Materials Literature
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Antimony-doped p-type ZnO films epitaxially grown on (0001) sapphire substrates were fabricated by pulsed laser deposition at 400–600°C in 5.0×10−2Torr oxygen without postdeposition annealing. The films grown at 600°C have among the highest reported hole concentration of 1.9×1017cm−3 for antimony doping, Hall mobility…
Hybrid vesicles: Magnetic nanoparticles (γ-Fe2O3) and quantum dots (CdSe/ZnS) can be entrapped in stable vesicles by emulsion processes. The hybrid vesicles (HVs) have distinct magnetic and fluorescence properties (see images; scale bars: 10 μm). Fluorescence detection allows magnetic manipulation and tracking of the…
V-doped ZnO films have been prepared on Si(111) substrates by direct current reactive magnetron cosputtering. Hysteresis loops of polarization–applied field characteristics with a remnant polarization of 0.2μC∕cm2 were obtained in (2.5at.%) V-doped ZnO films, indicating the ferroelectric behavior exists in this system…
Thin films of 5% Co-doped ZnO with a range of Al codoping exhibit a band-edge shift, which varies with carrier concentration as n2∕3. Carrier effective mass is 0.26me and mobility is ∼10cm2V−1s−1. The doped films, which contain coherent Co clusters of 4–8nm in size, exhibit a ferromagnetic moment of 0.3–1.0μB per coba…
Abstract In this study, flame retardancy properties of fabrics treated with phosphorous (P) doped and undoped SiO 2 thin films were developed by sol–gel technique. As to this aim, P‐doped and undoped SiO 2 film were coated on cotton fabric from the solutions prepared from P, Si‐based precursors, solvent, and chelating…
Abstract A “green” processing method, dual‐melt extrusion, was used to prepare thermoplastic starch/montmorillonite nanocomposites without organic reactions in the solution. XRD demonstrates that sorbitol enlarged the interlayer distance of MMT during the first step. MMT‐sorbitol, formamide and starch were used to obt…
The phenomenology of the laboratory glass transition is examined in the enthalpy landscape framework. It is shown that a generic description of the glassy state based on partitioning of the phase space caused by the finiteness of the time of observation explains all universal features of glass transition. Using this d…
A method to generate any liquid crystal pretilt angle is proposed and demonstrated. This method is based on deep ultraviolet photoalignment of a layer consisting of nanostructured domains of horizontal and vertical alignment polyimides. Competition between the two types of domains produces the controlled pretilt angle…
Large-area and aligned copper oxide nanowires have been synthesized by thermal annealing of copper thin films deposited onto silicon substrate. The effects of the film deposition method, annealing temperature, film thickness, annealing gas, and patterning by photolithography are systematically investigated. Long and a…
“Very minute in their dimensions” is how Faraday described the metal particles present in a fine dispersion of colloidal gold upon observing its interaction with red light 150 years ago (see picture for a laser-light version of his experiment). This observation would come to serve as the basis for the modern nanoscien…
In low temperature scanning tunneling microscopy (STM) experiments a cerium adatom on Ag(100) possesses two discrete states with significantly different apparent heights. These atomic switches also exhibit a Kondo-like feature in spectroscopy experiments. By extensive theoretical simulations we find that this behavior…
The authors explore computationally the formation of trilayer superlattices as an alternative approach to combining ferroelectricity with magnetism to form magnetoelectric multiferroics. It is found that the contribution to the superlattice polarization from trilayering is small compared to typical polarizations in co…
The authors report on the electrical and ultraviolet (UV) photoresponse properties of quasialigned ZnO nanowires (NWs)∕p-Si heterojunction grown by a low-temperature solvothermal technique. The current-voltage characteristic of a single ZnO NW∕p-Si junction measured by a scanning tunneling microscope shows a rectifyin…
We present an extension of the continuous damage fiber bundle model to describe the gradual degradation of highly heterogeneous materials under an increasing external load. Breaking of a fiber in the model is preceded by a sequence of partial failure events occurring at random threshold values. In order to capture the…
Bi 1 − x A x Fe O 3 ceramics (A=Ca,Sr,Pb) were sintered by conventional mixed oxide route. The crystallographic structure of all samples is characterized by the rhombohedral symmetry (space group R3c). The existence of switchable ferroelectric polarization is verified by piezoresponse force microscopy that is proven t…
We demonstrate the accuracy of the hypernetted chain closure and of the mean-field approximation for the calculation of the fluid-state properties of systems interacting by means of bounded and positive pair potentials with oscillating Fourier transforms. Subsequently, we prove the validity of a bilinear, random-phase…
We propose a new, cyclic-voltammetry based experimental technique that can not only differentiate between discontinuous and continuous phase transitions in an adsorbate layer, but also quite accurately recover equilibrium behavior from dynamic analysis of systems with a continuous phase transition. The Electrochemical…
We have performed {\it ab-initio} electronic structure calculations to determine the evolution of the electronic structure of WO$_3$ with Na doping. Na doping introduces an additional electron when introduced into WO$_3$. The ensuing electronic structure of Na doped WO$_3$, we find, is very similar to the electronic s…
A layered iron oxide \rfeo ($R$: rare-earth elements) is an exotic dielectric material with charge-order (CO) driven electric polarization and magnetoelectric effect caused by spin-charge coupling. In this paper, a theory of electronic structure and dielectric property in \rfeo is presented. Charge frustration in pair…
Li Nb O 3 -doped (Na,K)NbO3 lead-free piezoelectric ceramics were prepared by normal sintering, and the electrical properties were investigated with a special emphasis on the influence of sintering temperature. The ceramics synthesized at 1020–1080°C showed a phase transition from orthorhombic to tetragonal symmetry,…