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Investigation of the CuII/NCS−/dpk Reaction System in CH3OH [dpk = Di(2-pyridyl) Ketone]: Isolation, Structural Analysis and Magnetic Properties of a Dimer and a 1D Polymer with the Same Empirical Formula [Cu(NCS)2(dpk·CH3OH)]

Z.E. Serna、Roberto Cortés、M. Karmele Urtiaga 等 7 位作者2001-02-06European Journal of Inorganic Chemistry

Two polymorphous compounds with the general formula [Cu(NCS)2(dpk·CH3OH)]n (dpk = di-2-pyridyl-ketone) have been synthesised and have been characterised both structurally and magnetically. The dpk·CH3OH ligand is the result of the metal-promoted solvolysis of dpk in methanol and acts as a neutral donor. X-ray analysis…

Metal-Organic Frameworks: Synthesis and ApplicationsMetal complexes synthesis and propertiesMagnetism in coordination complexes

Growth of Ionic Crystals in Carbon Nanotubes

Mark Wilson、Paul A. Madden2001-02-06Journal of the American Chemical Society

ADVERTISEMENT RETURN TO ISSUEPREVCommunicationNEXTGrowth of Ionic Crystals in Carbon NanotubesMark Wilson and Paul A. MaddenView Author Information Physical and Theoretical Chemistry Laboratory Oxford University, South Parks Road, Oxford OX1 3QZ, U.K. Cite this: J. Am. Chem. Soc. 2001, 123, 9, 2101–2102Publication Dat…

Carbon Nanotubes in CompositesGraphene research and applicationsChemical and Physical Properties of Materials

Mössbauer, Crystallographic, and Density Functional Theoretical Investigation of the Electronic Structure of Bis-Ligated Low-Spin Iron(II) Phthalocyanines

Victor N. Nemykin、Nagao Kobayashi、Viktor Chernii 等 4 位作者2001-02-06European Journal of Inorganic Chemistry

We present the crystal structure of pcFe(4-methylpiperidine)2 as a first example of a low-spin iron(II) phthalocyanine (pc) complex bis-axially coordinated by aliphatic amines. It is shown that electronic rather than steric effects are responsible for the elongation of the Fe−N(axial) bond in pcFeL2 complexes. Using d…

Magnetism in coordination complexesPorphyrin and Phthalocyanine ChemistrySurface Chemistry and Catalysis

Tetrapyrrole Derivatives Substituted with Ferrocenylethynyl Moieties. Synthesis and Electrochemical Studies

Ka-Wo Poon、Wei Liu、Pui-Kwan Chan 等 7 位作者2001-02-06The Journal of Organic Chemistry

Up to eight redox-active ferrocenyl units have been incorporated, through the unsaturated ethynyl linkers, on the periphery of a series of cyclic tetrapyrrole derivatives including zinc(II) phthalocyanine and 2,3-naphthalocyanine, and nickel(II) meso-diphenylporphyrin. The synthesis of the former two macrocycles 4 and…

Porphyrin and Phthalocyanine ChemistryMolecular Junctions and NanostructuresFerrocene Chemistry and Applications

Crackling Noise

James P. Sethna、Karin A. Dahmen、Christopher R. Myers2001-02-06arXiv

Crackling noise arises when a system responds to changing external conditions through discrete, impulsive events spanning a broad range of sizes. A wide variety of physical systems exhibiting crackling noise have been studied, from earthquakes on faults to paper crumpling. Because these systems exhibit regular behavio…

cond-mat.dis-nnMaterials ScienceSoft Condensed Mattercond-mat.stat-mech

Possible coexistence of rotational and ferroelectric lattice distortions in rhombohedralPbZrxTi1−xO3

Marco Fornari、David J. Singh2001-02-06Physical review. B, Condensed matter

The competitions between ferroelectric and rotational instabilities in rhombohedral ${\mathrm{PbZr}}_{x}{\mathrm{Ti}}_{1\ensuremath{-}x}{\mathrm{O}}_{3}$ near $x=0.5$ are investigated using first-principles density-functional supercell calculations. As expected, we find a strong ferroelectric instability. However, we…

Ferroelectric and Piezoelectric MaterialsHigh-pressure geophysics and materialsMultiferroics and related materials

Orbital structure and magnetic ordering in layered manganites: Universal correlation and its mechanism

Satoshi Okamoto、Sumio Ishihara、Sadamichi Maekawa2001-02-06Physical review. B, Condensed matter

Correlation between orbital structure and magnetic ordering in layered manganites is examined. A level separation between the ${3d}_{{3z}^{2}\ensuremath{-}{r}^{2}}$ and ${3d}_{{x}^{2}\ensuremath{-}{y}^{2}}$ orbitals in a Mn ion is calculated in the ionic model for a large number of the compounds. It is found that the…

Magnetic and transport properties of perovskites and related materialsAdvanced Condensed Matter PhysicsElectronic and Structural Properties of Oxides

Observation of superconductivity in Y$_2$PdGe$_3$, structurally same as MgB$_2$

E. V. Sampathkumaran、Subham Majumdar2001-02-06arXiv

The results of electrical resistance (1.4 - 300 K), magnetization (2-300 K) and heat-capacity (2 - 50 K) measurements in Y$_2$PdGe$_3$, found to crystallize in a AlB$_2$-derived hexagonalstructure, are reported. The results establish that this compound is superconducting below 3 K. This obervation is interesting consi…

Materials ScienceSuperconductivity

Preparation of Monodispersed Fe−Mo Nanoparticles as the Catalyst for CVD Synthesis of Carbon Nanotubes

Yan Li、Jie Liu、Yongqian Wang 等 4 位作者2001-02-06OpenAlex

Uniform iron−molybdenum nanoparticles were prepared by thermal decomposition of metal carbonyl complexes using a mixture of long-chain carboxylic acid and long-chain amine as protective agents. The sizes of the nanoparticles can be systematically varied from 3 to 14 nm by changing the experimental conditions. High-res…

Advancements in Battery MaterialsCarbon Nanotubes in CompositesGraphene research and applications

Carbon Nanotubes as Superior Sorbent for Dioxin Removal

Richard Q. Long、Ralph T. Yang2001-02-06OpenAlex

ADVERTISEMENT RETURN TO ISSUEPREVCommunicationNEXTCarbon Nanotubes as Superior Sorbent for Dioxin RemovalRichard Q. Long and Ralph T. YangView Author Information Department of Chemical Engineering University of Michigan Ann Arbor, Michigan 48109-2136 Cite this: J. Am. Chem. Soc. 2001, 123, 9, 2058–2059Publication Date…

Carbon Nanotubes in CompositesGraphene research and applicationsNanopore and Nanochannel Transport Studies

Carrier-type reversal in Pb–Ge–Se glasses: Photopyroelectric measurements of thermal conductivity and heat capacity

J. R. Philip、R. Rajesh、Carlo Menon2001-02-05Applied Physics Letters

The thermal conductivity and heat capacity of Pb modified Ge–Se glasses, Pb20GexSe80−x (x=17–24) and PbyGe42−ySe58 (y=0–20), which exhibit carrier-type reversal from p type to n type at specific compositions, have been measured simultaneously by the photopyroelectric technique. The thermal conductivity as well as the…

Glass properties and applicationsPhase-change materials and chalcogenidesThermography and Photoacoustic Techniques

Quantum fluctuation effects on light absorption spectra of the one-dimensional extended Hubbard model

Norikazu Tomita、Keiichirō Nasu2001-02-05Physical review. B, Condensed matter

We study quantum fluctuation effects on light absorption spectra of one-dimensional (1D) interacting electron systems in the framework of the 1D extended Hubbard model. Our targets are halogen-bridged (HB) Ni(Ni-Br) complex and ${\mathrm{Sr}}_{2}{\mathrm{CuO}}_{3},$ which are typical 1D spin-density-wave or antiferrom…

Physics of Superconductivity and MagnetismMagnetism in coordination complexesOrganic and Molecular Conductors Research

Fabrication of CaS:Pb blue phosphor by incorporating dimeric Pb2+ luminescent centers

Sun Jin Yun、Yong Shin Kim、Sang‐Hee Ko Park2001-02-05Applied Physics Letters

The CaS:Pb phosphor emitting blue electroluminescence (EL) induced by dimeric Pb2+ luminescent centers was deposited using the controlled atomic layer deposition technique. The effect of the incorporation method and concentration of Pb2+ ions on the color of high luminance CaS:Pb phosphor was investigated at the depos…

Luminescence Properties of Advanced Materials

Identification of surface states on individual CdSe quantum dots by room-temperature conductance spectroscopy

Boaz Alperson、Israel Rubinstein、Gary Hodes2001-02-05Physical review. B, Condensed matter

We describe the direct observation of surface states on individual CdSe quantum dots by conductive scanning force spectroscopy at room temperature and the dependence of these states on size quantization and humidity conditions. Peaks corresponding to surface states that lie within the gap appear at both voltage polari…

Quantum Dots Synthesis And PropertiesChalcogenide Semiconductor Thin FilmsMolecular Junctions and Nanostructures

Attraction between Nanoparticles Induced by End-Grafted Homopolymers in Good Solvent

Jiunn-Ren Roan2001-02-05Physical Review Letters

The interactions between nanoparticles coated by end-grafted homopolymers of comparable size are studied using Edwards' self-consistent field (SCF) theory. The equilibrium monomer density distribution is obtained by solving the SCF equations in bispherical coordinates. It is shown that, because of the spherical geomet…

Surfactants and Colloidal SystemsPolymer Surface Interaction StudiesDendrimers and Hyperbranched Polymers

Theoretical study of the near-edge CuLx-ray absorption spectrum of copper phthalocyanine

S. Carniato、Yi Luo、Hans Ågren2001-02-05Physical review. B, Condensed matter

Copper tetraazaporphyrin is used as a model for copper phthalocyanine in theoretical simulations of the features observed at the Cu ${L}_{2,3}$ near-edge x-ray absorption spectra. Theoretical results obtained by a density-functional theory approach provided interpretations of the different features observed experiment…

Porphyrin and Phthalocyanine ChemistryElectrochemical Analysis and ApplicationsElectron and X-Ray Spectroscopy Techniques

Second-harmonic generation from silicon nanocrystals embedded in SiO2

Yongqiang Jiang、P.T. Wilson、M. C. Downer 等 5 位作者2001-02-05Applied Physics Letters

We present observations of optical second-harmonic generation (SHG) from silicon nanocrystals embedded in SiO2. SHG sensitivity to Si/SiO2 interface states, charge on the nanocrystals, and particle density gradients is demonstrated. SHG is proven to be a powerful noncontact nondestructive diagnosis tool for characteri…

Silicon Nanostructures and PhotoluminescenceSpectroscopy and Quantum Chemical StudiesSpectroscopy Techniques in Biomedical and Chemical Research

Direct Determination of Metastable Phase Diagram by Synchrotron Radiation Experiments on Undercooled Metallic Melts

Christian Notthoff、B. Feuerbacher、H. Franz 等 5 位作者2001-02-05Physical Review Letters

The phase selection process during the crystallization of undercooled metallic melts is studied in situ by combining the electromagnetic levitation technique with energy dispersive x-ray diffraction of synchrotron radiation. The crystallization of metastable bcc phase in binary Ni-V alloys was identified. A metastable…

Metallic Glasses and Amorphous AlloysSolidification and crystal growth phenomenaMetallurgical Processes and Thermodynamics

Influence of crystallite size distribution on the micro-Raman analysis of porous Si

Md. Nazrul Islam、Satyendra Kumar2001-02-05Applied Physics Letters

First-order Raman spectra from nanocrystalline semiconductors reflect the influence of crystallite sizes on the Raman shifts and line shapes. A Gaussian distribution in crystallite sizes is explicitly included to calculate the Raman spectra of porous silicon. Several porous-silicon samples were prepared using electroc…

Semiconductor materials and devicesSilicon Nanostructures and PhotoluminescenceNanowire Synthesis and Applications

Self-repair of ordered pattern of nanometer dimensions based on self-compensation properties of anodic porous alumina

Hideki Masuda、Masato Yotsuya、Mari Asano 等 7 位作者2001-02-05Applied Physics Letters

The self-repair of an ordered pattern of nanometer dimensions based on the self-compensation properties of anodic porous alumina is demonstrated. In a pretextured pattern formed on Al using the nanoindentation process with an array of convexes, the deficiency sites of the pattern were found to be compensated automatic…

Nanofabrication and Lithography TechniquesAnodic Oxide Films and NanostructuresNanoporous metals and alloys