Materials Literature
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How are the properties of a metal changed by strong inelastic scattering? We investigate this question within the two-dimensional t-J model using extended dynamical mean field theory and a generalized noncrossing approximation. Short-ranged antiferromagnetic fluctuations lead to a strongly incoherent single particle d…
Frequency Modulation Response of a Tunable Birefringent Mode Nematic Liquid Crystal Electrooptic Device Fabricated by Doping Nanoparticles of Pd Covered with Liquid-Crystal Molecules, Yoshikawa, Hiroaki, Maeda, Kenji, Shiraishi, Yukihide, Xu, Jun, Shiraki, Hiroyuki, Toshima, Naoki, Kobayashi, Shunsuke
The magnetic and electronic transport properties and the specific heat of La 1- x Ca x CoO 3 (0.05≤ x ≤0.5) have been investigated. In the whole composition range, the Co atoms are in an intermediate-spin (IS) state, and a spin glass or a ferromagnetic ordered state appears at low temperatures. The conductivity increa…
Self-assembled nanoporous materials have potential for many applications. Here we report unusual dendritic crystals from self-assembled nanoporous silicates and continuous morphological change of such materials through chemical means. We used hybrid organic silane and quaternary ammonium surfactants to prepare large d…
Rutile VO 2 nanorods have been synthesized by the precursor morphology controlled formation. The precursor single-crystal VO 2 hydrate nanorods have been obtained via the hydrothermal reaction of KOH, V 2 O 5, and hydrazine in a sealed autoclave at low temperature. The reducing agent N 2 H 4 plays a key role in the co…
Nitrogen (N) doping in ZnO is studied to realize reproducible p-type conductivity. Undoped ZnO layers prepared on a-face of sapphire substrates with H 2 O vapor-assisted growth showed n-type conductivity. However, N-doped ZnO (ZnO:N) layers grown in the similar manner showed the type conversion to p-type conductivity.…
The effect of ultrasonic vibration in the Reynolds number ( Re ) range of 1500 to 6000 on fluid flow in a square channel was investigated experimentally. An ultrasonic transducer was fixed at the center of the bottom of a square test channel, and a standing wave field was formed in this channel. The velocity of the fl…
We have investigated the interface effect on magnetic and transport properties in the superlattices composed of ferromagnetic La 1- x Sr x MnO 3 (LSMO) and non magnetic SrTiO 3 (STO) ( x = 0.2, 0.3, and 0.4). The interface of LSMO with STO was proved to show spin-canting, the degree of which critically depends on the…
The nonreducible mechanism of {(Ba 1- x Ca x )O} m TiO 2 ( m >1) ceramics fired in a reducing atmosphere was investigated by measuring the electrical conduction under various atmospheres at elevated temperatures. The high insulation resistance of the Ca-doped BaTiO 3 ceramics can be explained by the following three fa…
We design a new class of carbon-network materials with a periodically modified graphite sheet. The modified part corresponds to (6,6) carbon-nanotube geometry. Their tube parts form triangular lattice on graphite sheet. On these systems each tube has six heptagons at the bottom, giving rise to a seamless s p 2 -C netw…
A conventional high voltage wire-like plasma enhanced and spread by a pulsed microwave was used to study the oxidative coupling and reforming of CH 4 with CO 2 to CO, C 2 H 2, C 2 H 4, and H 2 . Under the conditions of atmospheric pressure, a flow rate of 200 mL/min (CH 4 /CO 2 = 1.5:1), peak microwave power of 120 W,…
M4DOTA, [(2S,5S,8S,11S)-4,7,10-tris-carboxymethyl-2,5,8,11-tetramethyl-1,4,7,10-tetraazacyclododecan-1-yl]acetic acid (2e), and M4DOTMA, (R)-2-[(2S,5S,8S,11S)-4,7,10-tris-((R)-1-carboxyethyl)-2,5,8,11-tetramethyl-1,4,7,10-tetraazacyclododecan-1-yl]propionic acid (3e), are derivatives of ligand DOTA (1e) that form ster…
Hydrated rare earth hexaborates H 3 LnB 6 O 12 (Ln = Sm−Lu) have been synthesized by using molten boric acid as the reaction medium. H 3 LnB 6 O 12 decomposes at certain temperatures to form anhydrous pentaborates LnB 5 O 9 (Ln = Sm−Er) or orthoborates LnBO 3 (Ln = Tm−Lu). The crystal structures of the hexaborates and…
Exposure of thin films of as-prepared single-walled carbon nanotubes (SWNT) to nitric acid induces dramatic bleaching of the first and second interband transitions of semiconducting tubes (S1 and S2). These near-IR absorption features can be restored by annealing of treated SWNT films to elevated temperatures. Anneali…
It is proved that a conducting channel transmitting perfectly without backscattering is present independent of energy in metallic carbon nanotubes for scatterers with potential range larger than the lattice constant. In the case that several traveling channels are present, the conductance decreases from the ideal valu…
Designable media can control properties of nanocomposite materials by spatially organizing nanoparticles. Here we theoretically study particle organization by ultrathin polymer films of grafted chains ("brushes"). Polymer-soluble nanoparticles smaller than a brush-determined threshold disperse in the film to a depth s…
A disk-shaped tridentate ligand 1 arranges silver(I) ions in a two-dimensional triangular and a three-dimensional tetrahedral fashion in the metal-ligand ratios, 3:2 and 1:1, respectively. The resulting sandwich-type (Ag312) and tetrahedral (Ag414) architectures are in a dynamic equilibrium in solution.
Successful treatment of cancer by boron neutron capture therapy (BNCT) requires the selective delivery of (10)B to constituent cells within a tumor. The expression of the folate receptor is amplified in a variety of human tumors and potentially might serve as a molecular target for BNCT. In the present study we have i…
Valence-band and conduction-band electronic structure of CrS (d=0) and Cr5S6 (d=0.17) has been investigated by means of photoemission and inverse-photoemission spectroscopies. Bandwidth of the valence bands of Cr5S6 (8.5 eV) is wider than that of CrS (8.1 eV), though the Cr 3d partial density of states evaluated from…
Total energy, binding energy, recombination rate (of the electron hole pair) for an exciton (X) bound in a parabolic two dimensional quantum dot by a donor impurity located on the z axis at a distance d from the dot plane, are calculated by using the Hartree formalism with a recently developed numerical method (PMM) f…