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Steady-state, effective-temperature dynamics in a glassy material

J. S. Langer、M. Lisa Manning2007-11-13Physical Review E

We present a shear-transformation-zone (STZ)-based analysis of numerical simulations by Haxton and Liu [Phys. Rev. Lett. 99, 195701 (2007)]. The extensive Haxton and Liu (HL) data sharply test the basic assumptions of the STZ theory, especially the central role played by the effective disorder temperature as a dynamic…

Liquid Crystal Research AdvancementsMaterial Dynamics and PropertiesTheoretical and Computational Physics

Spin-wave resonances inLa0.7Sr0.3MnO3films: Measurement of spin-wave stiffness and anisotropy field

M. Golosovsky、P. Monod、P. K. Muduli 等 4 位作者2007-11-13Physical Review B

We studied magnetic-field-dependent microwave absorption in epitaxial ${\mathrm{La}}_{0.7}{\mathrm{Sr}}_{0.3}\mathrm{Mn}{\mathrm{O}}_{3}$ films using an $9.5\phantom{\rule{0.3em}{0ex}}\mathrm{GHz}$ Bruker electron-spin-resonance spectrometer. By analyzing the angular and temperature dependence of the ferromagnetic and…

Magnetic and transport properties of perovskites and related materialsAdvanced Condensed Matter PhysicsMagnetic Properties of Alloys

Nonresonant microwave absorption in epitaxialLa0.7Sr0.3MnO3films and its relation to colossal magnetoresistance

M. Golosovsky、P. Monod、P. K. Muduli 等 6 位作者2007-11-13Physical Review B

We study magnetic-field-dependent nonresonant microwave absorption and dispersion in thin ${\mathrm{La}}_{0.7}{\mathrm{Sr}}_{0.3}\mathrm{Mn}{\mathrm{O}}_{3}$ films and show that it originates from colossal magnetoresistance. We develop a model for the magnetoresistance of a thin ferromagnetic film in an oblique magnet…

Magnetic and transport properties of perovskites and related materialsMultiferroics and related materialsAdvanced Condensed Matter Physics

Screening effects on field emission from arrays of (5,5) carbon nanotubes: Quantum mechanical simulations

Guihua Chen、Weiliang Wang、Jie Peng 等 7 位作者2007-11-13Physical Review B

The simulation of field electron emission from arrays of micrometer-long open-ended (5,5) carbon nanotubes is performed in the framework of quantum theory of many electrons. It is found that the applied external field is strongly screened when the spacing distance is shorter than the length of the carbon nanotubes. Th…

Carbon Nanotubes in CompositesMechanical and Optical ResonatorsNanopore and Nanochannel Transport Studies

Electron waves in chemically substituted graphene

N. M. R. Peres、F. D. Klironomos、S.-W. Tsai 等 6 位作者2007-11-13Europhysics Letters (EPL)

We present exact analytical and numerical results for the electronic spectra and the Friedel oscillations around a substitutional impurity atom in a graphene lattice. A chemical dopant in graphene introduces changes in the on-site potential as well as in the hopping amplitude. We employ a T -matrix formalism and find…

Graphene research and applicationsQuantum and electron transport phenomenaTopological Materials and Phenomena

Solvent-Induced Transition from Micelles in Solution to Cylindrical Microdomains in Diblock Copolymer Thin Films

Soo‐Jin Park、Jiayu Wang、Bokyung Kim 等 5 位作者2007-11-13Macromolecules

It is well-known that block copolymer thin films can be easily prepared on different substrates by spin coating. Here, we show that the cylindrical microdomains of polystyrene- b -poly(4-vinylpyridine) (PS- b -P4VP) copolymers can be oriented normal to the surface over a large area by spin coating in toluene/THF solve…

Advanced Polymer Synthesis and CharacterizationBlock Copolymer Self-AssemblyFluid Dynamics and Thin Films

Strain localization in a shear transformation zone model for amorphous solids

M. Lisa Manning、J. S. Langer、Jean M. Carlson2007-11-13Physical Review E

We model a sheared disordered solid using the theory of shear transformation zones (STZs). In this mean-field continuum model the density of zones is governed by an effective temperature that approaches a steady state value as energy is dissipated. We compare the STZ model to simulations by Shi [Phys. Rev. Lett. 98, 1…

Material Dynamics and PropertiesTheoretical and Computational PhysicsMetallic Glasses and Amorphous Alloys

Size-Tailored Synthesis and Luminescent Properties of One-Dimensional Gd2O3:Eu3+ Nanorods and Microrods

Jun Yang、Chunxia Li、Ziyong Cheng 等 7 位作者2007-11-13The Journal of Physical Chemistry C

Nearly monodisperse and well-defined one-dimensional (1D) Gd 2 O 3:Eu 3+ nanorods and microrods were successfully prepared through a large-scale and facile hydrothermal method followed by a subsequent heat treatment process, without using any catalyst or template. X-ray diffraction (XRD), thermogravimetric analysis an…

Advanced Photocatalysis TechniquesLuminescence Properties of Advanced MaterialsCatalytic Processes in Materials Science

Optical properties of metal nanoparticles with no center of inversion symmetry: Observation of volume plasmons

Maxim Sukharev、Jiha Sung、Kenneth G. Spears 等 4 位作者2007-11-13Physical Review B

We present theoretical and experimental studies of the optical response of L-shaped silver nanoparticles. The scattering spectrum exhibits several plasmon resonances that depend sensitively on the polarization of the incident electromagnetic field. The physical origin of the resonances is traced to different plasmon p…

Gold and Silver Nanoparticles Synthesis and ApplicationsPlasmonic and Surface Plasmon ResearchNonlinear Optical Materials Studies

Magnetic nanowires as permanent magnet materials

T. Maurer、F. Ott、G. Chaboussant 等 6 位作者2007-11-13arXiv

We present the fabrication of metallic magnetic nanowires using a low temperature chemical process. We show that pressed powders and magnetically oriented samples exhibit a very high coercivity (6.5 kOe at 140 K and 4.8 kOe at 300 K). We discuss the magnetic properties of these metamaterials and show that they have th…

Materials Science

A Physically Based Dynamic Model for Solid Oxide Fuel Cells

Caisheng Wang、M.H. Nehrir2007-11-13IEEE Transactions on Energy Conversion

This paper presents a physically based dynamic model for tubular solid oxide fuel cells (SOFCs) based on the electrochemical and thermodynamic characteristics inside SOFC. The diffusion, material conservation, electrochemical, and thermodynamic equations are used to develop the SOFC model. The effect of temperature on…

Advancements in Solid Oxide Fuel CellsFuel Cells and Related MaterialsCatalysis and Oxidation Reactions

The Mechanism of TBD-Catalyzed Ring-Opening Polymerization of Cyclic Esters

Luis Simón、Jonathan M. Goodman2007-11-13The Journal of Organic Chemistry

Triazabicyclodecene (TBD) has recently been shown to be an effective organocatalyst for the ring-opening polymerization (ROP) of cyclic esters. Using DFT methods, we have studied possible mechanisms of this reaction. Our studies explain not only the narrow polydispersity index (PDI) observed in the ROP of six-membered…

Organometallic Complex Synthesis and Catalysisbiodegradable polymer synthesis and propertiesCarbon dioxide utilization in catalysis

The anomalous behavior of the density of water in the range 30 K < T < 373 K

Francesco Mallamace、C. Branca、Matteo Broccio 等 6 位作者2007-11-13Proceedings of the National Academy of Sciences

The temperature dependence of the density of water, rho(T), is obtained by means of optical scattering data, Raman and Fourier transform infrared, in a very wide temperature range, 30 < T < 373 K. This interval covers three regions: the thermodynamically stable liquid phase, the metastable supercooled phase, and the l…

Phase Equilibria and ThermodynamicsMaterial Dynamics and PropertiesThermodynamic properties of mixtures

Single-walled Carbon Nanotubes: Geno- and Cytotoxic Effects in Lung Fibroblast V79 Cells

Elena R. Kisin、Ashley Murray、Michael P. Keane 等 11 位作者2007-11-13OpenAlex

With the development of nanotechnology, there is a tremendous growth of the application of nanomaterials, which increases the risk of human exposure to these nanomaterials through inhalation, ingestion, and dermal penetration. Among different types of nanoparticles, single-walled carbon nanotubes (SWCNT) with extremel…

Carbon Nanotubes in CompositesNanoparticles: synthesis and applicationsAir Quality and Health Impacts

Raman Spectroscopy of Nickel Sulfide Ni3S2

Zhe Cheng、Harry Abernathy、Meilin Liu2007-11-13OpenAlex

High Resolution Image Download MS PowerPoint Slide Raman spectra of nickel sulfides reported in previous studies are inconsistent due possibly to the difficulty in obtaining samples of the required purity in composition and phase. In this study, Raman spectra for both the low-temperature (heazlewoodite)- and the high-…

Advancements in Solid Oxide Fuel CellsThermal and Kinetic AnalysisElectronic and Structural Properties of Oxides

Control Strategy of Fuel Cell and Supercapacitors Association for a Distributed Generation System

Phatiphat Thounthong、Stéphane Raël、Bernard Davat2007-11-13OpenAlex

This paper proposes an innovative control strategy for a voltage-regulated dc hybrid power source employing polymer electrolyte membrane fuel cell as the main energy source and supercapacitors as the auxiliary power source for a distributed generation system. This strategy is based on a standard dc link voltage regula…

Supercapacitor Materials and FabricationFuel Cells and Related MaterialsElectric and Hybrid Vehicle Technologies

Oligonucleotide Loading Determines Cellular Uptake of DNA-Modified Gold Nanoparticles

David A. Giljohann、Dwight S. Seferos、Pinal C. Patel 等 6 位作者2007-11-13OpenAlex

The cellular internalization of oligonucleotide-modified nanoparticles is investigated. Uptake is dependent on the density of the oligonucleotide loading on the surface of the particles, where higher densities lead to greater uptake. Densely functionalized nanoparticles adsorb a large number of proteins on the nanopar…

Gold and Silver Nanoparticles Synthesis and ApplicationsAdvanced biosensing and bioanalysis techniquesRNA Interference and Gene Delivery

Inorganic semiconductor nanostructures and their field-emission applications

Xiaosheng Fang、Yoshio Bando、Ujjal K. Gautam 等 5 位作者2007-11-13OpenAlex

Inorganic semiconductor nanostructures are ideal systems for exploring a large number of novel phenomena at the nanoscale and investigating the size and dimensionality dependence of their properties for potential applications. The use of such nanostructures with tailored geometries as building blocks is also expected…

ZnO doping and propertiesGas Sensing Nanomaterials and SensorsNanowire Synthesis and Applications

Improvement of the Mechanical Properties of Soy Protein Isolate Based Plastics through Formulation and Processing

M. Baboi、Gowrishankar Srinivasan、J. L. Jane 等 4 位作者2007-11-12International Polymer Processing

Abstract This paper reviews the characterization of the base strength and impact of water absorption on biodegradable, namely, soy protein-based plastics prepared by different methods. The initial approach included using different quantities of soy hydrolysate plasticized with glycerol, which is widely known for its p…

Nanocomposite Films for Food Packagingbiodegradable polymer synthesis and propertiesMicroplastics and Plastic Pollution

Growth mode mapping and structural properties of controlled perovskite BaTiO3∕SrTiO3 heterostructure

Jin Long Li、Jianhua Hao、Zhang Ying 等 4 位作者2007-11-12Applied Physics Letters

Perovskite heteroepitaxy was investigated under various conditions using laser molecular beam epitaxy. Well-controlled BaTiO3∕SrTiO3 heterostructure was studied with in situ reflective high energy electron diffraction and ex situ atomic force microscopy, x-ray diffraction, and transmission electron microscopy. The gro…

Ferroelectric and Piezoelectric MaterialsPhotorefractive and Nonlinear OpticsElectronic and Structural Properties of Oxides