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Coherent, Mechanical Control of a Single Electronic Spin

Sungkun Hong、Michael S. Grinolds、Patrick Maletinsky 等 6 位作者2012-07-16Nano Letters

We demonstrate coherent quantum control of a single spin driven by the motion of a mechanical resonator. The motion of a mechanical resonator is magnetically coupled to the electronic spin of a single nitrogen-vacancy center in diamond. Synchronization of spin-addressing protocols to the motion of the driven oscillato…

Diamond and Carbon-based Materials ResearchForce Microscopy Techniques and ApplicationsMechanical and Optical Resonators

Fast switchable grating based on orthogonal photo alignments of ferroelectric liquid crystals

Abhishek Kumar Srivastava、Wei Hu、Vladimir G. Chigrinov 等 5 位作者2012-07-16Applied Physics Letters

We demonstrate a fast switchable grating based on ferroelectric liquid crystals and orthogonal planar alignment by means of photo alignments. Both 1D and 2D gratings have been constructed. The proposed diffracting element provides fast response time of around 20 μs, contrast of 7000:1 and high diffraction efficiency,…

Photonic and Optical DevicesLiquid Crystal Research AdvancementsPhotorefractive and Nonlinear Optics

Controllable spin-glass behavior and large magnetocaloric effect in Gd-Ni-Al bulk metallic glasses

Fang Yuan、Juan Du、Baolong Shen2012-07-16Applied Physics Letters

Glass-forming ability, spin-glass (SG) behavior, and magnetocaloric effect in Gd55NixAl45-x (x = 15, 20, 25, 30) metallic alloys were investigated. A ferromagnetic SG behavior was observed for glassy ribbons with compositions of x = 15, 20, and 25, but it disappeared for that of x = 30. Furthermore, the maximum magnet…

Theoretical and Computational PhysicsMagnetic and transport properties of perovskites and related materialsMetallic Glasses and Amorphous Alloys

Modeling of a vertical tunneling graphene heterojunction field-effect transistor

S. Bala Kumar、Gyungseon Seol、Jing Guo2012-07-16Applied Physics Letters

Vertical tunneling field-effect-transistor (FET) based on graphene heterojunctions with layers of hBN is simulated by self-consistent quantum transport simulations. It is found that the asymmetric p-type and n-type conduction is due to work function difference between the graphene contact and the tunneling channel mat…

Graphene research and applicationsDiamond and Carbon-based Materials ResearchAdvancements in Semiconductor Devices and Circuit Design

Insertion of Short Amino-Functionalized Single-Walled Carbon Nanotubes into Phospholipid Bilayer Occurs by Passive Diffusion

Sebastian Kraszewski、Alberto Bianco、Mounir Tarek 等 4 位作者2012-07-16PLoS ONE

Carbon nanotubes have been proposed to be efficient nanovectors able to deliver genetic or therapeutic cargo into living cells. However, a direct evidence of the molecular mechanism of their translocation across cell membranes is still needed. Here, we report on an extensive computational study of short (5 nm length)…

Carbon Nanotubes in CompositesLipid Membrane Structure and BehaviorNanopore and Nanochannel Transport Studies

The Vital Role of Buffer Anions in the Antioxidant Activity of CeO2 Nanoparticles

Ying Xue、Yanwu Zhai、Kebin Zhou 等 7 位作者2012-07-16Chemistry - A European Journal

Cerium oxide (CeO(2)) nanoparticles display excellent antioxidant properties by scavenging free radicals. However, some studies have indicated that they can cause an adverse response by generating reactive oxygen species (ROS). Hence, it is important to clarify the factors that affect the oxidant/antioxidant activitie…

Nanoparticles: synthesis and applicationsCarbon and Quantum Dots ApplicationsAdvanced Nanomaterials in Catalysis

High-Resolution Calorimetric Study of Pb(Mg1/3Nb2/3)O3 Single Crystal

Nikola Novak、Raša Pirc、Magdalena Wencka 等 4 位作者2012-07-16Physical Review Letters

Motivated by the long-standing unresolved enigma of the relaxor ferroelectric ground state, we performed a high-resolution heat capacity and polarization study of the field-induced phase transition in the relaxor ferroelectric single crystal Pb(Mg(1/3)Nb(2/3))O3 (PMN) oriented along the [110] direction. We show that t…

Ferroelectric and Piezoelectric MaterialsMultiferroics and related materialsMicrowave Dielectric Ceramics Synthesis

Structure and Bonding in Copper(I) Carbonyl and Cyanide Complexes

Robert D. Pike2012-07-16Organometallics

The coordination chemistry of copper(I) carbonyls and cyano complexes is reviewed. Primary attention is focused on structural chemistry, including coordination behavior, bridging modes, network formation, flexible coordination number, and reversible ligand binding. Additional coverage of infrared spectroscopy and orbi…

Metal-Organic Frameworks: Synthesis and ApplicationsMetal complexes synthesis and propertiesMagnetism in coordination complexes

Reduction of persistent photoconductivity in ZnO thin film transistor-based UV photodetector

Pavel Ivanoff Reyes、Chieh-Jen Ku、Ziqing Duan 等 6 位作者2012-07-16Applied Physics Letters

We report a ZnO-based thin film transistor UV photodetector with a back gate configuration. The thin-film transistor (TFT) aspect ratio W/L is 150 μm/5 μm and has a current on-off ratio of 1010. The detector shows UV-visible rejection ratio of 104 and cut-off wavelength of 376 nm. The device has low dark current of 5…

ZnO doping and propertiesThin-Film Transistor TechnologiesGa2O3 and related materials

Nickel Catalysts Supported on Barium Hexaaluminate for Enhanced CO Methanation

Jiajian Gao、Chunmiao Jia、Jing Li 等 7 位作者2012-07-16Industrial & Engineering Chemistry Research

We report the preparation and characterization of Ni nanoparticles supported on barium hexaaluminate (BHA) as CO methanation catalysts for the production of synthetic natural gas (SNG). BHA with a high thermal stability was synthesized by a coprecipitation method using aluminum nitrate, barium nitrate, and ammonium ca…

Catalytic Processes in Materials ScienceCatalysts for Methane ReformingCatalysis and Oxidation Reactions

Aggregation and Stabilization of Carboxylic Acid Functionalized Halloysite Nanotubes (HNT-COOH)

Yongho Joo、Yangjun Jeon、Sang Uck Lee 等 8 位作者2012-07-16The Journal of Physical Chemistry C

We modified the functional groups of holloysite nanotubes (HNT) from hydroxyl groups (HNT-OH) to carboxylic acids (HNT-COOH). Aggregation and dispersion properties of HNT-COOH under dry conditions were probed by scanning electron microscopy (SEM) and atomic force microscopy (AFM). Moreover, the degree of aggregation a…

Clay minerals and soil interactionsIron oxide chemistry and applicationsLayered Double Hydroxides Synthesis and Applications

Very high thermoelectric power factor in a Fe3O4/SiO2/p-type Si(100) heterostructure

Z. Viskadourakis、M. L. Paramês、O. Conde 等 5 位作者2012-07-16Applied Physics Letters

The thermoelectric and transport properties of a Fe3O4/SiO2/p-Si(100) heterostructure have been investigated between 100 and 300 K. Both Hall and Seebeck coefficients change sign from negative to positive with increasing temperature while the resistivity drops sharply due to tunneling of carriers into the p-Si(100). T…

Semiconductor materials and interfacesHeusler alloys: electronic and magnetic propertiesSurface and Thin Film Phenomena

Probing the three-dimensional strain inhomogeneity and equilibrium elastic properties of single crystal Ni nanowires

Edwin Fohtung、Jong Woo Kim、Keith Chan 等 6 位作者2012-07-16Applied Physics Letters

We employ three dimensional x-ray coherent diffraction imaging to map the lattice strain distribution, and to probe the elastic properties of a single crystalline Ni (001) nanowire grown vertically on an amorphous SiO2∥Si substrate. The reconstructed density maps show that with increasing wire width, the equilibrium c…

Microstructure and mechanical propertiesAdvanced Electron Microscopy Techniques and ApplicationsForce Microscopy Techniques and Applications

Remarkably high-temperature stable piezoelectric properties of Bi(Mg0.5Ti0.5)O3 modified BiFeO3–BaTiO3 ceramics

Changrong Zhou、Antonio Feteira、Xu Shan 等 8 位作者2012-07-16Applied Physics Letters

Dense (1-x)BiFe1-x(Mg0.5Ti0.5)xO3–yBaTiO3 (BFMT-BT, y=0.29, x=0-0.12) ceramics with a pseudocubic perovskite crystal structure exhibit remarkably high-temperature stable piezoelectric properties. In particular, x=0.03 BFMT-BT ceramics, with a Curie temperature, Tc, of ~425C, show a stable piezoelectric coefficient, d…

Ferroelectric and Piezoelectric MaterialsMultiferroics and related materialsDielectric properties of ceramics

Ultrafast Photoinduced Charge Separation in Metal–Semiconductor Nanohybrids

Denis Mongin、Ehud Shaviv、Paolo Maioli 等 7 位作者2012-07-16ACS Nano

Hybrid nano-objects formed by two or more disparate materials are among the most promising and versatile nanosystems. A key parameter in their properties is interaction between their components. In this context we have investigated ultrafast charge separation in semiconductor-metal nanohybrids using a model system of…

Gold and Silver Nanoparticles Synthesis and ApplicationsQuantum Dots Synthesis And PropertiesCopper-based nanomaterials and applications

Critical influence of target-to-substrate distance on conductive properties of LaGaO3/SrTiO3 interfaces deposited at 10−1 mbar oxygen pressure

C. Aruta、S. Amoruso、G. Ausanio 等 11 位作者2012-07-16Applied Physics Letters

We investigate pulsed laser deposition of LaGaO3/SrTiO3 at 10−1 mbar oxygen background pressure, demonstrating the critical effect of the target-to-substrate distance, dTS, on the interface sheet resistance, Rs. The interface turns from insulating to metallic by progressively decreasing dTS. The analysis of the LaGaO3…

Semiconductor materials and devicesMagnetic and transport properties of perovskites and related materialsElectronic and Structural Properties of Oxides

Excitation Dynamics in Low Band Gap Donor–Acceptor Copolymers and Blends

Björn Gieseking、Berthold Jäck、Eduard Preis 等 8 位作者2012-07-16Advanced Energy Materials

Abstract Donor–acceptor (D–A) type copolymers show great potential for the application in the active layer of organic solar cells. Nevertheless the nature of the excited states, the coupling mechanism and the relaxation pathways following photoexcitation are yet to be clarified. We carried out comparative measurements…

Organic Electronics and PhotovoltaicsPerovskite Materials and ApplicationsConducting polymers and applications

First-principles study of magnetism in Pd 3 Fe under pressure

Biswanath Dutta、Sumanta Bhandary、Subhradip Ghosh 等 4 位作者2012-07-16Physical Review B

Recent experiments on Pd${}_{3}$Fe intermetallics [M. L. Winterrose et al., Phys. Rev. Lett. 102, 237202 (2009)] have revealed that the system behaves like a classical invar alloy under high pressure. The experimental pressure-volume relation suggests an anomalous volume collapse and a substantial increase in bulk mod…

Magnetic properties of thin filmsRare-earth and actinide compoundsMagnetic Properties of Alloys

Bound state in continuum like solutions in one-dimensional hetero-structures

O. Panella、P. Roy2012-07-16arXiv

We examine the one dimensional Dirac equation with modulated or position dependent velocity. In particular, it is shown that using suitable velocity profiles it is possible to create bound state in continuum (BIC) like, as well as, discrete energy bound state solutions.

Materials Sciencehep-thmath-phmath.MPquant-ph

Weak localization and antilocalization in topological insulator thin films with coherent bulk-surface coupling

Ion Garate、Leonid Glazman2012-07-16Physical Review B

We evaluate quantum corrections to conductivity in an electrically gated thin film of a three-dimensional topological insulator. We derive approximate analytical expressions for the low-field magnetoresistance as a function of bulk doping and bulk-surface tunneling rate. Our results reveal parameter regimes for both w…

Graphene research and applicationsTopological Materials and PhenomenaQuantum many-body systems