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Electric-field controlled spin in bilayer triangular graphene quantum dots

A. D. Güçlü、Paweł Potasz、Paweł Hawrylak2011-07-25Physical Review B

We present theoretical results based on mean-field and exact many-body approaches showing that in bilayer triangular graphene quantum dots with zigzag edges, the magnetism can be controlled by an external vertical electric field. We demonstrate that without electric field, the spins of the two layers of the quantum do…

Graphene research and applications2D Materials and ApplicationsQuantum and electron transport phenomena

Ultrafast Coloring-Bleaching Performance of Nanoporous WO3–SiO2 Gasochromic Films Doped with Pd Catalyst

Dezeng Li、Guangming Wu、Guohua Gao 等 5 位作者2011-07-25ACS Applied Materials & Interfaces

The gasochromic performance and durability of WO(3)-based films can be improved by doping SiO(2) particles within WO(3) matrix forming nanoporous supporting network and dispersing Pd catalyst inside films with enhanced catalytic activity. Nanoporous WO(3)-SiO(2) composite films loaded with Pd catalyst were prepared by…

TiO2 Photocatalysis and Solar CellsGas Sensing Nanomaterials and SensorsTransition Metal Oxide Nanomaterials

A stable and switchable uniform lying helix structure in cholesteric liquid crystals

Chun‐Ta Wang、Weiyuan Wang、Tsung‐Hsien Lin2011-07-25Applied Physics Letters

This investigation demonstrates an electrically switchable uniformly lying helix (ULH) stable state in cholesteric liquid crystal. A stable ULH state can be achieved by applying the low-frequency (30 Hz) pulse electrical field via an electro-hydrodynamatic effect. The ULH state can be stably maintained with a helical…

Photonic and Optical DevicesLiquid Crystal Research AdvancementsNonlinear Dynamics and Pattern Formation

Reconfigurable gradient index using VO2 memory metamaterials

M. D. Goldflam、T. Driscoll、B. Chapler 等 12 位作者2011-07-25Applied Physics Letters

We demonstrate tuning of a metamaterial device that incorporates a form of spatial gradient control. Electrical tuning of the metamaterial is achieved through a vanadium dioxide layer which interacts with an array of split ring resonators. We achieved a spatial gradient in the magnitude of permittivity, writeable usin…

Metamaterials and Metasurfaces ApplicationsAcoustic Wave Phenomena ResearchTransition Metal Oxide Nanomaterials

Human primary bronchial epithelial cells respond differently to titanium dioxide nanoparticles than the lung epithelial cell lines A549 and BEAS-2B

Barbro Ekstrand‐Hammarström、Christine Akfur、Per Ola Andersson 等 6 位作者2011-07-25Nanotoxicology

We have compared the cellular uptake and responses of five preparations of nanocrystalline titanium dioxide (TiO(2)) between normal human bronchial epithelial (NHBE) cells and epithelial cell lines (A549 and BEAS-2B). The P25 nanoparticles, containing both anatase and rutile modifications, induced reactive oxygen spec…

Nanoparticles: synthesis and applicationsAir Quality and Health ImpactsInhalation and Respiratory Drug Delivery

Biodegradable Bicomponent Fibers from Renewable Sources: Melt‐Spinning of Poly(lactic acid) and Poly[(3‐hydroxybutyrate)‐co‐(3‐hydroxyvalerate)]

Rudolf Hufenus、Felix A. Reifler、Katharina Maniura‐Weber 等 5 位作者2011-07-25Macromolecular Materials and Engineering

Abstract PHBV is produced by bacteria as intracellular carbon storage. It is advantageous concerning biocompatibility and biodegradability, but its low crystallization rate hinders the melt‐processing of fibers. This problem can be overcome by combining PHBV with PLA in a core/sheath configuration and introducing a ne…

biodegradable polymer synthesis and propertiesElectrospun Nanofibers in Biomedical ApplicationsCarbon dioxide utilization in catalysis

1,2-BN Cyclohexane: Synthesis, Structure, Dynamics, and Reactivity

Wei Luo、Lev N. Zakharov、Shih‐Yuan Liu2011-07-25Journal of the American Chemical Society

BN/CC isosterism has emerged as a viable strategy to increase the structural diversity of carbon-based compounds. We present the first synthesis and characterization of the parent 1,2-BN cyclohexane, the BN-isostere of cyclohexane. 1,2-BN cyclohexane is an air- and water-stable compound that cleanly forms a trimer wit…

Hydrogen Storage and MaterialsBoron and Carbon Nanomaterials ResearchOrganoboron and organosilicon chemistry

Room temperature picowatt-resolution calorimetry

Seid Sadat、Yi Jie Chua、Woochul Lee 等 7 位作者2011-07-25Applied Physics Letters

Picowatt-resolution calorimetry is necessary for fundamental studies of nanoscale energy transport. Here, we report a microfabricated device capable of <4 pW resolution—an order of magnitude improvement over state-of-the-art room temperature calorimeters. This is achieved by the incorporation of two important f…

Advanced Thermoelectric Materials and DevicesThermal properties of materialsThermal Radiation and Cooling Technologies

Giant electric field controlled magnetic anisotropy in epitaxial BiFeO3-CoFe2O4 thin film heterostructures on single crystal Pb(Mg1/3Nb2/3)0.7Ti0.3O3 substrate

Zhiguang Wang、Yaodong Yang、Ravindranath Viswan 等 5 位作者2011-07-25Applied Physics Letters

We have deposited self-assembled BiFeO3 (BFO)-CoFe2O4 (CFO) thin films on Pb(Mg1/3Nb2/3)0.7Ti0.3O3 (PMN-PT) substrates and studied the change in magnetic anisotropy under different strain conditions induced by an applied electric field. After electric field poling, we observed (i) giant magnetization change: magnetiza…

Ferroelectric and Piezoelectric MaterialsMagnetic and transport properties of perovskites and related materialsMultiferroics and related materials

Assessment of glycosaminoglycan concentration changes in the intervertebral disc via chemical exchange saturation transfer

Galit Saar、Boyang Zhang、Wen Ling 等 6 位作者2011-07-25NMR in Biomedicine

In this study, it is shown that the chemical exchange saturation transfer (CEST) method for hydroxyl protons can be used to detect changes in glycosaminoglycan (GAG) concentration in the intervertebral disc. The method, termed gagCEST, was demonstrated ex vivo by correlating the CEST effect with the fixed charge densi…

Advanced MRI Techniques and ApplicationsRadioactive element chemistry and processingLanthanide and Transition Metal Complexes

Massless Dirac fermions in a laser field as a counterpart of graphene superlattices

Sergey Savel’ev、A. S. Alexandrov2011-07-25Physical Review B

We establish an analogy between spectra of Dirac fermions in laser fields and an electron spectrum of graphene superlattices formed by static one-dimensional periodic potentials. The general relations between a laser-controlled spectrum where electron momentum depends on the quasienergy and a superlattice miniband spe…

Graphene research and applicationsQuantum Mechanics and ApplicationsQuantum optics and atomic interactions

Characteristic and Mechanism of Methane Dehydroaromatization over Zn-Based/HZSM-5 Catalysts under Conditions of Atmospheric Pressure and Supersonic Jet Expansion

B. S. Liu、Yan Zhang、Jiao Liu 等 7 位作者2011-07-25The Journal of Physical Chemistry C

The catalytic performance of Zn-based/HZSM-5 catalysts prepared by wet impregnation method was investigated for the methane dehydroaromatization (MDA) reaction under the conditions of atmospheric pressure and supersonic jet expansion (SJE). The physical properties of the catalysts were characterized by Brunauer–Emmett…

Catalytic Processes in Materials ScienceCatalysts for Methane ReformingCatalysis and Oxidation Reactions

Hierarchical Self‐assembly of Microscale Cog‐like Superstructures for Enhanced Performance in Lithium‐Ion Batteries

Weixin Zhang、Mei Li、Qiang Wang 等 7 位作者2011-07-25Advanced Functional Materials

Abstract Assembling complex nanostructures on functional substrates such as electrodes promises new multi‐functional interfaces with synergetic properties capable of integration into larger‐scale devices. Here, we report a microemulsion‐mediated process for the preparation of CuO/Cu electrodes comprising a surface lay…

Advancements in Battery MaterialsCopper-based nanomaterials and applicationsNanomaterials for catalytic reactions

Facile Physical Route to Highly Crystalline Graphene

Meihua Jin、Tae Hyung Kim、Seong Chu Lim 等 10 位作者2011-07-25Advanced Functional Materials

Abstract A physical route is proposed to obtain highly crystalline graphene sheets with minimal oxygen content similar to the precursor graphite. The functional graphene sheets obtained from graphite oxide by low temperature thermal exfoliation are annealed at high temperature (1900 °C) in a vacuum (10 −6 torr). The D…

Advancements in Battery MaterialsGraphene research and applications2D Materials and Applications

Analysis of a Fast Fourier Transform Based Method for Modeling of Heterogeneous Materials

J. Vondřejc、J. Zeman、I. Marek2011-07-25arXiv

The focus of this paper is on the analysis of the Conjugate Gradient method applied to a non-symmetric system of linear equations, arising from a Fast Fourier Transform-based homogenization method due to (Moulinec and Suquet, 1994). Convergence of the method is proven by exploiting a certain projection operator reflec…

Materials Sciencecs.NAmath.NAphysics.comp-ph

Symmetry analysis of possible superconducting states in KxFeySe2superconductors

I. I. Mazin2011-07-25Physical Review B

A newly discovered family of Fe-based superconductors is isostructural with the so-called 122 family of Fe pnictides but has a qualitatively different doping state. Early experiments indicate that superconductivity is nodeless, yet prerequisites for the ${s}_{\ifmmode\pm\else\textpm\fi{}}$ nodeless state (generally be…

Rare-earth and actinide compoundsIron-based superconductors research

Electronic structure of gold, aluminum, and gallium superatom complexes

Olga Lopez‐Acevedo、Andre Z. Clayborne、Hannu Häkkinen2011-07-25Physical Review B

Using ab initio computational techniques on crystal determined clusters, we report on the similarities and differences of Al${}_{50}$(C${}_{5}$(CH${}_{3}{{)}_{5})}_{12}$, Ga${}_{23}$(N(Si(CH${}_{3}{)}_{3}$)${}_{2}$)${}_{11}$, and Au${}_{102}$(SC${}_{7}$O${}_{2}$H${}_{5}$)${}_{44}$ ligand-protected clusters. Each of th…

Gold and Silver Nanoparticles Synthesis and ApplicationsMolecular Junctions and NanostructuresNanocluster Synthesis and Applications

Electrospinning Superhydrophobic Fibers Using Surface Segregating End-Functionalized Polymer Additives

Sarah J. Hardman、Norazilawati Muhamad-Sarih、Helen J. Riggs 等 7 位作者2011-07-25Macromolecules

We describe here a facile route for the in situ modification of the surface properties of fibers produced by electrospinning polystyrene containing small quantities of compatible polymer additives, end-functionalized with 1–3 fluoroalkyl groups. Such additives undergo spontaneous surface segregation during the electro…

Surface Modification and SuperhydrophobicityAdvanced Sensor and Energy Harvesting MaterialsElectrospun Nanofibers in Biomedical Applications

Multiferroic Polymer Composites with Greatly Enhanced Magnetoelectric Effect under a Low Magnetic Bias

Jiezhu Jin、Sheng‐Guo Lu、Chalathorn Chanthad 等 6 位作者2011-07-25Advanced Materials

Multiferroic laminate composites consisting of chain-end cross-linked ferroelectric polymers and magnetostrictive Metglas are reported. The composites exhibit a greatly enhanced multiferroic voltage coefficient and sensitivity relative to analogous composites. These remarkable properties are attributed to high piezoel…

Ferroelectric and Piezoelectric MaterialsMultiferroics and related materialsSmart Materials for Construction

Importance of the Fermi-surface topology to the superconducting state of the electron-doped pnictide Ba(Fe1−xCox)2As2

Chang Liu、Ari Palczewski、R. S. Dhaka 等 12 位作者2011-07-25Physical Review B

We used angle-resolved photoemission spectroscopy and thermoelectric power to study the poorly explored, highly overdoped side of the phase diagram of Ba(Fe${}_{1\ensuremath{-}x}$Co${}_{x}$)${}_{2}$As${}_{2}$ high-temperature superconductor. Our data demonstrate that several Lifshitz transitions---topological changes…

Iron-based superconductors researchIntellectual Capital and Performance Analysis