Materials Literature
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We investigate the response of a terahertz metamaterial depending on the unit cell density. The fundamental inductive capacitive (LC) resonance has its highest quality (Q) factor for a critical period Pc=λ/n, with λ being the LC resonance wavelength and n being the refractive index of the substrate. This occurs due to…
Distinguishing from the traditional characterization on high-field leakage current density-voltage relationship, the field-dependent permittivity from the polarization derivative is used to solve the space-charge-limited conduction, and the simulated leakage current densities are compared with the previous experimenta…
A chitosan/porous silicon biosensing platform for the detection of carboxylic acid-containing drugs in water is prepared and characterized. Parasitic layer-free films of mesoporous silicon are electrochemically etched and functionalized by covalent attachment of chitosan oligomers. The presence of the chitosan species…
A nonconjugated fluorescent molecule with a triarylboron acceptor and an alkylamine donor has been found to display bright green fluorescence due to charge transfer through space, which can be reversibly deactivated by blocking either the donor or acceptor site. Binding of the fluoride ion to boron switches the fluore…
We use classical molecular dynamics to evaluate the thermal conductivity $\ensuremath{\kappa}(T)$ from the heat-flux correlation $⟨\mathbf{j}(0)\mathbf{j}(t)⟩$ for a two-dimensional Lennard-Jones triangular lattice. Our work, which follows Ladd, Moran, and Hoover [Phys. Rev. B 34, 5058 (1986)], finds large deviations…
Graphene layers have been grown by molecular beam epitaxy (MBE) on the (0001¯) C-face of SiC and have been characterized by atomic force microscopy, low energy electron diffraction (LEED), and UV photoelectron spectroscopy. Contrary to the graphitization process, the step-terrace structure of SiC is fully preserved du…
The aim of this study was to prepare and characterize membranes of silk fibroin (SF) and chitosan (CHI) blends. Moreover, a conformation transition of SF to a more stable form induced by the addition of CHI was verified. Blend membranes were prepared, after pH adjustment, in different ratios, and physical integrity, c…
A simple isocyanate-free method to synthesize poly(trimethylene carbonate hydroxy-urethane)s is described. The strategy first involves the synthesis of α,ω-di(cyclic carbonate) telechelic polycarbonate precursors upon ring-opening polymerization of trimethylene carbonate using a cyclic carbonate alcohol as chain trans…
The nonlinear dielectric properties of dense BaTiO3 ceramics with grain size of 1 μm–90 nm were investigated. In the finest ceramics, the permittivity reduces below 1000 and a remarkable nonhysteretic linear dc-tunability [ε(E)] is obtained at high field, above 40 kV/cm. The observed behavior was explained by consider…
We propose a topological order parameter for interacting topological insulators, expressed in terms of the full Green's functions of the interacting system. We show that it is exactly quantized for a time reversal invariant topological insulator, and it can be experimentally measured through the topological magneto-el…
An electrostatic quantum dot cannot be formed in monolayer graphene because of the Klein tunneling. However, a dot can be formed with the help of a uniform magnetic field. As shown here, a spatial modulation of the Dirac gap leads to confined states with discrete energy levels, thus defining a dot, without applying ex…
In this work, we experimentally demonstrate a novel and simple approach that uses off-the-shelf optical elements to enhance the collection efficiency from a single emitter. The key component is a solid immersion lens made of diamond, the host material for single color centers. We improve the excitation and detection o…
A series of near-infrared solid-state emitters based on the dicyanoisophorone electron acceptor group was synthesized. The solid-state spectroscopic properties were studied by UV−visible absorption spectroscopy and fluorescence spectroscopy and analyzed in light of the single crystal structures obtained by X-ray diffr…
We describe a test particle approach based on dynamical density functional theory (DDFT) for studying the correlated time evolution of the particles that constitute a fluid. Our theory provides a means of calculating the van Hove distribution function by treating its self and distinct parts as the two components of a…
The current status of research and development of carbon nanotubes (CNTs) electron field emitters is reviewed. The physical aspects of electron field emission that underlie the unique emission properties of CNTs are considered. Physical effects and phenomena affecting the emission characteristics of CNT cathodes are a…
This work defines the crystallinity of cellulose I materials on a dry-weight basis. Theoretical and experimental developments in X-ray diffraction lead to a crystallinity determination method that is estimated to reach 1σ accuracies of better than 0.05 (crystallinity defined between 0 and 1). The method is based on Ri…
A polymer triple-shape memory effect represents one of the most recent discoveries in the rapidly expanding field of shape memory polymers. It refers to the capability of a polymer to memorize two temporary shapes and subsequently recover them, all in one shape memory cycle. Although several examples of triple-shape p…
The effects of applied microwave power, gas flow rate and precursor composition on the substrate-free gas-phase synthesis of graphene were investigated. Graphene was produced through the delivery of ethanol droplets into argon plasmas, and a decrease in the flow rate of the gas used to generate the plasmas resulted in…
We present a derivation of the recently proposed eighth-order phase-field crystal model [A. Jaatinen, Phys. Rev. E 80, 031602 (2009)] for the crystallization of a solid from an undercooled melt. The model is used to study the planar growth of a two-dimensional hexagonal crystal, and the results are compared against si…
In this letter we not only show improvement in the performance but also in the reliability of 30nm thick biaxially strained SiGe (20%Ge) channel on Si p-MOSFETs. Compared to Si channel, strained SiGe channel allows larger hole mobility (μh) in the transport direction and alleviates charge flow towards the gate oxide.…