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Organic Nanostructured Host–Guest Materials Containing Three Dyes

Chiara Botta、Greta Pătrinoiu、Pierre Picouet 等 12 位作者2004-10-04Advanced Materials

Dyes inserted into the parallel nanochannels of a fully organic crystal show efficient light conversion over a wide visible spectral region, with 100 % conversion from UV to blue light. The Figure shows crystals containing either two (bottom) or three (top) dyes under UV illumination, and a top view of the structure o…

Conducting polymers and applicationsPorphyrin and Phthalocyanine ChemistryLuminescence and Fluorescent Materials

Quantum Superposition of High Spin States in the Single Molecule MagnetNi4

E. del Barco、Andrew D. Kent、En‐Che Yang 等 4 位作者2004-10-04Physical Review Letters

Quantum tunneling of the magnetization in a single molecule magnet has been studied in experiments that combine microwave spectroscopy with high sensitivity magnetic measurements. By monitoring spin-state populations in the presence of microwave radiation, the energy splittings between low lying superpositions of high…

Magnetism in coordination complexesLanthanide and Transition Metal ComplexesElectron Spin Resonance Studies

Distributed control of thermoelectric coolers

D. G. Walker、Kenneth D. Frampton、R. D. Harvey2004-10-04OpenAlex

Thermoelectric refrigeration has been studied for use in electronics cooling applications. Because of their low efficiency, a significant amount of additional heat is produced that must be removed from the device by passive means. However, even well-designed passive heat removal systems are faced with physical limitat…

Advanced Thermoelectric Materials and DevicesThermal properties of materialsThermal Radiation and Cooling Technologies

Thermoelectric PbTe thin film for superresolution optical data storage

Hyun Seok Lee、Byung‐ki Cheong、Taek Sung Lee 等 8 位作者2004-10-04Applied Physics Letters

To find its practical use in ultrahigh density optical data storage, superresolution (SR) technique needs a material that can render a high SR capability at no cost of durability against repeated readout and write. Thermoelectric materials appear to be promising candidates due to their capability of yielding phase-cha…

Chalcogenide Semiconductor Thin FilmsPhotorefractive and Nonlinear OpticsPhase-change materials and chalcogenides

Transmission electron microscopy and transistor characteristics of the same carbon nanotube

Jannik C. Meyer、Dirk Obergfell、Siegmar Roth 等 5 位作者2004-10-04Applied Physics Letters

A technique is presented which allows one to combine TEM investigations with transport measurements and potentially a wide range of other investigations on the same nanoobject. Using this technique, we have obtained high-resolution transmission electron microscopy images and transport investigations including transfer…

Carbon Nanotubes in CompositesGraphene research and applicationsFullerene Chemistry and Applications

Highly photoconductive amorphous carbon nitride films prepared by cyclic nitrogen radical sputtering

T. Katsuno、Shugo Nitta、Hitoe Habuchi 等 5 位作者2004-10-04Applied Physics Letters

We report on the growth of amorphous carbon nitride films (a-CNx) showing the highest conductivity to date. The films were prepared using a layer-by-layer method (a-CNx:LL), by the cyclical nitrogen radical sputtering of a graphite radical, alternated with a brief hydrogen etch. The photosensitivity S of these films i…

Semiconductor materials and devicesDiamond and Carbon-based Materials ResearchThin-Film Transistor Technologies

Computer simulation of photoinduced mass transport on azobenzene polymer films by particle method

Daisuke Barada、Mitsuru Itoh、Toyohiko Yatagai2004-10-04Journal of Applied Physics

The formation and erasure of photoinduced surface relief gratings (SRGs) on azobenzene-containing polymers are simulated using a calculation model based on the moving-particle semi-implicit method. For the convection calculation, an anisotropic diffusion model is proposed. The gradient force of the optical electric fi…

Liquid Crystal Research AdvancementsOptical Coatings and GratingsElectrowetting and Microfluidic Technologies

Finite-Size Effects on the Structure of Grain Boundaries

Emmanuelle A. Marquis、J. C. Hamilton、Douglas L. Medlin 等 4 位作者2004-10-04Physical Review Letters

We present a combined experimental and theoretical analysis of the structure of finite-sized Sigma 3 [112] grain boundaries in Au. High-resolution electron microscopy shows lattice translations at the grain boundary, with the magnitude of the translation varying along the finite-sized grain boundaries. The presence of…

Microstructure and mechanical propertiesMetal and Thin Film MechanicsDiamond and Carbon-based Materials Research

Experimental analysis of the coalescence process via head-on collisions in a time-dependent flow

Marcos Borrell、Yosang Yoon、L. Gary Leal2004-10-04Physics of Fluids

The present study experimentally investigates the mechanisms involved in the flow-induced coalescence process for two equal-sized drops (polybutadiene drops suspended in a polydimethylsiloxane matrix), by taking advantage of the capability of the computer-controlled “four-roll mill” to carry out head-on collisions. In…

Surface Modification and SuperhydrophobicityPolymer crystallization and propertiesRheology and Fluid Dynamics Studies

Domain structure of sintered SmCo5 magnets studied by magneticforce microscopy

W. Szmaja、Jarosław Grobelny、M. Cichomski2004-10-04Applied Physics Letters

The domain structure of sintered SmCo5 permanent magnets at the surface perpendicular to the alignment axis was investigated by magnetic force microscopy (MFM). The main domains forming a maze pattern of typically 3–5μm in width and surface reverse spikes of typically 1–2μm in size are observed. This coarse domain str…

Magnetic properties of thin filmsMagnetic and transport properties of perovskites and related materialsMagnetic Properties of Alloys

Extending the limits of air cooling with thermoelectrically enhanced heat sinks

Jim Bierschenk、David A. Johnson2004-10-04OpenAlex

The prospects of using thermoelectric coolers (TECs) as a means to enhance heat sink performance and extend the limits of air cooling for electronics has considerable appeal when one considers the alternatives of liquid cooling. Historical analyses of TECs for electronics cooling only considered "off-the-shelf" TECs,…

Advanced Thermoelectric Materials and DevicesThermal properties of materialsThermal Radiation and Cooling Technologies

Enhanced thermal contact conductance using carbon nanotube arrays

Jun Xu、Timothy S. Fisher2004-10-04OpenAlex

Novel heat-conduction interfaces that employ carbon nanotube (CNT) arrays have been fabricated and studied experimentally. A reference calorimeter testing rig in a high vacuum environment with infrared temperature measurement has been established. Arrays of mat-type carbon nanotube layers have been grown directly on s…

Carbon Nanotubes in CompositesThermal properties of materialsAdhesion, Friction, and Surface Interactions

Optical constants of porous silicon films and multilayers determined by genetic algorithms

V. Torres‐Costa、Raúl J. Martín‐Palma、J.M. Martı́nez-Duart2004-10-04Journal of Applied Physics

Porous silicon (PS) can be optically described as a homogeneous mixture of air, silicon, and, eventually, silicon dioxide, which explains the great tunability of its refractive index. This behavior makes porous silicon a very interesting material for the development of interference filters for use in optoelectronic ap…

Semiconductor materials and devicesSilicon Nanostructures and PhotoluminescenceNanowire Synthesis and Applications

Maxwell–Wagner effect in hexagonal BaTiO3 single crystals grown by containerless processing

Jianding Yu、Paul‐François Paradis、Takehiko Ishikawa 等 4 位作者2004-10-04Applied Physics Letters

Oxygen-deficient hexagonal BaTiO3 single crystals, with dielectric constant ε′∼105 and loss component tan δ∼0.13 at room temperature and a linear temperature dependence of ε′ in the range 70–100K, was analyzed by impedance spectroscopy analysis. Two capacitors, bulk and interfacial boundary layer, were observed, and t…

Ferroelectric and Piezoelectric MaterialsMultiferroics and related materialsDielectric properties of ceramics

Large Spectral Birefringence in Photoaddressable Polymer Films

B. L. Lachut、Stefan A. Maier、Harry A. Atwater 等 7 位作者2004-10-04Advanced Materials

A photoaddressable azobenzene-side-chain polymer (see Figure) optimized to exhibit a large optical birefringence of Δn = 0.5 at 650 nm is described. The birefringence extends well into the telecommunication wavelength region, which, together with the high optical transparency above 650 nm, promises applications for in…

Photonic and Optical DevicesLiquid Crystal Research AdvancementsPhotochromic and Fluorescence Chemistry

Self‐Catalysis and Phase Transformation in the Formation of CdSe Nanosaws

Yifu Ding、Chengwei Ma、Zhong Lin Wang2004-10-04Advanced Materials

A wurtzite-structured CdSe nanosaw (see Figure) is formed by a two-step process: a fast-growth process along [010] creates the main ribbon, while a subsequent side-growth process along [0001] creates the one-sided teeth. The growth of the teeth is suggested to be a combined result of secondary epitaxial nucleation pro…

Quantum Dots Synthesis And PropertiesChalcogenide Semiconductor Thin FilmsCopper-based nanomaterials and applications

Microwave loss mechanisms in Ba0.25Sr0.75TiO3 thin film varactors

Andrei Vorobiev、Pär Rundqvist、K. Khamchane 等 4 位作者2004-10-04Journal of Applied Physics

Parallel-plate Au(Pt)∕Ba0.25Sr0.75TiO3∕(Pt)Au thin film varactors were fabricated on high resistance Si substrates and characterized at dc, rf, and microwave frequencies. In the frequency range 10–45 GHz the varactors show relatively low losses, with loss tangent less than 0.025 at 45 GHz. Due to the thick and highly…

Ferroelectric and Piezoelectric MaterialsAcoustic Wave Resonator TechnologiesMicrowave Dielectric Ceramics Synthesis

Transparent current spreading layers for optoelectronic devices

Adrian Porch、D.V. Morgan、R. M. Perks 等 5 位作者2004-10-04Journal of Applied Physics

In this paper we develop a simple model based on a leaky transmission line to assess the electrical performance of transparent current spreading layers for application to surface light emitting diodes. Figures of merit suitable for device design are obtained and these are applied to a range of material systems reporte…

ZnO doping and propertiesSemiconductor materials and devicesThin-Film Transistor Technologies

Energy spectra of backscattered electrons in Auger electron spectroscopy: comparison of Monte Carlo simulations with experiment

Zejun Ding、H. M. Li、Kenta Goto 等 5 位作者2004-10-04Journal of Applied Physics

The primary energy dependecne and atomic-number dependence of backscattered electrons in Auger electron spectroscopy in the EN(E) mode have been investigated both theoretically and experimentally. A Monte Carlo simulation method with inclusion of cascade-secondary-electron production has been used to calculate the ful…

X-ray Spectroscopy and Fluorescence AnalysisElectron and X-Ray Spectroscopy TechniquesSurface and Thin Film Phenomena

Anisotropy and magnetotransport in ordered magnetic antidot arrays

Fernando Castaño、Kornelius Nielsch、C. A. Ross 等 5 位作者2004-10-04Applied Physics Letters

Magnetic films containing ordered arrays of holes (“antidots”) with period ∼200nm have been prepared using porous anodic alumina substrates with square and hexagonal symmetries. Large area (∼cm2) single-layer CoFe ordered antidot arrays show well-defined in-plane magnetic anisotropy related to the symmetry of the arra…

Magnetic properties of thin filmsAnodic Oxide Films and NanostructuresNanoporous metals and alloys