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1/∞[ZrPSe6−]: A Soluble Photoluminescent Inorganic Polymer and Strong Second Harmonic Generation Response of Its Alkali Salts

Santanu Banerjee、Christos D. Malliakas、Joon I. Jang 等 5 位作者2008-08-21Journal of the American Chemical Society

Zirconium selenophosphate compounds with a unique polar structure show strong second harmonic generation and they dissolve in polar solvent to produce photoluminescent solutions.

Organometallic Compounds Synthesis and CharacterizationNonlinear Optical Materials ResearchCrystal Structures and Properties

Combined effects of crystallographic orientation, stacking fault energy and grain size on deformation twinning in fcc crystals

Wei‐Zhong Han、Z. F. Zhang、S.D. Wu 等 4 位作者2008-08-21The Philosophical Magazine A Journal of Theoretical Experimental and Applied Physics

The combined effects of crystallographic orientation, stacking fault energy (SFE) and grain size on deformation twinning behavior in several face-centred cubic (fcc) crystals were investigated experimentally and analytically. Three types of fcc crystals, Al single crystals, Cu single crystals and polycrystalline Cu–3%…

Aluminum Alloys Composites PropertiesMagnesium Alloys: Properties and ApplicationsMicrostructure and mechanical properties

Magnetic order of the iron spins in NdFeAsO

Ying Chen、J. W. Lynn、Jian Li 等 10 位作者2008-08-21Physical Review B

Polarized and unpolarized neutron-diffraction measurements have been carried out to investigate the iron magnetic order in undoped NdFeAsO. Antiferromagnetic order is observed below 141(6) K, which is in close proximity to the structural distortion observed in this material. The magnetic structure consists of chains o…

Physics of Superconductivity and MagnetismIron-based superconductors researchRare-earth and actinide compounds

Chiral Recognition of Amino Acids Based on Cyclodextrin‐Capped Quantum Dots

Cuiping Han、Haibing Li2008-08-21Small

Water-soluble and stable semiconductor CdSe/ZnS quantum dots (QDs) are prepared by using β- and α-cyclodextrin (CD) as surface-coating agents by using a simple sonochemical method, which allows highly enantioselective fluorescent recognition of amino acids (see image). When CD-QDs are treated with L-amino acids (see i…

Molecular Sensors and Ion DetectionQuantum Dots Synthesis And PropertiesAdvanced biosensing and bioanalysis techniques

Magneto-Optical-Trap-Based, High Brightness Ion Source for Use as a Nanoscale Probe

James Hanssen、Shannon B. Hill、Jon Orloff 等 4 位作者2008-08-21Nano Letters

We report on the demonstration of a low emittance, high brightness ion source based on magneto-optically trapped neutral atoms. Our source has ion optical properties comparable to or better than those of the commonly used liquid metal ion source. In addition, it has several advantages that offer new possibilities, inc…

Diamond and Carbon-based Materials ResearchForce Microscopy Techniques and ApplicationsCold Atom Physics and Bose-Einstein Condensates

Fermi surfaces of single layer dielectrics on transition metals

T. Greber、M. Corso、J. Osterwalder2008-08-21arXiv

Single sheets of hexagonal boron nitride on transition metals provide a model system for single layer dielectrics. The progress in the understanding of h-BN layers on transition metals of the last 10 years are shortly reviewed. Particular emphasis lies on the boron nitride nanomesh on Rh(111), which is a corrugated si…

Materials Science

Solvent-Free Synthesis of Janus Colloidal Particles

Shan Jiang、Mitchell J. Schultz、Qian Chen 等 5 位作者2008-08-21Langmuir

Taking advantage of the quick and efficient access of vapor to surfaces, a simple, solvent-free method is demonstrated to synthesize Janus colloidal particles in large quantity and with high efficiency. First, at the liquid-liquid interface of emulsified molten wax and water, untreated silica particles adsorb and are…

Proteins in Food SystemsPickering emulsions and particle stabilizationSurfactants and Colloidal Systems

Quantum Clusters of Gold Exhibiting FRET

Madathumpady Abubaker Habeeb Muhammed、Ajay Kumar Shaw、Samir Kumar Pal 等 4 位作者2008-08-21The Journal of Physical Chemistry C

Fluorescence resonance energy transfer between the metal core and the ligand in Au 25 SG 18 (SG-glutathione thiolate) is demonstrated using dansyl chromophores attached to the cluster core through glutathione linkers. The dansyl chromophore functionalization of the cluster has been carried out by two different routes.…

Advanced Nanomaterials in CatalysisNanocluster Synthesis and ApplicationsPharmacological Effects and Toxicity Studies

Direct Observation of Dark Excitons in Individual Carbon Nanotubes: Inhomogeneity in the Exchange Splitting

Ajit Srivastava、Han Htoon、Victor I. Klimov 等 4 位作者2008-08-21Physical Review Letters

We report the direct observation of spin-singlet dark excitons in individual single-walled carbon nanotubes through low-temperature micro-magneto-photoluminescence spectroscopy. A magnetic field (B) applied along the tube axis brightened the dark state, leading to the emergence of a new emission peak. The peak rapidly…

Quantum and electron transport phenomenaMechanical and Optical ResonatorsCarbon Nanotubes in Composites

Switching magnetic vortex core by a single nanosecond current pulse

Keisuke Yamada、Shinya Kasai、Yoshinobu Nakatani 等 5 位作者2008-08-21arXiv

In a ferromagnetic nanodisk, the magnetization tends to swirl around in the plane of the disk and can point either up or down at the center of this magnetic vortex. This binary state can be useful for information storage. It is demonstrated that a single nanosecond current pulse can switch the core polarity. This meth…

cond-mat.otherMaterials Science

Electrons and holes in Si quantum well: a room-temperature transport and drag resistance study

M. Prunnila、S. J. Laakso、J. M. Kivioja 等 4 位作者2008-08-21arXiv

We investigate carrier transport in a single 22 nm-thick double-gated Si quantum well device, which has independent contacts to electrons and holes. Conductance, Hall density and Hall mobility are mapped in a broad double-gate voltage window. When the gate voltage asymmetry is not too large only either electrons or ho…

Materials Sciencecond-mat.dis-nn

Scattering of phonons on two-level systems in disordered crystals

Dragoş-Victor Anghel、Dmitry Churochkin2008-08-21arXiv

We calculate the scattering rates of phonons on two-level systems in disordered trigonal and hexagonal crystals. We apply a model in which the two-level system, characterized by a direction in space, is coupled to the strain field of the phonon via a tensor of coupling constants. The structure of the tensor of couplin…

cond-mat.dis-nnMaterials Science

One-, Two-, and Three-Dimensional Arrays of Eu 3+ -4,4,5,5,5-pentafluoro-1-(naphthalen-2-yl)pentane-1,3-dione complexes: Synthesis, Crystal Structure and Photophysical Properties

D. B. Ambili Raj、S. Biju、M. L. P. Reddy2008-08-21Inorganic Chemistry

A novel beta-diketone, 4,4,5,5,5-pentafluoro-1-(naphthalen-2-yl)pentane-1,3-dione (HPFNP), which contains polyfluorinated alkyl group, as well as the long conjugated naphthyl group, has been used for the synthesis of a series of new tris(beta-diketonate)europium(III) complexes of the general formula Eu(PFNP)3 x L [whe…

Lanthanide and Transition Metal ComplexesRadioactive element chemistry and processingMagnetism in coordination complexes

Uptake of Colloidal Polyelectrolyte‐Coated Particles and Polyelectrolyte Multilayer Capsules by Living Cells

Almudena Muñoz Javier、Oliver Kreft、Maximilian Semmling 等 13 位作者2008-08-21Advanced Materials

Rigid particles as well as soft capsules can be ingested by cells and stored in acidic compartments around the nucleus. TEM and fluorescence images show that the rigid particles retain their original spherical shape whereas the hollow and thus more flexible capsules are deformed and squeezed upon the incorporation pro…

Polymer Surface Interaction StudiesDendrimers and Hyperbranched PolymersNanoparticle-Based Drug Delivery

Electronic structure and nesting-driven enhancement of the RKKY interaction at the magnetic ordering propagation vector in Gd2PdSi3 and Tb2PdSi3

D. S. Inosov、D. V. Evtushinsky、A. Koitzsch 等 15 位作者2008-08-21arXiv

We present first-time measurements of the Fermi surface and low-energy electronic structure of intermetallic compounds Gd2PdSi3 and Tb2PdSi3 by means of angle-resolved photoelectron spectroscopy (ARPES). Both materials possess a flower-like Fermi surface consisting of an electron barrel at the G point surrounded by sp…

Materials ScienceStrongly Correlated Electrons

Magnetic ordering in the static intermediate-valent cerium compound Ce2RuZn4

Volker Eyert、Ernst-Wilhelm Scheidt、Wolfgang Scherer 等 5 位作者2008-08-21arXiv

The low-temperature behavior of Ce2RuZn4 has been investigated. Specific heat and magnetic susceptibility data reveal an antiferromagnetic transition at a Neel temperature of 2 K. Ce2RuZn4 is a static intermediate-valent compound with two crystallographically independent cerium atoms. The magnetic data clearly show th…

Strongly Correlated ElectronsMaterials Science

GaMnAs: layers, wires and dots

Janusz Sadowski2008-08-21arXiv

Thin layers of GaMnAs ferromagnetic semiconductor grown by molecular beam epitaxy on GaAs(001) substrates were studied. To improve their magnetic properties the post-growth annealing procedures were applied, using the surface passivation layers of amorphous arsenic. This post growth treatment effectively increases the…

Materials Science

Stress induced stripe formation in Pd/W(110)

T. O. Mentes、A. Locatelli、L. Aballe 等 4 位作者2008-08-21arXiv

A stress-induced stripe phase of submonolayer Pd on W(110) is observed by low-energy electron microscopy. The temperature dependence of the pattern is explained by the change both in the boundary free energy and elastic relaxation energy due to the increasing boundary width. The stripes are shown to disorder when the…

Materials Science

Frustration-driven successive metamagnetic transitions in TbB4

T. Inami、K. Ohwada、Y. H. Matsuda 等 8 位作者2008-08-21arXiv

Resonant magnetic x-ray diffraction experiments on the Shastry-Sutherland lattice TbB$_4$ were carried out under strong pulsed magnetic fields up to 30 T. TbB$_4$ exhibits a multi-step magnetization process above 16 T when magnetic fields are applied along the c-axis. We examined the intensity of the 010 magnetic refl…

cond-mat.otherMaterials Science