Materials Literature
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Lining up: Highly symmetrically arranged ZnO nanowire arrays (see image) are produced by laser-interference lithography and a chemical vapor transport process. The nanowires show a narrow diameter distribution and uniform spacing. A liquid-phase-assisted vapor–solid mechanism is proposed for one-to-one synthesized ZnO…
The investigation of the role of interactions in magnetic wire arrays is complex and often subject to strong simplifications. In this paper we obtained analytical expressions for the magnetostatic interactions between wires and investigate the range of validity of dipole-dipole, first order and second order approximat…
The Born-Oppenheimer approximation (BO) has proven effective for the accurate determination of chemical reactions, molecular dynamics and phonon frequencies in a wide range of metallic systems. Graphene, recently discovered in the free state, is a zero band-gap semiconductor, which becomes a metal if the Fermi energy…
The interaction between graphene layers is analyzed using a local orbital occupancy approach and second-order perturbation theory. This perturbation theory yields the van der Waals forces which are calculated, within the local orbital approach, using an atom-atom interaction approximation and the local density of stat…
We report here the results from a glasshouse trial of several transgenic sugarcane (Saccharum spp. hybrids) lines accumulating the bacterial polyester polyhydroxybutyrate (PHB) in plastids. The aims of the trial were to characterize the spatio-temporal pattern of PHB accumulation at a whole-plant level, to identify fa…
We discuss methods for imaging the nonequilibrium spin polarization of electrons in Fe/GaAs spin transport devices. Both optically- and electrically-injected spin distributions are studied by scanning magneto-optical Kerr rotation microscopy. Related methods are used to demonstrate electrical spin detection of optical…
We consider the model of the optical switching center - a system with the following properties: It has two (or more) metastable states |1>, |2>, separated by a potential barrier U; it can switch from one state to another by absorbing the photons with energy proportional to U; the transition from |1> to |2> is allowed…
The temperature dependent energy transfer rate between charge carriers and lattice has been experimentally investigated in ferromagnetic semiconductors. Studied 100 nm thick low-temperature MBE grown Mn_{x}Ga_{1-x}As samples had manganese concentrations x=3.7 % and 4.0 %. Curie temperatures estimated from temperatures…
Back in the saddle: Copper corroles do not contain a CuIII ion, but rather a well-hidden CuII ion. A comparative crystallographic and theoretical study (see spin-density representation) of isostructural corroloid complexes with copper ions in different formal oxidation states suggests that the divalent state is stabil…
We investigate a disordered version of a thermodynamic fiber bundle model proposed by Selinger, Wang, Gelbart, and Ben-Shaul a few years ago. For simple forms of disorder, the model is analytically tractable and displays some new features. At either constant stress or constant strain, there is a non monotonic increase…
Ground-state structures and other experimentally relevant isomers of Au(15) (-) to Au(24) (-) clusters are determined through joint first-principles density functional theory and photoelectron spectroscopy measurements. Subsequent calculations of molecular O(2) adsorption to the optimal cluster structures reveal a siz…
We investigate the relationships among magnetic, dielectric, and ferroelectric properties of a frustrated spin system $\mathrm{Mn}\mathrm{W}{\mathrm{O}}_{4}$, which undergoes several magnetic phase transitions including a commensurate-incommensurate and a collinear-noncollinear transition. Dielectric and pyroelectric…
We apply the self-interaction corrected local spin density approximation to study the electronic structure and magnetic properties of the spinel ferrites $\mathrm{Mn}{\mathrm{Fe}}_{2}{\mathrm{O}}_{4}$, ${\mathrm{Fe}}_{3}{\mathrm{O}}_{4}$, $\mathrm{Co}{\mathrm{Fe}}_{2}{\mathrm{O}}_{4}$, and $\mathrm{Ni}{\mathrm{Fe}}_{2…
The magnetic exchange between epitaxial thin films of the multiferroic (antiferromagnetic and ferroelectric) hexagonal YMnO3 oxide and a soft ferromagnetic (FM) layer is used to couple the magnetic response of the FM layer to the magnetic state of the antiferromagnetic one. We will show that biasing the ferroelectric…
We show that Friedel oscillations (FO) in grapehene are strongly affected by the chirality of electrons in this material. In particular, the FO of the charge density around an impurity show a faster (deltarho approximately r;{-3}) decay than in conventional 2D electron systems and do not contribute to a linear tempera…
Liberating hydrogen: Strong Lewis or Brønsted acids react with ammonia–borane (H3NBH3) to form an in situ boronium cation, resulting in the formation of a mixture of cyclic and acyclic BNHx oligomers and the liberation of H2 (see scheme). A proposed mechanism is supported by an examination of the reaction thermodynami…
This study investigates the aqueous stability of multi-walled carbon nanotubes (MWNTs) in the presence of natural organic matter (NOM). MWNTs were readily dispersed as an aqueous suspension in both model NOM (Suwannee River NOM (SR-NOM)) solutions and natural surface water (actual Suwannee River water with unaltered N…
We study two-component single-file diffusion inside a narrow channel that at its ends is open and connected with particle reservoirs. Using a two-species version of the symmetric simple exclusion process as a model, we propose a hydrodynamic description of the coarse-grained dynamics with a self-diffusion coeffcient t…
The synthesis of (group I) hydrochloric acid-doped poly(aniline-co-toluidine), poly(aniline-co-thiophene), poly(aniline-co-o-phenylenediamine), and poly(aniline-co-2-aminopyridine) as well as their hydrochloric acid-doped homopolymers of polyaniline, poly-m-toluidine, poly-o-phenylene diamine, and poly-2-aminopyridine…
Abstract We report the effect of organosilica precursor isomers on the interfacial interaction between polyimide and organosilica in polyimide/organosilica hybrid composite films. Poly(4,4′‐oxydianiline biphenyltetracarboxamic acid) (BPDA‐ODA PAA) was used as the polyimide precursor, while the organosilica was made us…