Materials Literature
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We study the surface plasmons (SPs) that exist at the interface between air and a metamaterial constructed of split ring resonators (SRRs). The SRR metamaterial possesses a frequency band in the microwave regime $(12.5--14\phantom{\rule{0.3em}{0ex}}\mathrm{GHz})$ over which the permeability is negative. We apply an at…
A quartz crystal microbalance with dissipation monitoring (QCM-D) was used to assess the physical properties of interpenetrating polymer networks (IPNs) through swelling experiments in ambient humidity and in phosphate-buffered saline (PBS), pH 7.4. The IPNs, based on acrylamide (AAm) and poly(ethylene glycol) (pEG),…
Understanding the effect of Mn substitution for Fe in Co ferrite presents a challenge because there are three different transition-metal ions distributed among two distinct crystallographic and magnetic sublattices with complicated superexchange and anisotropic interactions. In this study, a series of six powder sampl…
Studies have shown that poly(lactic-co-glycolic acid) (PLGA) films with nanometer surface features promote vascular endothelial and smooth muscle cell adhesion. The objective of this in vitro research was to begin to understand the mechanisms behind this observed increase in vascular cell adhesion. Results provided ev…
Current trends in the miniaturization of microwave devices have prompted considerable interest in studying electromagnetic transport in nanoscale systems. Understanding the effect of physical structure and the role of interfaces is critical for gaining insight into the electromagnetic and magnetic properties of nanost…
Wasp-waist and pot-belly hysteresis loops have been observed in many materials. When only the major loop is reported, the results are insufficient to establish which processes are involved. We present two models for wasp-waist materials that produce virtually indistinguishable major loops, but show that first-order re…
The fundamental optical properties of Ga-doped ZnO films grown by metalorganic chemical vapor deposition were investigated by room-temperature transmittance and photoluminescence (PL) spectroscopy. The Burstein–Moss (BM) shift of the absorption edge energy is observed at the carrier concentration up to 2.47×1019cm−3.…
We present a quantitative study of the thickness dependence of the polarization and piezoelectric properties in epitaxial (001) PbZr0.52Ti0.48O3 films grown on (001) SrRuO3-buffered (001) SrTiO3 substrates. High-resolution transmission electron microscopy reveals that even the thinnest films (∼8nm) are fully relaxed w…
High-quality single-crystal diamond films, homoepitaxially grown by microwave chemical vapor deposition, have been used to produce diamond-based photodetectors. Such devices were tested over a very wide spectral range, from the extreme ultraviolet (UV) (20 nm) up to the near IR region (2400 nm). An optical parametric…
Nanosized anatase (≤10 nm), rutile (≤10 nm), and brookite (∼70 nm) titania particles have been successfully synthesized via sonication and hydrothermal methods. Gold was deposited with high dispersion onto the surfaces of anatase, rutile, brookite, and commercial titania (P25) supports through a deposition−precipitati…
We report a Car-Parrinello molecular dynamics study of the liquid-liquid phase transition in phosphorus. We employed a gradient corrected density functional (B-LYP) to describe the electronic structure and performed simulations at constant pressure. Upon increasing pressure we observed, along the 1500 K isotherm, a st…
A series of wurtzite MgZnO quasi-ternary alloys, which consist of wurtzite MgO∕ZnO superlattices, were grown by molecular-beam epitaxy on sapphire substrates. By changing the thicknesses of ZnO layers and/or of MgO layers of the superlattice, the band-gap energy was artificially tuned from 3.30to4.65eV. The highest ba…
Phase transitions into a new phase that is itself metastable are common; instead of the equilibrium phase nucleating a metastable phase does so. When this occurs the system is sometimes said to be obeying Ostwald's rule. We show how this can happen when there are impurities present that reduce the barrier to heterogen…
The paramagnetic phase of heavy fermion systems is investigated, using a non-perturbative local moment approach to the asymmetric periodic Anderson model within the framework of dynamical mean field theory. The natural focus is on the strong coupling Kondo-lattice regime wherein single-particle spectra, scattering rat…
Relativistic band theoretical calculations reveal that intrinsic spin Hall conductivity in hole-doped archetypical semiconductors Ge, GaAs and AlAs is large $[\sim 100 (\hbar/e)(Ωcm)^{-1}]$, showing the possibility of spin Hall effect beyond the four band Luttinger Hamiltonian. The calculated orbital-angular-momentum…
Employing a local moment approach to the periodic Anderson model within the framework of dynamical mean-field theory, direct comparison is made between theory and experiment for the dc transport and optical conductivities of paramagnetic heavy fermion and intermediate valence metals. Four materials, exhibiting a diver…
We investigate the process of slow intergranular crack propagation by the finite element method model, and show that branching is induced by partial arresting of crack front owing to the geometrical randomness of grain boundaries. A possible scenario for branching instability of crack propagation in disordered continu…
We investigated the effect of mean-field electron correlations on the band electronic structure of Co, Ni, and Pd ultra-thin monatomic nanowires, at the breaking point, by means of density-functional calculations in the self-interaction corrected LDA approach (LDA+SIC) and alternatively by the LDA+$U$ scheme. We find…
The time decay of the thermo-remanent magnetization (TRM) in Fe-Cr giant magnetoresistive (GMR) multilayers has been investigated. The magnetization in these multilayers relaxes as a function of time after being cooled in a small magnetic field of 100 Oe to a low temperature and then the magnetic field is switched off…
Silicon-based quantum-computer architectures have attracted attention because of their promise for scalability and their potential for synergetically utilizing the available resources associated with the existing Si technology infrastructure. Electronic and nuclear spins of shallow donors (e.g. phosphorus) in Si are i…