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Crystal Structures of Branched-Chain Amino Acid Aminotransferase Complexed with Glutamate and Glutarate: True Reaction Intermediate and Double Substrate Recognition of the Enzyme,

Masaru Goto、I. Miyahara、Hideyuki Hayashi 等 5 位作者2003-03-15Biochemistry

Branched-chain amino acid aminotransferase (BCAT), which has pyridoxal 5'-phosphate as a cofactor, is a key enzyme in the biosynthetic pathway of hydrophobic amino acids (leucine, isoleucine, and valine). The enzyme reversibly catalyzes the transfer of the amino group of a hydrophobic amino acid to 2-oxoglutarate to f…

RNA and protein synthesis mechanismsEnzyme Structure and FunctionProtein Structure and Dynamics

Newtonian Flow Behavior of Hyperbranched High-Molecular-Weight Polyethylenes Produced with a Pd−Diimine Catalyst and Its Dependence on Chain Topology

Zhibin Ye、Shiping Zhu2003-03-15Macromolecules

ADVERTISEMENT RETURN TO ISSUEPREVCommunication to the...Communication to the EditorNEXTNewtonian Flow Behavior of Hyperbranched High-Molecular-Weight Polyethylenes Produced with a Pd−Diimine Catalyst and Its Dependence on Chain TopologyZhibin Ye and Shiping ZhuView Author Information Department of Chemical Engineering…

Dendrimers and Hyperbranched PolymersPolymer Surface Interaction StudiesSynthetic Organic Chemistry Methods

Synthesis and Protonation Behavior of Comblike Poly(ethyleneimine)

Ger J. M. Koper、René C. van Duijvenbode、Danny Stam 等 5 位作者2003-03-15Macromolecules

Comblike poly(ethyleneimine) (PEI) with −(CH 2 CH 2 )N(CH 2 CH 2 NH 2 )− as the repeating unit has been synthesized by employing a protecting group strategy, and analyzed by potentiometric titration. If the degree of protonation is plotted as a function of pH, the titration curve shows three protonation steps separate…

Fuel Cells and Related MaterialsAdvanced Polymer Synthesis and CharacterizationDendrimers and Hyperbranched Polymers

Dynamic Recrystallization Based on Twinning in Coarse-Grained Mg

Oleg Sitdikov、Rustam Kaibyshev、Taku Sakai2003-03-15Materials science forum

Mechanism of dinamic recrystallization (DRX) associated with twinning are proposed and discussed on the results of microstructure evolution during warm and hot deformation of a coarse-grained Mg

Magnesium Alloys: Properties and ApplicationsMicrostructure and mechanical propertiesMetallurgy and Material Forming

Dissolution of Bombyx mori Silk Fibroin in the Calcium Nitrate Tetrahydrate−Methanol System and Aspects of Wet Spinning of Fibroin Solution

Sung-Won Ha、Young H. Park、Samuel M. Hudson2003-03-15Biomacromolecules

There are still several problems associated with the spinning of dialyzed silk fibroin solutions. In this work some of these problems have been examined. The calcium nitrate tetrahydrate-methanol system was used to dissolve the silk fibroin. A compositional phase diagram was constructed at various concentrations of th…

Surface Modification and SuperhydrophobicitySilk-based biomaterials and applicationsSilkworms and Sericulture Research

A procedure for setting up high-throughput nanolitre crystallization experiments. II. Crystallization results

James Brown、Thomas S. Walter、L. Carter 等 34 位作者2003-03-15Journal of Applied Crystallography

An initial tranche of results from day-to-day use of a robotic system for setting up 100 nl-scale vapour-diffusion sitting-drop protein crystallizations has been surveyed. The database of over 50 unrelated samples represents a snapshot of projects currently at the stage of crystallization trials in Oxford research gro…

Protein purification and stabilityEnzyme Structure and FunctionProtein Structure and Dynamics

Amphiphobic Carbon Nanotubes as Macroemulsion Surfactants

Howard Wang、Erik K. Hobbie2003-03-15Langmuir

Single-walled carbon nanotubes (SWNTs) are insoluble in either water or oil. When mixtures of SWNTs, water, and toluene are sheared vigorously, a macroscopic emulsion of water droplets forms in toluene, with the SWNTs residing at the interface between the immiscible fluids, acting as a natural “surfactant” or interpha…

Pickering emulsions and particle stabilizationSurface Modification and SuperhydrophobicityCarbon Nanotubes in Composites

Superconductivity at 14.2 K in Layered Organics under Extreme Pressure

Hiromi Taniguchi、M. Miyashita、Kenichi Uchiyama 等 10 位作者2003-03-15Journal of the Physical Society of Japan

We demonstrate that an organic Mott insulator, β'-(BEDT-TTF) 2 ICl 2 , is metallized by application of extremely high pressure by means of the cubic anvil press. When the metallic state is stabilized, superconductivity with the highest transition-temperature ( T c ) among the organic systems appears. The lower limit o…

Rare-earth and actinide compoundsOrganic and Molecular Conductors ResearchMagnetism in coordination complexes

On the Mechanism of Ion Transport through Polyphosphazene Solid Polymer Electrolytes: NMR, IR, and Raman Spectroscopic Studies and Computational Analysis of 15N-Labeled Polyphosphazenes

Thomas A. Luther、Frederick F. Stewart、Joanne Budzien 等 8 位作者2003-03-15The Journal of Physical Chemistry B

Comprehensive investigation of lithium ion complexation with 15 N-labeled polyphosphazenes 15 N -poly[bis(2-(2-methoxyethoxy)ethoxy)phosphazene] ( 15 N -MEEP) and 15 N -poly-[((2-allylphenoxy) 0.12 (4-methoxyphenoxy) 1.02 (2-(2-methoxyethoxy)ethoxy) 0.86 )phosphazene] ( 15 N -HPP) was performed by NMR, IR, and Raman s…

Advanced Battery Materials and TechnologiesFlame retardant materials and propertiesPolymer crystallization and properties

Analysis of the small-angle intensity scattered by a porous and granular medium

Olivier Spalla、Sandrine Lyonnard、Fabienne Testard2003-03-15Journal of Applied Crystallography

Using X-ray scattering over a large range of scattering vectors, it is shown how to measure both the pore volume fraction and pore specific surface of an assembly of porous grains forming a powder. Depending on the presence or not of solvent in the inner pores and in the intergranular media, the scattered signal per u…

X-ray Diffraction in CrystallographyCultural Heritage Materials AnalysisRadiation Shielding Materials Analysis

Carrier States and Ferromagnetism in Diluted Magnetic Semiconductors

Masao Takahashi、Kenn Kubo2003-03-15arXiv

Applying the dynamical coherent potential approximation to a simple model, we have systematically studied the carrier states in $A_{1-x}$Mn$_xB$-type diluted magnetic semiconductors (DMS's). The model calculation was performed for three typical cases of DMS's: The cases with strong and moderate exchange interactions i…

Materials Science

Triangular Nanoframes Made of Gold and Silver

Gabriella S. Métraux、Y. Charles Cao、Rongchao Jin 等 4 位作者2003-03-15OpenAlex

Silver nanoprisms (∼74-nm edge length) were etched with HAuCl 4 to generate gold−silver alloy framework structures. Interestingly, these triangular nanoframes possess no strong surface plasmon bands in the ultraviolet or visible regions of the optical spectrum. By adding a mild reducing agent, l -ascorbic acid, gold a…

Nanoporous metals and alloysGold and Silver Nanoparticles Synthesis and ApplicationsPlasmonic and Surface Plasmon Research

X-Cell: a novel indexing algorithm for routine tasks and difficult cases

Marcus A. Neumann2003-03-15OpenAlex

X-Cell is a novel indexing algorithm that makes explicit use of systematic absences to search for possible indexing solutions from cells with low numbers of calculated reflections to cells with high numbers of reflections. Space groups with the same pattern of systematic absences are grouped together in powder extinct…

Crystallography and molecular interactionsMachine Learning in Materials ScienceX-ray Diffraction in Crystallography

Ab Initio Study of Doped Carbon Nanotube Sensors

Shu Peng、Kyeongjae Cho2003-03-15OpenAlex

Recently great advances have been made in demonstrating the viability of using carbon nanotubes (CNTs) to detect the presence of chemical gases such as NO 2, NH 3, and O 2, and they have led to the design of a new breed of sensor devices. Based on intrinsic CNTs, the devices are capable of detecting small concentratio…

Nanopore and Nanochannel Transport StudiesCarbon Nanotubes in CompositesMechanical and Optical Resonators

Green Emission to Probe Photoinduced Charging Events in ZnO−Au Nanoparticles. Charge Distribution and Fermi-Level Equilibration

Vaidyanathan Subramanian、Eduardo E. Wolf、Prashant V. Kamat2003-03-15OpenAlex

Photoinduced electron accumulation in ZnO nanoparticles results in the bleaching of the exciton band as well as quenching of green emission. In the absence of an electron scavenger, photogenerated electrons are stored near the conduction band edge and promote charge recombination via a nonradiative process. By exposin…

Quantum Dots Synthesis And PropertiesCopper-based nanomaterials and applicationsZnO doping and properties

Mussel Adhesive Protein Mimetic Polymers for the Preparation of Nonfouling Surfaces

Jeffrey L. Dalsin、Bi−Huang Hu、Bruce P. Lee 等 4 位作者2003-03-15OpenAlex

A new biomimetic strategy for modification of biomaterial surfaces with poly(ethylene glycol) (PEG) was developed. The strategy exploits the adhesive characteristics of 3,4-dihydroxyphenylalanine (DOPA), an important component of mussel adhesive proteins, to anchor PEG onto surfaces, rendering the surfaces resistant t…

Marine Biology and Environmental ChemistryPolymer Surface Interaction StudiesKnee injuries and reconstruction techniques

An intensity evaluation method:EVAL-14

A. J. M. Duisenberg、Loes M. J. Kroon-Batenburg、A.M.M. Schreurs2003-03-15OpenAlex

A reflection intensity integration method is presented based upon ab initio calculation of three-dimensional ( x , y , ω) reflection boundaries from a few physical crystal and instrument parameters. It is especially useful in challenging circumstances, such as the case of a crystal that is far from spherical, anisotro…

Solid-state spectroscopy and crystallographyAcoustic Wave Resonator TechnologiesX-ray Diffraction in Crystallography

Liquid-crystalline metallophthalocyanines containing late first-row transition metals

Jurgen Sleven、Thomas Cardinaels、Christiane Görller‐Walrand 等 4 位作者2003-03-14ARKIVOC

Cobalt(II), nickel(II), copper(II) and zinc(II) phthalocyanines substituted by eight alkoxy chains in the peripheral (2,3,9,10,16,17,23,24) positions were prepared. The alkoxy chain lengths are octyloxy (C 8 H 17 O), dodecyloxy (C 12 H 25 O) and hexadecyloxy (C 16 H 33 O). Studies by polarized optical microscopy and h…

Magnetism in coordination complexesPorphyrin and Phthalocyanine ChemistryPhotochemistry and Electron Transfer Studies

Diffusion-Corrected Simultaneous Multilayer Growth Model

Qiang Fu、Thomas Wagner2003-03-14Physical Review Letters

A diffusion-corrected simultaneous multilayer (DCSM) model was developed, taking into account up-step and down-step diffusion of adatoms and enabling rapid identification of different film growth modes. This DCSM model was applied to the initial growth of Cr on (100) ${\mathrm{S}\mathrm{r}\mathrm{T}\mathrm{i}\mathrm{O…

Electron and X-Ray Spectroscopy TechniquesSemiconductor materials and devicesSurface and Thin Film Phenomena