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Spin-Lattice Order in Frustrated ZnCr2O4

Sungdae Ji、S.-H. Lee、C. Broholm 等 7 位作者2009-07-15Physical Review Letters

Using synchrotron x-ray and neutron diffraction, we disentangle spin-lattice order in highly frustrated ZnCr2O4 where magnetic chromium ions occupy the vertices of regular tetrahedra. Upon cooling below 12.5 K the quandary of antialigning spins surrounding the triangular faces of tetrahedra is resolved by establishing…

Magnetic and transport properties of perovskites and related materialsMultiferroics and related materialsAdvanced Condensed Matter Physics

Missing Metallofullerene with C80 Cage

Hidefumi Nikawa、Tomoya Yamada、Baopeng Cao 等 9 位作者2009-07-15Journal of the American Chemical Society

Many insoluble metallofullerenes are called missing metallofullerenes. These metallofullerenes have not yet been isolated despite their detection in raw soot using mass spectrometry. They have been anticipated to show unique structures and properties that differ considerably from those of soluble metallofullerenes. He…

Advanced Chemical Physics StudiesGraphene research and applicationsFullerene Chemistry and Applications

Xenogenic Transplantation of Human Mesenchymal Stem Cells in a Critical Size Defect of the Sheep Tibia for Bone Regeneration

Philipp Niemeyer、Thomas Schönberger、Joachim Hahn 等 9 位作者2009-07-15Tissue Engineering Part A

Mesenchymal stem cells (MSCs) represent an attractive cell population for the regeneration of mesenchymal tissues. Their special immunological characteristics suggest that MSCs could be used in nonautologous applications. In this study, the regenerative capacity of human and ovine MSCs was assessed in an ovine critica…

Mesenchymal stem cell researchElectrospun Nanofibers in Biomedical ApplicationsTissue Engineering and Regenerative Medicine

Supersoft Elasticity in Polydomain Nematic Elastomers

John S. Biggins、M. Warner、Kaushik Bhattacharya2009-07-15Physical Review Letters

We consider the equilibrium stress-strain behavior of polydomain liquid crystal elastomers (PLCEs). We show that there is a fundamental difference between PLCEs cross-linked in the high temperature isotropic and low temperature aligned states. PLCEs cross-linked in the isotropic state then cooled to an aligned state w…

Liquid Crystal Research AdvancementsAdvanced Materials and MechanicsAdhesion, Friction, and Surface Interactions

Transmission electron microscopy investigation of CoFeB/MgO/CoFeB pseudospin valves annealed at different temperatures

S. V. Karthik、Y. K. Takahashi、Tadakatsu Ohkubo 等 6 位作者2009-07-15Journal of Applied Physics

We have investigated the microstructure and local chemistry of Ta/Ru/Ta/CoFeB/MgO/CoFeB/Ta/Ru magnetic tunnel junctions with different values of tunneling magnetoresistance (TMR) as a result of annealing at different temperatures. Annealing at 500 °C led to the templated crystallization of the amorphous CoFeB layer ha…

Magnetic properties of thin filmsZnO doping and propertiesCopper Interconnects and Reliability

Conductive oxide thin films: Model systems for understanding and controlling surface plasmon resonance

Mark D. Losego、Alina Efremenko、Crissy Rhodes 等 6 位作者2009-07-15Journal of Applied Physics

Degeneratively doped conductive oxides represent a unique host for exploring the inter-relationship between the properties of charge carriers and their collective plasmonic response. These materials often lack interband transitions that obfuscate interpretation of spectral response in elemental metals, and unlike meta…

ZnO doping and propertiesSemiconductor materials and devicesThin-Film Transistor Technologies

Emergence of noncollinear anisotropies from interfacial magnetic frustration in exchange-bias systems

E. Jiménez、J. Julio Camarero、Jordi Sort 等 9 位作者2009-07-15Physical Review B

Exchange bias, referred to the interaction between a ferromagnet (FM) and an antiferromagnet (AFM), is a fundamental interfacial magnetic phenomenon, which is key to current and future applications. The effect was discovered half a century ago, and it is well established that the spin structures at the FM/AFM interfac…

Magnetic properties of thin filmsTheoretical and Computational PhysicsMagnetic Properties and Applications

Plasmon Dispersion in Coaxial Waveguides from Single-Cavity Optical Transmission Measurements

René de Waele、Stanley P. Burgos、Albert Polman 等 4 位作者2009-07-15Nano Letters

We determine the plasmon dispersion relation in coaxial waveguides composed of a circular channel separating a metallic core and cladding. Optical transmission measurements are performed on isolated coaxial nanoapertures fabricated on a Ag film using focused ion-beam lithography. The dispersion depends strongly on the…

Gold and Silver Nanoparticles Synthesis and ApplicationsPlasmonic and Surface Plasmon ResearchPhotonic and Optical Devices

Ice friction: The effects of surface roughness, structure, and hydrophobicity

Anne‐Marie Kietzig、Savvas G. Hatzikiriakos、Peter Englezos2009-07-15Journal of Applied Physics

The effect of surface roughness, structure, and hydrophobicity on ice friction is studied systematically over a wide range of temperature and sliding speeds using several metallic interfaces. Hydrophobicity in combination with controlled roughness at the nanoscale is achieved by femtosecond laser irradiation to mimic…

Surface Modification and SuperhydrophobicityAdhesion, Friction, and Surface InteractionsWinter Sports Injuries and Performance

Modeling of Set/Reset Operations in NiO-Based Resistive-Switching Memory Devices

C. Cagli、F. Nardi、Daniele Ielmini2009-07-15IEEE Transactions on Electron Devices

Resistive-switching memory (RRAM) devices are attracting a considerable interest in view of their back-end integration, fast programming, and high scalability. Prediction of the programming voltages and currents as a function of the operating conditions is an essential task for developing compact and numerical models…

Advanced Memory and Neural ComputingTransition Metal Oxide NanomaterialsFerroelectric and Negative Capacitance Devices

One-Dimensional CdS/α-Fe2O3 and CdS/Fe3O4 Heterostructures: Epitaxial and Nonepitaxial Growth and Photocatalytic Activity

Le Wang、Hongwei Wei、Yingju Fan 等 5 位作者2009-07-15The Journal of Physical Chemistry C

One-dimensional (1D) heterostructures of uniform CdS nanowires separately decorated with hematite (α-Fe 2 O 3 ) nanoparticles or magnetite (Fe 3 O 4 ) microspheres were successfully synthesized via a two-step solvothermal deposition method. Each CdS nanowire had a uniform diameter of 40−50 nm and a length ranging from…

Quantum Dots Synthesis And PropertiesIron oxide chemistry and applicationsCopper-based nanomaterials and applications

Characteristics of InAs/GaNAs strain-compensated quantum dot solar cell

Yoshitaka Okada、Ryuji Oshima、Ayami Takata2009-07-15Journal of Applied Physics

We have fabricated and compared the performance of GaAs-based p-i-n quantum dot solar cells with ten multilayer stacked structures of self-assembled InAs quantum dots embedded with GaNxAs1−x strain-compensating spacer layers. Reducing the thickness of the spacer layer, and hence increasing the nitrogen composition in…

Semiconductor Quantum Structures and DevicesQuantum Dots Synthesis And PropertiesAdvanced Semiconductor Detectors and Materials

Direct evidence for a dry molten globule intermediate during the unfolding of a small protein

Santosh Kumar Jha、Jayant B. Udgaonkar2009-07-15Proceedings of the National Academy of Sciences

Little is known about how proteins begin to unfold. In particular, how and when water molecules penetrate into the protein interior during unfolding, thereby enabling the dissolution of specific structure, is poorly understood. The hypothesis that the native state expands initially into a dry molten globule, in which…

Protein Structure and DynamicsProteins in Food SystemsEnzyme Structure and Function

Gold Nanoparticles Functionalized with Gadolinium Chelates as High-Relaxivity MRI Contrast Agents

Loïck Moriggi、Caroline Cannizzo、Eddy Dumas 等 6 位作者2009-07-15Journal of the American Chemical Society

Water-dispersible gold nanoparticles functionalized with paramagnetic gadolinium have been fully characterized, and the NMRD profiles show very high relaxivities up to 1.5 T. Characterization using TEM images and dynamic light scattering indicate a particle size distribution from 2 to 15 nm. The gold cores of the nano…

Advanced MRI Techniques and ApplicationsLanthanide and Transition Metal ComplexesMRI in cancer diagnosis

Design Methodology for a Miniaturized Frequency Selective Surface Using Lumped Reactive Components

Hui Lai Liu、Kenneth Lee Ford、R.J. Langley2009-07-15IEEE Transactions on Antennas and Propagation

The design methodology is described for a miniaturized frequency selective surface (FSS) using lumped reactive components. Capacitive and inductive elements are utilized in metallic patches to create current loops similar to that observed in bandpass aperture type FSS. It is shown that the resonant frequency of the FS…

Antenna Design and AnalysisMetamaterials and Metasurfaces ApplicationsAdvanced Antenna and Metasurface Technologies

Transferrin as a Luminal Target for Negatively Charged Liposomes in the Inflamed Colonic Mucosa

Boaz Tirosh、Nadine Khatib、Yechezkel Barenholz 等 5 位作者2009-07-15Molecular Pharmaceutics

The need for improved specificity in the local treatment of inflammatory bowel diseases (IBD) led us to use negatively charged liposomes to target the inflamed colonic epithelium. The purpose of the present study was to elucidate the cause for our previous observations that such liposomes accumulate, preferentially, i…

Nanoparticle-Based Drug DeliveryDrug Transport and Resistance MechanismsInfant Nutrition and Health

Photocurrent transients in all-polymer solar cells: Trapping and detrapping effects

Christopher R. McNeill、Inchan Hwang、Neil C. Greenham2009-07-15Journal of Applied Physics

We have studied photocurrent transients in all-polymer bulk-heterojunction solar cells based on poly(3-hexylthiophene) and poly((9,9-dioctylfluorene)-2,7-diyl-alt-[4,7-bis(3-hexylthien-5-yl)-2,1,3-benzothiadiazole]-2′,2″-diyl). By illuminating devices with square pulses of light of varying intensity, we reveal nonline…

Organic Electronics and PhotovoltaicsThin-Film Transistor TechnologiesConducting polymers and applications

Nanofluidic Diodes Based on Nanotube Heterojunctions

Ruoxue Yan、Wenjie Liang、Rong Fan 等 4 位作者2009-07-15Nano Letters

The mechanism of tuning charge transport in electronic devices has recently been implemented into the nanofluidic field for the active control of ion transport in nanoscale channels/pores. Here we report the first synthesis of longitudinal heterostructured SiO(2)/Al(2)O(3) nanotubes. The ionic transport through these…

Graphene research and applicationsSemiconductor materials and devicesNanopore and Nanochannel Transport Studies

Gas diffusion ultrabarriers on polymer substrates using Al2O3 atomic layer deposition and SiN plasma-enhanced chemical vapor deposition

P. F. Carcia、R. Scott McLean、Markus D. Groner 等 5 位作者2009-07-15Journal of Applied Physics

Thin films grown by Al2O3 atomic layer deposition (ALD) and SiN plasma-enhanced chemical vapor deposition (PECVD) have been tested as gas diffusion barriers either individually or as bilayers on polymer substrates. Single films of Al2O3 ALD with thicknesses of ≥10 nm had a water vapor transmission rate (WVTR) of ≤5×10…

Semiconductor materials and devicesThin-Film Transistor TechnologiesCopper Interconnects and Reliability

gem -Dichlorocyclopropanes as Abundant and Efficient Mechanophores in Polybutadiene Copolymers under Mechanical Stress

Jeremy M. Lenhardt、Ashley L. Black、Stephen L. Craig2009-07-15Journal of the American Chemical Society

When gem-dichlorocyclopropane (gDCC) copolymers derived from polybutadiene are subjected to ultrasonication, the gDCCs undergo ring opening to form 2,3-dichloroalkenes. The reactivity is not observed in low-molecular-weight (6.5 kDa) copolymers or side-chain gDCCs, consistent with mechanically induced reactivity due t…

Carbon Nanotubes in CompositesForce Microscopy Techniques and ApplicationsMechanical and Optical Resonators