsed laser deposition. The influence of the deposition conditions on the phase purity was studied. Due to similar thermodynamic stability spaces, a pyrochlore phase often coexists with the PFN perovskit…
A mixed quantum mechanical and Monte Carlo method for calculating Auger spectra from nanoclusters is presented. The approach, based on a cluster method, consists of two steps. Ab initio quantum mechanical calculations are first performed to obtain accurate energy and probability distributions of the generated Auger el…
Biphasic Janus particles with a precisely tunable internal morphology are fabricated using a novel, versatile, and robust technique. This technique can be used in conjunction with microfluidics to produce monodisperse particles, or can be combined with bulk emulsification techniques to produce large quantities of part…
The development of one-dimensional fluorescent nanowires (1D-NWs) and their higher-dimensional architectures such as nanowebs and nanofabrics (2D-NFs) could open a new area in nanomaterials science and nanotechnology. In particular, fluorescent pi-electronic 1D-NWs are considered promising materials for realizing inno…
As the concentration of intrinsic defects becomes sufficiently high in O-deficient ZnO, interactions between defects lead to a significant reduction in their formation energies. We show that the formation of both O vacancies and Zn interstitials becomes significantly enhanced by a strong attractive interaction between…
Shape effects of synthetic carriers are largely unexplored in vivo, although recent findings suggest that flexible filaments can persist in the circulation even if microns in length. Here, to better assess biodistribution, a near-infrared fluorophore (NIRF) was incorporated into such block copolymer "filomicelles", an…
A series of 122 phase BaFe 2− x Ni x As 2 ( x =0, 0.055, 0.096, 0.18 and 0.23) single crystals was grown by the self-flux method and a dome-like Ni doping dependence of the superconducting transition temperature was discovered. The transition temperature T c on reaches a maximum of 20.5 K at x =0.096, and it drops to…
We use dynamic light scattering and computer simulations to study equilibrium dynamics and dynamic heterogeneity in concentrated suspensions of colloidal hard spheres. Our study covers an unprecedented density range and spans seven decades in structural relaxation time, tau(alpha0, including equilibrium measurements a…