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Geometry Enhancement of Nanoscale Energy Deposition by X-rays

C. Lee、Neal Cheng、Rob Davidson 等 4 位作者2012-04-11The Journal of Physical Chemistry C

A theorem is established to show that nanoscale energy deposition in water by X-rays can be greatly enhanced via the geometry of nanostructures. The calculated results show that enhancement over background water can reach over 60 times for a single nanoshell made of gold. Other geometries and nanostructures are invest…

Graphene research and applicationsRadiation Therapy and DosimetryElectron and X-Ray Spectroscopy Techniques

Trapping of three-dimensional Holstein polarons by various impurities

Hadi Ebrahimnejad、Mona Berciu2012-04-11Physical Review B

We study the bound states of a three-dimensional Holstein polaron near various kinds of single impurities, using the momentum-average approximation. We show that the electron-phonon coupling is responsible for a strong renormalization of the impurity potential, resulting in an effective potential with significant reta…

Physics of Superconductivity and MagnetismQuantum and electron transport phenomenaMagnetic and transport properties of perovskites and related materials

PTFE–PMMA core–shell colloidal particles as building blocks for self‐assembled opals: synthesis, properties and optical response

Diego Antonioli、Simone Deregibus、Guido Panzarasa 等 11 位作者2012-04-11Polymer International

Abstract A seeded surfactant‐free methyl methacrylate emulsion polymerization is employed to prepare core–shell particles with predetermined size and narrow size distribution. The particle size is determined by the ratio between methyl methacrylate (MMA, shell) and polytetrafluoroethylene (PTFE, core). Monodisperse pa…

Quantum Dots Synthesis And PropertiesPhotonic Crystals and ApplicationsNonlinear Optical Materials Studies

Rainbow Radiating Single-Crystal Ag Nanowire Nanoantenna

Taejoon Kang、Wonjun Choi、Ilsun Yoon 等 7 位作者2012-04-11Nano Letters

Optical antennas interface an object with optical radiation and boost the absorption and emission of light by the objects through the antenna modes. It has been much desired to enhance both excitation and emission processes of the quantum emitters as well as to interface multiwavelength channels for many nano-optical…

Gold and Silver Nanoparticles Synthesis and ApplicationsPlasmonic and Surface Plasmon ResearchNear-Field Optical Microscopy

Controlled Modification of Protein-Repelling Self-Assembled Monolayers by Ultraviolet Light: The Effect of the Wavelength

Y.L. Jeyachandran、Andreas Terfort、Michael Zharnikov2012-04-11The Journal of Physical Chemistry C

Exposure of protein-repelling oligo(ethylene glycol) (OEG) terminated alkanethiolate (AT) monolayers to ultraviolet (UV) light results in the damage of the OEG chains and photooxidation of the thiolate headgroups, which can be used for controlled tuning of protein-repelling properties within the so-called UV direct wr…

Polymer Surface Interaction StudiesMolecular Junctions and NanostructuresNanofabrication and Lithography Techniques

Homopolar 2-Pole Radial Permanent-Magnet Biased Magnetic Bearing With Low Rotating Loss

Jiancheng Fang、Xi Wang、Tong Wei 等 5 位作者2012-04-11IEEE Transactions on Magnetics

To satisfy the low loss requirement of magnetically suspended rotors, such as energy-storage flywheel, a novel radial permanent-magnet biased magnetic bearing (RPMB) with low rotating loss due to low flux fluctuation frequency in rotor core called homopolar 2-pole RPMB was proposed. A rotating loss separation method w…

Electric Motor Design and AnalysisMagnetic Bearings and Levitation DynamicsMagnetic Properties of Alloys

Low-loss plasmonic metamaterial based on epitaxial gold monocrystal film

V.A. Fedotov、T. Uchino、Jun‐Yu Ou2012-04-11Optics Express

We demonstrate high-finesse plasmonic metamaterial with strong resonant response in the near-IR spectral range fabricated using a thin low-loss film of gold monocrystal. The monocrystal was grown using specially formulated simplified crystal growth procedure based on epitaxial deposition, which makes it readily access…

Gold and Silver Nanoparticles Synthesis and ApplicationsMetamaterials and Metasurfaces ApplicationsPlasmonic and Surface Plasmon Research

Analytic Theory of the Resonance Properties of Metallic Nanoslit Arrays

Jae Woong Yoon、Myoung Jin Jung、Seok Ho Song 等 4 位作者2012-04-11IEEE Journal of Quantum Electronics

By applying formulation based on time reversibility, we provide the analytic theory of resonance properties of metallic nanoslit arrays. We model lossy resonant systems in which a resonance is induced by a single quasi-bound mode (QBM). It is consistent with the Fano resonance theory of quantum interference of auto-io…

Gold and Silver Nanoparticles Synthesis and ApplicationsPlasmonic and Surface Plasmon ResearchPhotonic Crystals and Applications

Time-Resolved Photoinduced Thermoelectric and Transport Currents in GaAs Nanowires

Leonhard Prechtel、Milan Padilla、Nadine Erhard 等 7 位作者2012-04-11Nano Letters

In order to clarify the temporal interplay of the different photocurrent mechanisms occurring in single GaAs nanowire based circuits, we introduce an on-chip photocurrent pump-probe spectroscopy with a picosecond time resolution. We identify photoinduced thermoelectric, displacement, and carrier lifetime limited curre…

Advanced Thermoelectric Materials and DevicesAdvancements in Semiconductor Devices and Circuit DesignNanowire Synthesis and Applications

High-temperature nanoindentation behavior of Al/SiC multilayers

Saeid Lotfian、J.M. Molina-Aldareguía、Kyle Yazzie 等 5 位作者2012-04-11Philosophical Magazine Letters

Nanoscale Al/SiC composite laminates have unique properties, such as high strength, high toughness, and damage tolerance. In this article, the high-temperature nanoindentation response of Al/SiC nanolaminates is explored from room temperature up to 300°C. Selected nanoindentations were analyzed postmortem using focuse…

Advanced ceramic materials synthesisMetal and Thin Film MechanicsAluminum Alloys Composites Properties

Double-SOI Wafer-Bonded CMUTs With Improved Electrical Safety and Minimal Roughness of Dielectric and Electrode Surfaces

Peiyu Zhang、Glen Fitzpatrick、Tyler Harrison 等 5 位作者2012-04-11Journal of Microelectromechanical Systems

Despite myriad potential advantages over piezoelectric ultrasound transducers, capacitive micromachined ultrasound transducers (CMUTs) have not yet seen widespread commercial implementation. The possible reasons for this may include key issues of the following: (1) long-term device reliability and (2) electrical safet…

Ferroelectric and Piezoelectric MaterialsUltrasonics and Acoustic Wave PropagationElectrical and Bioimpedance Tomography

Heparan Sulfate Proteoglycan-Mediated Entry Pathway for Charged Tri-Platinum Compounds: Differential Cellular Accumulation Mechanisms for Platinum

Heveline Silva、Fréderic Frézard、Erica J. Peterson 等 6 位作者2012-04-11Molecular Pharmaceutics

We examined the mechanism of accumulation of charged polynuclear platinum complexes (PPCs) based on analogy of polyarginine interactions with the cell surface heparan sulfate proteoglycan (HSPG) family of protein-linked glycosoaminoglycan polysaccharides (GAGs). GAGS such as heparan sulfate (HS) and chondroitin sulfat…

RNA Interference and Gene DeliveryPolymer Surface Interaction StudiesDendrimers and Hyperbranched Polymers

Rhodanese Functions as Sulfur Supplier for Key Enzymes in Sulfur Energy Metabolism

Clément Aussignargues、Marie-Cécile Giuliani、Pascale Infossi 等 7 位作者2012-04-11Journal of Biological Chemistry

How microorganisms obtain energy is a challenging topic, and there have been numerous studies on the mechanisms involved. Here, we focus on the energy substrate traffic in the hyperthermophilic bacterium Aquifex aeolicus. This bacterium can use insoluble sulfur as an energy substrate and has an intricate sulfur energy…

Enzyme Structure and FunctionMetalloenzymes and iron-sulfur proteinsMicrobial Community Ecology and Physiology

Structure–Property Relationships of Inorganically Surface-Modified Zeolite Molecular Sieves for Nanocomposite Membrane Fabrication

Megan E. Lydon、Kinga A. Unocic、Tae‐Hyun Bae 等 5 位作者2012-04-11The Journal of Physical Chemistry C

A multiscale experimental study of the structural, compositional, and morphological characteristics of aluminosilicate (LTA) and pure-silica (MFI) zeolite materials surface-modified with MgO x H y nanostructures is presented. These characteristics are correlated with the suitability of such materials in the fabricatio…

Zeolite Catalysis and SynthesisMembrane Separation and Gas TransportCovalent Organic Framework Applications

Determination of the optical properties of La 2−x Ba x CuO 4 for several dopings, including the anomalous x=18 phase

C. C. Homes、M. Hücker、Q. Li 等 7 位作者2012-04-11Physical Review B

The optical properties of single crystals of the high-temperature superconductor La${}_{2\ensuremath{-}x}$Ba${}_{x}$CuO${}_{4}$ have been measured over a wide frequency and temperature range for light polarized in the a-b planes and along the $c$ axis. Three different Ba concentrations have been examined, $x=0.095$ wi…

Physics of Superconductivity and MagnetismMagnetic and transport properties of perovskites and related materialsAdvanced Condensed Matter Physics

Photoinduced Reactivity of Doxorubicin: Catalysis and Degradation

Krzysztof Nawara、Paweł Krysiński、G. J. Blanchard2012-04-11The Journal of Physical Chemistry A

Doxorubicin exhibits unusual photoreactivity in aqueous solutions. Our data show that there are two distinct photoreactive pathways for doxorubicin. One is a two-step process that leads to the formation of 3-methoxysalicylic acid, a stable degradation product. The other pathway is a photoreduction of doxorubicin to fo…

Porphyrin and Phthalocyanine ChemistryChemotherapy-induced cardiotoxicity and mitigationElectron Spin Resonance Studies

Mapping spin-polarized transitions with atomic resolution

P. Schattschneider、Bernhard Schaffer、Inga Ennen 等 4 位作者2012-04-11Physical Review B

The coupling of angstrom-sized electron probes with spin-polarized electronic transitions shows that the inelastically scattered probe electron is in a mixed state containing electron vortices with nonzero orbital angular momentum. These electrons create an asymmetric intensity distribution in energy filtered diffract…

Magnetic properties of thin filmsAdvanced Electron Microscopy Techniques and ApplicationsElectron and X-Ray Spectroscopy Techniques

Surface Click Reactions on Polymeric Nanocapsules for Versatile Functionalization

Grit Baier、Joerg Max Siebert、Katharina Landfester 等 4 位作者2012-04-11Macromolecules

One-step synthesis of poly(butyl cyanoacrylate- co -propargyl cyanoacrylate) (P(BCA/PCA)) and polyurethane (PUR) azide nanocapsules for direct covalent and variable functionalization is reported. The capsules in the size range between 230 and 350 nm were synthesized in an inverse (water-in-oil) miniemulsion system thr…

Polymer Surface Interaction StudiesMonoclonal and Polyclonal Antibodies ResearchClick Chemistry and Applications

Adsorption Behavior of Fe(II) and Fe(III) Ions on Thiourea Cross-Linked Chitosan with Fe(III) as Template

Jun Dai、Fenglian Ren、Chunyuan Tao2012-04-11Molecules

A new type of thiourea cross-linked chitosan with Fe(III) as template (TCCTS template) was synthesized. The adsorption of Fe(II) and Fe(III) on this TCCTS template was studied. The factors affecting adsorption such as pH and contact time were considered. The results showed that the optimum pH value for adsorption was…

Adsorption and biosorption for pollutant removalCovalent Organic Framework ApplicationsNanomaterials for catalytic reactions

Influence of Solvents and Surface Treatment on Photovoltaic Response of DSSC Based on Natural Curcumin Dye

C.O. Sreekala、I. Jinchu、K. S. Sreelatha 等 8 位作者2012-04-11IEEE Journal of Photovoltaics

Dye-sensitized solar cells have recently drawn much attention because of their cost effectiveness and easy manufacturing process. However, the challenge lies in minimizing the cost of sensitizer dyes and the platinum-based counter electrode. Natural dyes such as red cabbage, red perilla, rosella, blue pea, and curcumi…

TiO2 Photocatalysis and Solar CellsAdvanced Photocatalysis TechniquesConducting polymers and applications