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Spin glass phase in the four-state three-dimensional Potts model

A. Cruz、L. A. Fernández、A. Gordillo-Guerrero 等 20 位作者2009-05-07Physical Review B

We perform numerical simulations, including parallel tempering, a four-state Potts glass model with binary random quenched couplings using the JANUS application-oriented computer. We find and characterize a glassy transition, estimating the critical temperature and the value of the critical exponents. Nevertheless, th…

Material Dynamics and PropertiesTheoretical and Computational PhysicsComplex Systems and Time Series Analysis

High-yield kraft pulping of Eucalyptus grandis Hill ex Maiden biotreated by Ceriporiopsis subvermispora under two different culture conditions

Marcos Paulo Vicentim、Robson de Almeida Faria、André Ferraz2009-05-07Holzforschung

Abstract In the present study, it was evaluated how two different culture conditions for the biotreatment of Eucalyptus grandis by Ceriporiopsis subvermispora affect a subsequent high-yield kraft pulping process. Under the varied culture conditions investigated, different extracellular enzyme activities were observed.…

Advanced Cellulose Research StudiesEnzyme-mediated dye degradationLignin and Wood Chemistry

ThePseudomonas aeruginosa liuE gene encodes the 3-hydroxy-3-methylglutaryl coenzyme A lyase, involved in leucine and acyclic terpene catabolism

Mauricio Chávez-Avilés、Alma Laura Díaz-Pérez、Homero Reyes de la Cruz 等 4 位作者2009-05-07FEMS Microbiology Letters

The enzymes involved in the catabolism of leucine are encoded by the liu gene cluster in Pseudomonas aeruginosa PAO1. A mutant in the liuE gene (ORF PA2011) of P. aeruginosa was unable to utilize both leucine/isovalerate and acyclic terpenes as the carbon source. The liuE mutant grown in culture medium with citronello…

Microbial Natural Products and BiosynthesisEnzyme Structure and FunctionPlant biochemistry and biosynthesis

Silicon-nitride surface passivation of submicrometer silicon waveguides for low-power optical switches

Joris Van Campenhout、William M. J. Green、Xiaoping Liu 等 6 位作者2009-05-07Optics Letters

We report on a Si(3)N(4)-based surface-passivation technique for increasing free-carrier lifetimes in submicrometer silicon-on-insulator waveguides by up to 2 orders of magnitude. The carrier lifetime was measured by injecting free carriers into a critically coupled ring resonator through photoexcitation by short pump…

Photonic and Optical DevicesSemiconductor materials and devicesSilicon Nanostructures and Photoluminescence

X-ray Crystal Analysis of a TASP: Structural Insights of a Cavitein Dimer

Jon O. Freeman、Woo Cheol Lee、M.E.P. Murphy 等 4 位作者2009-05-07Journal of the American Chemical Society

Cavitein Q4 is a template assembled synthetic protein designed for X-ray crystallographic analysis. It is based on a previous monomeric helical bundle cavitein (N1GG) that consists of four identical parallel helical peptides. Crystals that were grown in the presence of bromide ions were used to solve the initial phase…

Protein Structure and DynamicsChemical Synthesis and AnalysisEnzyme Structure and Function

Nanoaggregates from Thiophene/Phenylene Co-Oligomers

Manuela Schiek、Frank Balzer、Katharina Al‐Shamery 等 5 位作者2009-05-07The Journal of Physical Chemistry C

The growth of thiophene/phenylene cooligomers is investigated on the basal surface of muscovite mica. Both the phenyl end-capped 5,5′-di-4-biphenylyl-2,2′-bithiophene (PPTTPP) and the thienyl end-capped 4,4′-di-2,2′-bithienylbiphenyl (TTPPTT) co-oligomers form fiberlike nanostructures from molecules lying on the subst…

Organic Electronics and PhotovoltaicsConducting polymers and applicationsSynthesis and properties of polymers

Enhancement of the superconducting transition temperature in cuprate heterostructures

Lilach Goren、Ehud Altman2009-05-07Physical Review B

Is it possible to increase ${T}_{c}$ by constructing cuprate heterostructures, which combine the high pairing energy of underdoped layers with the large carrier density of proximate overdoped layers? We investigate this question within a model bilayer system using an effective theory of the doped Mott insulator. Inter…

Physics of Superconductivity and MagnetismMagnetic and transport properties of perovskites and related materialsAdvanced Condensed Matter Physics

Magnetic transitions in ultra-small nanoscopic magnetic rings: Theory and experiments

Deepak Singh、R. Krotkov、Mark Tuominen2009-05-07Physical Review B

In this paper, we report on experimental and theoretical investigations of magnetic transitions in cobalt rings of size (diameter, width and thickness) comparable to the exchange length of cobalt. Magnetization measurements and calculations were performed for two sets of magnetic ring arrays: ultra-small magnetic ring…

Magnetic properties of thin filmsMagnetic Properties and ApplicationsMagnetic Properties of Alloys

Selective enzyme impregnation of chips to reduce specific refining energy in alkaline peroxide mechanical pulping

PETER W. HART、Darrell M. Waite、Luc Thibault 等 7 位作者2009-05-07Holzforschung

Abstract Eucalyptus wood chips were impregnated with various blends of fiber modifying enzymes prior to preconditioning refiner chemical-alkaline peroxide mechanical pulp processing. The process includes chemical pretreatment and two stages of refining. The energy consumption was compared at the same Canadian standard…

Biofuel production and bioconversionAdvanced Cellulose Research StudiesLignin and Wood Chemistry

Production, characterization and properties of chloridized mesoporous activated carbon from waste tyres

Jianzhong Zhu、Buchang Shi、Jianguo Zhu 等 7 位作者2009-05-07Waste Management & Research The Journal for a Sustainable Circular Economy

In this study, chloridized mesoporous activated carbons (ClMAC) were prepared from used tyres. Their pore structure, surface chemistry and adsorptive capacities of toluene were investigated with nitrogen gas adsorption, Fourier transform infrared spectroscopy (FT-IR) and bench adsorptive experiments. A series of activ…

Adsorption and biosorption for pollutant removalMetal-Organic Frameworks: Synthesis and ApplicationsCatalytic Processes in Materials Science

Penetration depth, multiband superconductivity, and absence of muon-induced perturbation in superconducting PrOs4Sb12

Lei Shu、D. E. MacLaughlin、W. P. Beyermann 等 11 位作者2009-05-07Physical Review B

Transverse-field muon spin rotation $(\text{TF-}\ensuremath{\mu}\text{SR})$ experiments in the heavy-fermion superconductor ${\text{PrOs}}_{4}{\text{Sb}}_{12}({T}_{c}=1.85\text{ }\text{K})$ suggest that the superconducting penetration depth $\ensuremath{\lambda}(T)$ is temperature independent at low temperatures, cons…

Physics of Superconductivity and MagnetismRare-earth and actinide compoundsIron-based superconductors research

Tokamak plasma self-organization and the possibility to have the peaked density profile in ITER

K. A. Razumova、В. Ф. Андреев、A. Ya. Kislov 等 13 位作者2009-05-07Nuclear Fusion

The self-organization of a tokamak plasma is a fundamental turbulent plasma phenomenon, which leads to the formation of a self-consistent pressure profile. This phenomenon has been investigated in several tokamaks with different methods of heating. It is shown that the normalized pressure profile has a universal shape…

Magnetic confinement fusion researchLaser-Plasma Interactions and DiagnosticsFusion materials and technologies

Collagen mRNA levels changes during colorectal cancer carcinogenesis

Hanne Skovbjerg、Dorit Anthonsen、Inger Marie Bowitz Lothe 等 6 位作者2009-05-07BMC Cancer

BACKGROUND: Invasive growth of epithelial cancers is a complex multi-step process which involves dissolution of the basement membrane. Type IV collagen is a major component in most basement membranes. Type VII collagen is related to anchoring fibrils and is found primarily in the basement membrane zone of stratified e…

Cell Adhesion Molecules ResearchConnective tissue disorders researchCollagen: Extraction and Characterization

Nuclear Spin‐Noise Spectra of Hyperpolarized Systems

Hervé Desvaux、Denis Marion、Gaspard Huber 等 4 位作者2009-05-07Angewandte Chemie International Edition

Spin-noise appeal: Detection of NMR spin-noise is very appealing when dilute hyperpolarized species are considered. Continuous monitoring of the noise absorption at the Larmor frequency enables determination of T(1) and T(2)*, independently of the static magnetic field. An inductively coupled microcoil located inside…

Advanced NMR Techniques and ApplicationsSolid-state spectroscopy and crystallographyAtomic and Subatomic Physics Research

Structural Characterization and Remarkable Axial Ligand Effect on the Nucleophilic Reactivity of a Nonheme Manganese(III)–Peroxo Complex

Jamespandi Annaraj、Jaeheung Cho、Yong‐Min Lee 等 7 位作者2009-05-07Angewandte Chemie

Abstract Seitlich angedockt: In dem Mangan(III)‐Komplex 1 mit einem 13‐gliedrigen makrocyclischen Liganden ist ein Peroxoligand durch Side‐on‐η2‐Koordination gebunden. Die Reaktivität von 1 wird durch Einführung anionischer Liganden in trans‐Stellung zur Peroxogruppe beeinflusst. Elektronische und strukturelle Änderun…

Magnetism in coordination complexesPorphyrin and Phthalocyanine ChemistryMetal-Catalyzed Oxygenation Mechanisms

Critical charge dynamics of superconducting La2−xSrxCuO4 thin films probed by complex microwave spectroscopy: Anomalous changes of the universality class by hole doping

T. Ohashi、Haruhisa Kitano、I. Tsukada 等 4 位作者2009-05-07Physical Review B

We study the critical charge dynamics of the superconducting to the normal-state transition for ${\text{La}}_{2\ensuremath{-}x}{\text{Sr}}_{x}{\text{CuO}}_{4}$ (LSCO) thin films with a wide range of the Sr concentration by measuring the frequency-dependent excess parts of the complex microwave conductivity, which is i…

Physics of Superconductivity and MagnetismAdvanced Condensed Matter PhysicsIron-based superconductors research

Chemical Reactions in 2D: Self-Assembly and Self-Esterification of 9(10),16-Dihydroxypalmitic Acid on Mica Surface

José A. Heredia‐Guerrero、Miguel A. San‐Miguel、Mark S.P. Sansom 等 5 位作者2009-05-07Langmuir

9(10),16-Dihydroxypalmitic acid (diHPA) is a particularly interesting polyhydroxylated fatty acid (1) because it is the main monomer of cutin, the most abundant biopolyester in nature, and (2) because the presence of a terminal and a secondary hydroxyl group in midchain positions provides an excellent model to study t…

Mesoporous Materials and CatalysisAnalytical Chemistry and ChromatographyCrystallization and Solubility Studies

Nedd4-2–Mediated Ubiquitination Facilitates Processing of Surfactant Protein–C

Juliana J. Conkright、Karen S. Apsley、Emily P. Martin 等 8 位作者2009-05-07American Journal of Respiratory Cell and Molecular Biology

We previously proposed a model of surfactant protein (SP)-C biosynthesis in which internalization of the proprotein from the limiting membrane of the multivesicular body to internal vesicles represents a key step in the processing and secretion of SP-C. To test this hypothesis, alanine mutagenesis of the N-terminal pr…

Epigenetics and DNA MethylationUbiquitin and proteasome pathwaysSupramolecular Self-Assembly in Materials

Synthesis, Structure, Conductivity, and Calculated Nonlinear Optical Properties of Two Novel Bis(triphenylphosphane)copper(I) Dithiocarbamates

Abhinav Kumar、H. Mayer‐Figge、William S. Sheldrick 等 4 位作者2009-05-07European Journal of Inorganic Chemistry

Abstract A centrosymmetric binuclear [{Cu(PPh3)2}2(piperzdtc)] (1) [piperzdtc2– = piperazinebis(dithiocarbamate)] and another mononuclear [{Cu(PPh3)2}(BzMedtc)] (2) (BzMedtc– = N‐benzyl‐N‐methyldithiocarbamate) complex have been synthesized and characterized by elemental analyses, IR, 1H, 13C, and 31P NMR spectroscopy…

Crystal structures of chemical compoundsOrganic and Molecular Conductors ResearchOrganometallic Compounds Synthesis and Characterization

Local structure of reaction intermediates probed by time-resolved x-ray absorption near edge structure spectroscopy

Grigory Smolentsev、Gemma Guilera、Moniek Tromp 等 5 位作者2009-05-07The Journal of Chemical Physics

A method for the analysis of time-resolved x-ray absorption near edge structure (XANES) spectra is proposed. It combines principal component analysis of the series of experimental spectra, multidimensional interpolation of theoretical XANES as a function of structural parameters, and ab initio XANES calculations. It a…

Advanced Chemical Physics StudiesX-ray Spectroscopy and Fluorescence AnalysisMachine Learning in Materials Science