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Polarization of Valence Band Holes in the (Ga,Mn)As Diluted Magnetic Semiconductor

V. F. Sapega、M. Moreno、M. Ramsteiner 等 5 位作者2005-04-04Physical Review Letters

We report on direct measurements of the impurity band hole polarization in the diluted magnetic semiconductor (Ga,Mn)As. The polarization of impurity band holes in a magnetic field is strongly enhanced by antiferromagnetic exchange interaction with Mn ions. The temperature dependence of the hole polarization shows a s…

ZnO doping and propertiesGa2O3 and related materialsPhysics of Superconductivity and Magnetism

Aktive Zentren an Oxidoberflächen: Die ZnO‐katalysierte Methanolsynthese aus CO und H2

Melanie Kurtz、Jennifer Strunk、Olaf Hinrichsen 等 7 位作者2005-04-04Angewandte Chemie

Ist da noch ein Platz frei? Für die Bildung von Methanol aus CO und H2 an ZnO-Oberflächen wird auf der Grundlage von Rechnungen und Experimenten ein Mechanismus vorgeschlagen, bei dem CO an Sauerstoff-Fehlstellen des Heterogenkatalysators adsorbiert (siehe Bild; C rot, H weiß, O grau, Zn schwarz). Beigemischtes CO2 bl…

Catalysts for Methane ReformingAdvanced Chemical Physics StudiesCatalytic Processes in Materials Science

Magnetization manipulation in (Ga,Mn)As by subpicosecond optical excitation

G. V. Astakhov、A. V. Kimel、G. M. Schott 等 11 位作者2005-04-04Applied Physics Letters

We demonstrate complete reversal of a full magnetic hysteresis loop of the magnetic semiconductor (Ga,Mn)As by ultrashort optical excitation with a single subpicosecond light pulse, with obvious implications for ultrafast magneto-optical recording. Our approach utilizes the fourfold magnetic anisotropy of (Ga,Mn)As, i…

ZnO doping and propertiesMagnetic properties of thin filmsMagneto-Optical Properties and Applications

Quantum-dot-based multiplexed fluorescence resonance energy transfer

Aaron R. Clapp、Igor L. Medintz、Harry T. Uyeda 等 5 位作者2005-04-04Proceedings of SPIE, the International Society for Optical Engineering/Proceedings of SPIE

Colloidal semiconductor quantum dots (QDs) have narrow photoemission bandwidths and broad absorption spectra that are ideal for multiplexing applications. In contrast to organic dyes, which require a complex arrangement of excitation sources and filters to generate multiple signals, many populations of QDs can be simu…

Nanocluster Synthesis and ApplicationsQuantum Dots Synthesis And PropertiesAdvanced Biosensing Techniques and Applications

Nanofibers from functionalized para-phenylene molecules

Manuela Schiek、Arne Lützen、Rainer Koch 等 7 位作者2005-04-04Applied Physics Letters

Tens to hundreds of micrometers long organic nanofibers have been generated from methoxy functionalized quaterphenylene molecules. The mutual alignment of the fibers is similar to that of previously reported nanofibers from para-hexaphenylene, and they emit intense, blue light centered at 400 nm with well resolved hig…

Photonic Crystals and ApplicationsOrganic Electronics and PhotovoltaicsLuminescence and Fluorescent Materials

Verification of Hume-Rothery electron concentration rule inCu5Zn8andCu9Al4γbrasses byab initioFLAPW band calculations

Ryoji Asahi、Hirokazu Sato、Tsunehiro Takeuchi 等 4 位作者2005-04-04Physical Review B

Both ${\mathrm{Cu}}_{5}{\mathrm{Zn}}_{8}$ and ${\mathrm{Cu}}_{9}{\mathrm{Al}}_{4}$ $\ensuremath{\gamma}$ brasses containing 52 atoms in its cubic cell have been recognized as a typical Hume-Rothery alloy phase, since these structurally complex compounds are stabilized at the same electron concentration of 1.61 electro…

Magnetic properties of thin filmsAluminum Alloy Microstructure PropertiesQuasicrystal Structures and Properties

Photostimulated luminescence from fluorochlorozirconate glass ceramics and the effect of crystallite size

Stefan Schweizer、L. W. Hobbs、M. Secu 等 7 位作者2005-04-04Journal of Applied Physics

We report the results from a study of europium-doped fluorochlorozirconate glasses that have been thermally processed to induce nucleation and crystallization of BaCl2 crystallites. The resulting glass ceramics show a photostimulated luminescence (PSL) effect with a conversion efficiency which is up to 80% of that fou…

Glass properties and applicationsRadiation Detection and Scintillator TechnologiesLuminescence Properties of Advanced Materials

Unexpected periodicity in the quasi-two-dimensional Mott insulator1T−TaS2revealed by angle-resolved photoemission

L. Perfetti、Thomas Gloor、Frédéric Mila 等 5 位作者2005-04-04Physical Review B

High-resolution angle-resolved photoemission data from the insulating phase of the charge-density-wave (CDW) material $1T\text{\ensuremath{-}}{\mathrm{TaS}}_{2}$ reveal the backfolding of the electronic bands associated with the CDW superlattice, but also an additional, unexpected periodicity. This periodicity is cons…

Magnetic and transport properties of perovskites and related materialsElectronic and Structural Properties of OxidesOrganic and Molecular Conductors Research

Helicoid to Spiral Ribbon Transition

Rouzbeh Ghafouri、Robijn Bruinsma2005-04-04Physical Review Letters

We present a continuum description for the transition between the helicoid and spiral ribbon structures of chiral materials. At a critical value of the ratio between the bending and stretching moduli, the Föppl-von Kármán number, we encounter a continuous buckling transition from a straight helicoid to a spiral ribbon…

Liquid Crystal Research AdvancementsMicro and Nano RoboticsAdvanced Materials and Mechanics

Microscale modeling of kinking nonlinear elastic solids

Michel W. Barsoum、T. Zhen、Aiguo Zhou 等 5 位作者2005-04-04Physical Review B

Recently we identified and classified a class of solids as kinking nonlinear elastic (KNE) because they deform by the formation of kink bands. KNE solids represent a large family that include, among others, layered ternary carbides and nitrides, layered oxides and semiconductors, zinc, cadmium, graphite, ice, and the…

Advanced ceramic materials synthesisMetal and Thin Film MechanicsMXene and MAX Phase Materials

Ferromagnetic percolation in MnxGe1−x dilute magnetic semiconductor

An‐Ping Li、Jian Shen、J. R. Thompson 等 4 位作者2005-04-04Applied Physics Letters

We have studied the magnetic and magnetotransport properties of Mn-doped Ge grown by molecular-beam epitaxy. This group-IV dilute ferromagnetic semiconductor exhibits two magnetic transitions. An upper critical temperature TC* (∼112K for x∼0.05) is evident from the extrapolated Curie–Weiss susceptibility and from the…

Semiconductor Quantum Structures and DevicesZnO doping and propertiesMagnetic and transport properties of perovskites and related materials

4p states and X-Ray Spectroscopy

Jun-ichi Igarashi、Manabu Takahashi2005-04-04arXiv

The 4p states in transition metals and their compounds usually play minor roles on their physical quantities. Recent development of resonant x-ray scattering (RXS) at the K-edge of transition metals, however, casts light on the 4p states, because the signals on orbital and magnetic superlattice spots are brought about…

Materials Science

Transition from Ferromagnetism to Antiferromagnetism in Ga$_{1-x}$Mn$_x$N

Gustavo M. Dalpian、Su-Huai Wei2005-04-04arXiv

Using density functional theory, we study the magnetic stability of the Ga$_{1-x}$Mn$_x$N alloy system. We show that unlike Ga$_{1-x}$Mn$_x$As, which shows only ferromagnetic (FM) phase, Ga$_{1-x}$Mn$_x$N can be stable in either FM or antiferromagnetic phases depending on the alloy concentration. The magnetic order ca…

Materials Science

Direct observation of negative electron affinity in hydrogen-terminated diamond surfaces

Daisuke Takeuchi、Hiromitsu Kato、Gum-Chol Ri 等 9 位作者2005-04-04Applied Physics Letters

Total photoyield experiments are applied to characterize p-, intrinsic, and n-type diamond with hydrogen-terminated surfaces. On all hydrogen-terminated samples a photoelectron threshold energy of 4.4 eV is detected which is discussed in detail in this letter. We attribute this threshold to the energy gap between the…

Advanced Optical Sensing TechnologiesPhotocathodes and Microchannel PlatesDiamond and Carbon-based Materials Research

Systematic ab initio study of the optical properties of BN nanotubes

Guang‐Yu Guo、J. C. Lin2005-04-04Physical Review B

A systematic ab initio study of the optical and electronic properties of BN nanotubes within density functional theory in the local density approximation is performed. Specifically, the optical dielectric function $\ensuremath{\epsilon}$ and the band structure of the single-walled zigzag [(5,0),(6,0),(9,0),(12,0),(15,…

MXene and MAX Phase MaterialsGraphene research and applicationsBoron and Carbon Nanomaterials Research

Dispersive photoluminescence decay by geminate recombination in amorphous semiconductors

Kazuhiko Seki、K. Murayama、M. Tachiya2005-04-04arXiv

The photoluminescence decay in amorphous semiconductors is described by power law $t^{-delta}$ at long times. The power-law decay of photoluminescence at long times is commonly observed but recent experiments have revealed that the exponent, $delta sim 1.2-1.3$, is smaller than the value 1.5 predicted from a geminate…

Materials Sciencecond-mat.stat-mech

Metallic atomic wires on a patterned dihydrogeneted Si(001)

Bikash C Gupta、Inder P. Batra2005-04-04arXiv

Electronic structure calculations for atomic wire of metals like Al, Ga and In are performed for a patterned dihydrogeneted Si(001):1 $\times$ 1 in search of structures with metallic behavior. The dihydrogeneted Si(001) is patterned by depassivating hygrozen atoms only from one row of Si atoms along the [1$\bar{1}$0]…

Materials Science

Band structure model of magnetic coupling in semiconductors

Gustavo M. Dalpian、Su-Huai Wei、X. G. Gong 等 5 位作者2005-04-04arXiv

We present a unified band structure model to explain magnetic ordering in Mn-doped semiconductors. This model is based on the $p$-$d$ and $d$-$d$ level repulsions between the Mn ions and host elements and can successfully explain magnetic ordering observed in all Mn doped II-VI and III-V semiconductors such as CdTe, G…

Materials Science

Solitons and decoherence in left-handed metamaterials

M. Marklund、P. K. Shukla、L. Stenflo 等 4 位作者2005-04-04arXiv

We present exact electromagnetic solitary pulses that can be experimentally obtained within nonlinear left-handed metamaterials. The effect of pulse decoherence on the modulation instability of partially incoherent electromagnetic waves is also investigated. The results may contribute to a better understanding of nonl…

Materials Sciencenlin.PS

Solid phase epitaxy of ferromagnetic MnAs dots on GaMnAs layers

J. Sadowski、M. Adell、J. Kanski 等 9 位作者2005-04-04arXiv

Formation of MnAs quantum dots in a regular ring-like distribution has been found on MBE-grown (GaMn)As surfaces after low-temperature annealing under As capping. The Mn was supplied by out-diffusing Mn interstitials from (GaMn)As. With 5 at% substitutional Mn the quantum dots appeared for (GaMn)As layers thicker than…

Materials Science