Materials Literature
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Optical and morphological properties of fluorocarbon films (CFx) deposited on Si substrates from CHF3 in a reactive ion etcher were studied by spectroscopic ellipsometry (SE). The study has led for 0.3–1.5μm thick films to a thickness-independent, roughnessless, apparently nongraded two-layer model that requires the C…
The lattice dynamical results of silicon nanostructures with all three different degrees of confinement (nanoslabs, nanowires, nanodots) are systematically analysed and presented using an adiabatic bond charge model. In the direction of propagation of these structures, it is found that the phonon branches change from…
We describe the first demonstration of PbTe-based, cross-plane quantum-dot superlattice (QDSL) unicouple thermoelectric generator devices fabricated from nanostructured, thick-film materials (∼100μm). Both n- and p-type QDSL materials were investigated. With ∼220K temperature difference across small thermoelements (∼9…
We have chemically modified metal nanoslit array surfaces with alkanethiol self-assembled monolayers and have characterized the resulting spectral shift of optical transmission. Adsorption of a self-assembled monolayer (1.5nm thick) on a silver nanoslit array (slit width of 30–50nm and grating period of 360nm) is foun…
Low temperature photoluminescence spectra of synthetic $\mathrm{PbS}$ crystals having the natural isotopic abundance (95% $^{32}S$) are compared with crystals grown using 99% $^{34}S$. An anomalous decrease in the band gap energy of $6.5\ifmmode\pm\else\textpm\fi{}2\phantom{\rule{0.3em}{0ex}}{\mathrm{cm}}^{\ensuremath…
The Hugoniot and critical shear strength of shock-compressed metals can be obtained directly from molecular dynamics simulations without recourse to surface velocity profiles and their analyses. Results from simulations in aluminum containing an initial distribution of microscopic defects are shown to agree with exper…
We study the effect of vacancies and charged impurities on the performance of carbon nanotube transistors by self-consistently solving the three-dimensional Poisson and Schrödinger equations. We find that a single vacancy or charged impurity can decrease the drive current by more than 25% from the ballistic current. T…
CdTe-coated magnetic polystyrene nanospheres (MPN) were prepared via a stepwise electrostatic self-assembly approach, and the conjugation of epidermal growth factor (EGF) to the MPN/CdTe core–shell nanocomposites was prepared by using 1-ethyl-3(3-dimethylamino propyl)-carbodiimide (EDC) as a cross-linking reagent. The…
Nanodiamond films were deposited using different microwave plasma chemical vapor deposition schemes following several nucleation pretreatment methods. The nucleation efficiency and the films structure were investigated using scanning and transmission electron microscopy and Raman spectroscopy. C2 dimer growth (CH4 and…
Individual single-wall carbon nanotubes (SWNTs) exhibited continuous-wave stimulated Raman scattering (SRS). The Raman gain is a few orders higher, and the threshold power is a few orders lower, than values ever reported for other bulk materials and is explained as the result of both the large nonlinear property and e…
The K-shell jump ratio, jump factor and the ratio of total to K-shell photoelectric cross section at K edge have been determined for Hf, Ta, Au and Pb by adopting a novel method. In this method, continuous external bremsstrahlung (EB) photons are produced in a thin nickel elemental converter by beta particles from a 9…
Poly (vinyl alcohol) (PVA) and L-lactic acid (LA) were compounded to get biodegradable polymeric film with useful mechanical, thermal, and bacteriostatic properties for possible medical or packaging applications. Samples with various concentrations of LA were prepared by using the solvent cast technique and characteri…
In this paper we discuss continuum models of phase separation in polymer solutions, with emphasis on the thermodynamic foundation of these models. We demand that these models obey a free energy dissipation relation, which in the present context plays the role of the second law of thermodynamics, since the system is is…
We correlate topography and diffraction measurements to demonstrate that grain orientation profoundly influences polishing rates in polycrystalline diamond synthesized by chemical vapor deposition. Grains oriented with {111} or {100} planes perpendicular to the surface normal polish at significantly lower rates compar…
Many years have been devoted to study the behaviour of solids submitted to impinging particles like ions or neutrons. The nuclear evaluations describe more and more accurately the various neutron–atom interactions. Anisotropic neutron–atom cross-sections are now available for many elements. Moreover, clear mathematica…
We report a rather high dependence of the dielectric permittivity on the magnetic field in La2∕3Ca1∕3MnO3. The variation is maximum at around 270K, little above the Curie temperature TC, and it reaches a 35% under only 0.5T. We attribute this phenomenon to the space-charge or interfacial polarization produced between…
Electron field emission measurements on individual carbon nanotubes (CNTs) were performed inside a transmission electron microscope. Controlled removal of carbon atoms at the tip of the CNT was realized and various tip structures were fabricated. In particular, a capped CNT was opened and an opened CNT was converted i…
In this paper, we present our work on an optical biosensor for the detection of the interaction between a DNA single strand and its complementary oligonucleotide, based on the porous silicon (PSi) microtechnology. The crucial point in this sensing device is how to make a stable and repeatable link between the DNA prob…
Aligned single-crystal WO2.9 nanowires are grown directly from tungsten substrates at high rates using a flame synthesis method. The nanowires have diameters of 20–50nm, lengths >10μm, coverage density of 109–1010cm−2, and growth rates >1μm∕min. Growth occurs by the vapor-solid mechanism, with local gas-…
The synthesis and densification of fairly dense nanocrystalline SrTiO 3 and its characterization are described in this paper in detail. Significant grain growth was avoided by the application of a two‐stage sintering process using hot pressing. High‐resolution transmission electron microscopy and electron energy loss…